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21.
Characterizing the optimal operation of photocatalytic degradation of BDE-209 by nano-sized TiO2 总被引:1,自引:0,他引:1
Ka Lai Chow Yu Bon Man Jin Shu Zheng Yan Liang Nora Fung Yee Tam Ming Hung Wong 《环境科学学报(英文版)》2012,24(9):1670-1678
Brominated flame retardants have been widely used in industry. There is a rapid growing public concern for their availabilities in the environment. Advanced oxidation process (AOP) is a promising and efficient technology which may be used to remove emerging chemicals such as brominated flame retardants. This project aims at investigating optimal operational conditions for the removal of BDE-209 using nano-scaled titanium(IV) oxide. The residual PBDE congeners after photocatalytical degradation of BDE-209 by TiO2 were analysed by gas chromatography-mass spectrometry (GC-MS). It was found that the degradability of BDE-209 by TiO2 was attributed to its photocatalytic activity but not the small size of the particles. The half-life of removing BDE-209 by TiO2 was 3.05 days under visible light. Tetra- and penta-BDEs were the major degraded products of BDE-209. Optimum conditions for photocatalytical degradation of BDE-209 was found to be at pH 12 (93% ± 1%), 5, 10, 20 mg/L (93.0% ± 1.70%, 91.6% ± 3.21%, 91.9% ± 0.952%, respectively), respectively of humic acid and in the form of anatase/rutile TiO2 (82% ± 3%). Hence, the efficiency of removing BDE-209 can be maximized while being cost effective at the said operating conditions. 相似文献
22.
Shiping Zhou Changqun Duan Wong Hang Gi Michelle Fazhong Yang Xuehua Wang 《环境科学学报(英文版)》2011,23(4):676-680
Toxicities were assessed for a pyrethroid (cypermethrin) and an organophosphate insecticide (chlorpyrifos) individually and in
combination. A series of tests were conducted on di erent responses (acute, chronic, behavioral) of earthworms of species Eisenia
fetida andrei in the ecological risk assessment of these pesticides. The results showed that the toxicity of the mixture of cypermethrin
and chlorpyrifos was significantly higher than either of these pesticides individually, especially on the earthworm’s chronic responses.
At a concentration of 5 mg/kg, the mixture caused significant reductions on the growth and reproduction rates of earthworms, but did
not cause any significant e ect when the individual was tested. The increase in toxicity of the pesticide mixture means that the use of
toxicity data obtained exclusively from single-pesticide experiments may underestimate the ecological risk of pesticides that actually
present in the field. 相似文献
23.
Environmental impact and human exposure to PCBs in Guiyu, an electronic waste recycling site in China 总被引:3,自引:0,他引:3
PCB levels in fish (collected from local rivers), atmosphere and human milk samples have been studied to determine the exposure levels of PCBs for local residents and e-waste workers in Guiyu, a major electronic waste scrapping center in China. The source appointment and correlation analyses showed that homologue composition of PCBs in 7 species of fish were consistent and similar to commercial PCBs Aroclor 1248. PCB levels in air surrounding the open burning site were significantly higher than those in residential area. Inhalation exposure contributed 27% and 93% to the total body loadings (the sum of dietary and inhalation exposure) of the local residents, and e-waste workers engaged in open burning respectively. Total PCB concentrations in human milk ranged from N.D. to 57.6 ng/g lipid, with an average of 9.50 ng/g lipid. The present results indicated that commercial PCBs derived from e-waste recycling are major sources of PCBs accumulating in different environmental media, leading to the accumulation of high chlorinated biphenyls in human beings. 相似文献
24.
Due to the favorable weather, abundant water resources and fertile soil, the area has been known as the homeland for crops and fish. However, being one of the most developed regions in China, the environmental quality of the Pearl River delta has deteriorated due to recent socio-economic changes during the past two decades. The drivers are industrialization and economic growth, population growth and agricultural development; and the pressures are water pollution which include nutrients and suspended solids, pesticides, other persistent toxic substances (PAHs and PCBs) and oil. These have imposed various impacts such as eutrophication, formation of red tides and biomagnification of organic contaminants through food chains. In response to these, regulatory measures have been established by the Environmental Protection Bureau of Guangdong Province, joining forces with environmental protection authorities in all urban cities and most counties, in addition to the Hong Kong Environmental Protection Department, to control pollution in order to prevent further environmental deterioration and economic loss. The present paper is an attempt by following the DPSIR approach promoted by the OECD in the early 1990s and further developed by IGBP LOICZ to review the environmental quality of Pearl River with emphasis on water quality and the impact of rapid socio-economic changes. 相似文献
25.
W. M. Choi C. L. Lam W. Y. Mo M. H. Wong 《Environmental science and pollution research international》2016,23(8):7186-7194
The fast growing of global aquaculture industry accompanied with increasing pressure on the supply and price of traditional feed materials (e.g., fish meal and soy bean meal). This circumstance has urged the need to search alternative sources of feed stuff. Food waste was used as feed stuff in rearing fish which possess substantial protein and lipid. Grass carp are major species reared in Hong Kong with lower nutritional requirements; it is also an ideal species for investigating the feasibility of using food waste as fish feeds for local aquaculture industry. The growth and immunity, reflected by total protein, total immunologlobulin (IgI), and nitroblue tetrazolium (NBT) activity of grass carp blood, were depressed when feeding with food waste feeds without enzymes. However, the supplementation of bromelain and papain in fish feed enhanced the efficient use of food waste by grass carp, which in turn improved the fish immunity. The present results indicated that the addition of those enzymes could enhance the feed utilization by fish and hematological parameters of grass carp, and the improvement on growth and immunity superior to the control (commercial feed) was observed with the addition of bromelain and papain supplement. Addition of 1 and 2 % mixture of bromelain and papain could significantly enhance the lipid utilization in grass carp. 相似文献
26.
John N. Kittinger Trisann M. Bambico Dwayne Minton Alyssa Miller Manuel Mejia Nahaku Kalei Bradley Wong Edward W. Glazier 《Regional Environmental Change》2016,16(2):301-313
Environmental restoration projects are commonly touted for their ecological positives, but such projects can also provide significant socioeconomic and cultural benefits to local communities. We assessed the social dimensions of a large-scale coral reef restoration project in Maunalua Bay, O‘ahu, where >1.32 million kg of invasive marine macroalgae was removed from 11 hectares (90,000 m2; 23 acres) of impacted coral reef in an urbanized setting. We interviewed 131 community stakeholders and analyzed both quantitative and qualitative data to assess human uses of the environment, assess perceptions of environmental health, and characterize social dimensions (+/?) associated with the invasive algae removal effort. Results indicate substantial direct economic benefits, including the creation of more than 60+ jobs, benefiting more than 250 individuals and 81 households. The project helped develop a skilled workforce in a local business dedicated to environmental restoration and increased the capacity of community organizations to address other threats to reefs and watersheds. Other major benefits include revitalization of Native Hawaiian cultural practices and traditions and the successful use of harvested invasive algae as compost by local farmers. Our results show the project heightened community awareness and a broader sense of stewardship in the area, creating enabling conditions for collective community action. Our findings show that restoration projects that explicitly incorporate efforts to build community awareness, involvement, and a shared responsibility for a site may ultimately create the long-term capacity for sustainable stewardship programs. We conclude by discussing lessons learned for engaging productively with communities in environmental restoration and stewardship, which remains a central focus in conservation worldwide. 相似文献
27.
Duohong Chen Xinhui Bi Jinping Zhao Laiguo Chen Jihua Tan Bixian Mai Jiamo Fu Minghung Wong 《Environmental pollution (Barking, Essex : 1987)》2009,157(3):1051-1057
Diurnal air samples were collected from the E-waste dismantling region Guiyu and the underwear industry region Chendian. This was the first report to present the diurnal variation of PBDEs in the atmosphere. The average concentrations of 11 PBDE congeners were 11,742 pg m−3 in the daytime, and 4830 pg m−3 at night in Guiyu, while the concentrations were lower in Chendian with 376 pg m−3 in the daytime, and 237 pg m−3 at night. BDE-209 accounted for 22% and 31.3% of the total PBDEs in Guiyu and Chendian, respectively. The diurnal variation trends of BDE-47, -99, -153, -183, and -209 were also analyzed in detail in the two regions. 相似文献
28.
The main objective of this study was to investigate occurrence of polycyclic aromatic hydrocarbons (PAHs) in the sources of the drinking water supply of Hong Kong. The main emphasis was on the Dongjiang River in mainland China which is the major source, supplying 80% of the total consumption in Hong Kong (the remaining 20% is obtained from rain water). Sediments were collected from four sites along the Dongjiang River and four reservoirs in Hong Kong during both the dry and wet weather seasons. The concentrations of total PAHs in the sediments ranged between 36 and 539 microg/kg dry wt. The lower levels were detected at the upstream site on the Dongjiang River and at the reservoirs in Hong Kong (44-85 microg/kg dry wt), while the mid- and downstream sites on the Dongjiang River were more polluted (588-658 microg/kg dry wt). Examination of the PAH profiles revealed that the mid- and downstream sections of the Dongjiang River contained high percentages of 4,5,6-ring PAHs, similar to the amounts of atmospheric particulate matter and road dust collected during the dry weather season from the Pearl River Delta region as reported in the literature. Seasonal changes were revealed in the reservoirs of Hong Kong, with higher PAH levels in the wet weather season than in the dry weather season. For those reservoirs in Hong Kong that store water from the Dongjiang River, a distinct seasonal pattern was also observed, namely, that under dry weather season conditions the PAHs found in the sediments were primarily from petrogenic source, while under wet weather season conditions they were from pyrolytic sources. No such pattern was detected in the reservoirs which stored only rain water. 相似文献
29.
Atmospheric visibility impairment has gained increasing concern as it is associated with the existence of a number of aerosols as well as common air pollutants and produces unfavorable conditions for observation, dispersion, and transportation. This study analyzed the atmospheric visibility data measured in urban and suburban Hong Kong (two selected stations) with respect to time-matched mass concentrations of common air pollutants including nitrogen dioxide (NO(2)), nitrogen monoxide (NO), respirable suspended particulates (PM(10)), sulfur dioxide (SO(2)), carbon monoxide (CO), and meteorological parameters including air temperature, relative humidity, and wind speed. No significant difference in atmospheric visibility was reported between the two measurement locations (p > or = 0.6, t test); and good atmospheric visibility was observed more frequently in summer and autumn than in winter and spring (p < 0.01, t test). It was also found that atmospheric visibility increased with temperature but decreased with the concentrations of SO(2), CO, PM(10), NO, and NO(2). The results showed that atmospheric visibility was season dependent and would have significant correlations with temperature, the mass concentrations of PM(10) and NO(2), and the air pollution index API (correlation coefficients mid R: R mid R: > or = 0.7, p < or = 0.0001, t test). Mathematical expressions catering to the seasonal variations of atmospheric visibility were thus proposed. By comparison, the proposed visibility prediction models were more accurate than some existing regional models. In addition to improving visibility prediction accuracy, this study would be useful for understanding the context of low atmospheric visibility, exploring possible remedial measures, and evaluating the impact of air pollution and atmospheric visibility impairment in this region. 相似文献
30.
Much progress has been made in recent years to address the estimation of summary statistics, using data that are subject to censoring of results that fall below the limit of detection (LOD) for the measuring instrument. Truncated data methods (e.g., Tobit regression) and multiple-imputation are two approaches for analyzing data results that are below the LOD. To apply these methods requires an assumption about the underlying distribution of the data. Because the log-normal distribution has been shown to fit many data sets obtained from environmental measurements, the common practice is to assume that measurements of environmental factors can be described by log-normal distributions. This article describes methods for obtaining estimates of percentiles and their associated confidence intervals when the results are log-normal and a fraction of the results are below the LOD. We present limited simulations to demonstrate the bias of the proposed estimates and the coverage probability of their associated confidence intervals. Estimation methods are used to generate summary statistics for 2,3,7,8-tetrachloro dibenzo-p-dioxin (2,3,7,8-TCDD) using data from a 2001 background exposure study in which PCDDs/PCDFs/cPCBs in human blood serum were measured in a Louisiana population. Because the congener measurements used in this study were subject to variable LODs, we also present simulation results to demonstrate the effect of variable LODs on the multiple-imputation process. 相似文献