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31.
Schomberg HH Gaskin JW Harris K Das KC Novak JM Busscher WJ Watts DW Woodroof RH Lima IM Ahmedna M Rehrah D Xing B 《Journal of environmental quality》2012,41(4):1087-1095
Interest in the use of biochar from pyrolysis of biomass to sequester C and improve soil productivity has increased; however, variability in physical and chemical characteristics raises concerns about effects on soil processes. Of particular concern is the effect of biochar on soil N dynamics. The effect of biochar on N dynamics was evaluated in a Norfolk loamy sand with and without NHNO. High-temperature (HT) (≥500°C) and low-temperature (LT) (≤400°C) biochars from peanut hull ( L.), pecan shell ( Wangenh. K. Koch), poultry litter (), and switchgrass ( L.) and a fast pyrolysis hardwood biochar (450-600°C) were evaluated. Changes in inorganic, mineralizable, resistant, and recalcitrant N fractions were determined after a 127-d incubation that included four leaching events. After 127 d, little evidence of increased inorganic N retention was found for any biochar treatments. The mineralizable N fraction did not increase, indicating that biochar addition did not stimulate microbial biomass. Decreases in the resistant N fraction were associated with the high pH and high ash biochars. Unidentified losses of N were observed with HT pecan shell, HT peanut hull, and HT and LT poultry litter biochars that had high pH and ash contents. Volatilization of N as NH in the presence of these biochars was confirmed in a separate short-term laboratory experiment. The observed responses to different biochars illustrate the need to characterize biochar quality and match it to soil type and land use. 相似文献
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Naphthenic acids are naturally-occurring, aliphatic or alicyclic carboxylic acids found in petroleum. Water used to extract bitumen from the Athabasca oil sands becomes toxic to various organisms due to the presence of naphthenic acids released from the bitumen. Natural biodegradation was expected to be the most cost-effective method for reducing the toxicity of the oil sands process water (OSPW). However, naphthenic acids are poorly biodegraded in the holding ponds located on properties leased by the oil sands companies. In the present study, chemical oxidation using ozone was investigated as an option for mitigation of this toxicity. Ozonation of sediment-free OSPW was conducted using proprietary technology manufactured by Seair Diffusion Systems Inc. Ozonation for 50min generated a non-toxic effluent (based on the Microtox bioassay) and decreased the naphthenic acids concentration by approximately 70%. After 130min of ozonation, the residual naphthenic acids concentration was 2mgl(-1): <5% of the initial concentration in the filtered OSPW. Total organic carbon did not change with 130min of ozonation, whereas chemical oxygen demand decreased by approximately 50% and 5-d biochemical oxygen demand increased from an initial value of 2mgl(-1) to a final value of 15mgl(-1). GC-MS analysis showed that ozonation resulted in an overall decrease in the proportion of high molecular weight naphthenic acids (n> or = 22). 相似文献
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Warren C Duzgoren-Aydin NS Weston J Willett KL 《Environmental monitoring and assessment》2012,184(2):1107-1119
Hurricanes are relatively frequent ecological disturbances that may cause potentially long-term impacts to the coastal environment.
Hurricane Katrina hit the Mississippi Gulf Coast in August 2005, and caused a storm surge with the potential to change the
trace element content of coastal surface sediments. In this study, surface estuarine and marine sediments were collected monthly
following the storm from ten sites along the Mississippi Gulf Coast (Mobile Bay, Grand Bay Bayous Heron and Cumbest, Pascagoula,
Ocean Springs, Biloxi Gulf, Back Biloxi Bay, Gulfport Gulf, Gulfport Courthouse Rd, and Gulfport Marina). Concentrations of
V, Cr, Mn, Fe, Co, Ni, Zn, As, Cd, and Pb were measured by inductively coupled plasma–mass spectrometry to evaluate their
temporal and spatial variations in the year following Hurricane Katrina. Sediments were characterized by pH, particle size
distribution and total carbon and nitrogen content. Trace element contents of the sediments were determined in both <2 mm
and <63 μm grain size fractions. Results revealed no significant temporal and spatial variability in trace element concentrations,
in either size fraction. Potential ecological risk of the sediments was assessed by using NOAA SQuiRTs’ guideline values;
most concentrations remained below probable adverse effects guidelines to marine organisms suggesting that trace elements
redistributed by Hurricane Katrina would not cause an adverse impact on resident organisms. Instead, the concentrations of
trace elements were site-dependent, with specific contaminants relating to the use of the area prior to Hurricane Katrina. 相似文献
37.
Maria Luisa Cohen 《The Environmentalist》1988,8(4):305-308
The Festival described in this article won the Golden Ball Award for education of the Italian Academy of Lincei. Dr Maria Luisa Cohen, the author, was honoured with the Tree of Learning Award for 1988, by the Commission on Education and Training of the IUCN, for her services to environmental education and her promotion and participation in the Festival. 相似文献
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Barry P. Rochelle M. Robbins Church Warren A. Gebert David J. Graczyk William R. Krug 《Journal of the American Water Resources Association》1988,24(1):35-41
ABSTRACT: As part of the U.S. Environmental Protection Agency's effort to determine the long-term effects of acidic deposition on surface water chemistry, annual runoff was estimated for about 1000 ungaged sites in the eastern U.S. using runoff contour maps. One concern in using contour maps was that a bias may be introduced in the runoff estimates due to the size of the 1000 ungaged sites relative to the size of the watersheds used in developing the maps. To determine if a bias was present the relationship between the annual runoff (expressed as depth) and the watershed area for the Northeast (NE) and Southern Blue Ridge Province (SBRP) was tested using five regional data bases. One short-term data base (1984 Water Year, n = 531) and two long-term data bases (1940–57, n = 134 and 1951–80, n = 342) were used in the NE. In the SBRP one short-term database (1984 Water Year, n = 531) and one long-term data base (1951–80, n = 60) were used. For the NE and the SBRP, runoff was not directly correlated with watershed area using the five regional databases. Also, runoff normalized by precipitation was not related to watershed area. 相似文献
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