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1.
Processes involved in uptake and release of nitrogen dioxide from soil and building stones into the atmosphere 总被引:1,自引:0,他引:1
Atmospheric NO2 was taken up by samples of various soils and building stones. The NO2 uptake rate constants were highest in soil samples taken during the summer months. However, the NO2 uptake rate constants of the soils and building stones were not significantly correlated with any of the following variables: moisture, pH, ammonium, nitrite, or nitrate. NO2 uptake by soil and stone was not abolished by autoclaving indicating a chemical uptake process. NO2 uptake by acidic and air-dry soils and stones resulted in nearly stoichiometric reduction of NO2 to NO. This reduction was enhanced by the addition of ferrous iron and was further enhanced by incubation under 1 ppmv SO2. The results suggest that NO2 reduction may be coupled to oxidation of ferrous to ferric iron which may be reduced again by atmospheric SO2 thus regenerating the ferrous iron content of the soil or stone. Conversion of NO2 to NO was not observed in neutral or/and moist soils and stones. NO2 was also taken up by purified and sterilized quartz sand moistend with water. This uptake was enhanced by addition of humic material but not by addition of bacteria which both had been extracted from genuine soil. Under most conditions, only uptake but no release of NO2 was observed. However, NO2 was released in air-dry soils that were heated to 45–65°C, or in ammonium-fertilized soil or stone that was drying up at room temperature. Under the latter conditions mimicking field practice, the NO2 release reached rates that were similar to the NO release rates. 相似文献
2.
E. Conrad Lamon Song S. Qian Daniel D. Richter 《Journal of the American Water Resources Association》2004,40(5):1219-1229
ABSTRACT: Dynamic linear models (DLM) and seasonal trend decomposition (STL) using local regression, or LOESS, were used to analyze the 50‐year time series of suspended sediment concentrations for the Yadkin River, measured at the U.S. Geological Survey station at Yadkin College, North Carolina. A DLM with constant trend, seasonality, and a log10 streamflow regressor provided the best model to predict monthly mean log10 suspended sediment concentrations, based on the forecast log likelihood. Using DLM, there was evidence (odds approximately 69:1) that the log10 streamflow versus log10 suspended sediment concentration relationship has changed, with an approximate 20 percent increase in the log10 streamflow coefficient over the period 1981 to 1996. However, sediment concentrations in the Yadkin River have decreased during the decade of the 1990s, which has been accompanied by a concomitant increase in streamflow variability. Although STL has been shown to be a versatile trend analysis technique, DLM is shown to be more suitable for discovery and inference of structural changes (trends) in the model coefficient describing the relationship between flow and sediment concentration. 相似文献
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Michael Greenberg Joanna Burger Michael Gochfeld David Kosson Karen Lowrie Henry Mayer Charles W. Powers Conrad D. Volz Vikram Vyas 《补救:环境净化治理成本、技术与工艺杂志》2005,16(1):91-105
This article discusses creating a sustainably protective engineered and human management system in perpetuity for sites with long‐lived radiological and chemical hazards. This is essential at this time because the federal government is evaluating its property as assets and attempting to reduce its holdings, while seeking to assure that health and ecosystems are not put at risk. To assist those who have a stake in the remediation, management, and stewardship of these and analogous privately owned sites, this article discusses current end‐state planning by reviewing the federal government's accelerated efforts to reduce its footprint and how those efforts relate to sustainability. The article also provides a list of questions organized around six elements of risk management and primary, secondary, and tertiary disease and injury prevention. Throughout the article, the U.S. Department of Energy (DOE) is used as an example of an organization that seeks to reduce its footprint, manage its budget, and be a steward of the sites that it is responsible for. However, the approach and questions are appropriate for land controlled by the Department of Defense (DOD), the General Services Administration (GSA), and other public and private owners of sites with residual contamination. © 2005 Wiley Periodicals, Inc. 相似文献
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This study sought to identify the primary indicators for evaluating shelter assistance following natural disasters and then to develop a shelter evaluation instrument based on these indicators. Electronic databases and the ‘grey’ literature were scoured for publications with a relation to post‐disaster shelter assistance. Indicators for evaluating such assistance were extracted from these publications. In total, 1,525 indicators were extracted from 181 publications. A preliminary evaluation instrument was designed from these 1,525 indicators. Shelter experts checked the instrument for face and content validity, and it was revised subsequently based on their input. The revised instrument comprises a version for use by shelter agencies (48 questions that assess 23 indicators) and a version for use by beneficiaries (52 questions that assess 22 indicators). The instrument can serve as a standardised tool to enable groups to gauge whether or not the shelter assistance that they supply meets the needs of disaster‐affected populations. 相似文献
6.
Miller WA Lewis DJ Pereira MD Lennox M Conrad PA Tate KW Atwill ER 《Journal of environmental quality》2008,37(5):1875-1882
A systems approach was used to evaluate environmental loading of Cryptosporidium oocysts on five coastal dairies in California. One aspect of the study was to determine Cryptosporidium oocyst concentrations and loads for 350 storm runoff samples from dairy high use areas collected over two storm seasons. Selected farm factors and beneficial management practices (BMPs) associated with reducing the Cryptosporidium load in storm runoff were assessed. Using immunomagnetic separation (IMS) with direct fluorescent antibody (DFA) analysis, Cryptosporidium oocysts were detected on four of the five farms and in 21% of storm runoff samples overall. Oocysts were detected in 59% of runoff samples collected near cattle less than 2 mo old, while 10% of runoff samples collected near cattle over 6 mo old were positive. Factors associated with environmental loading of Cryptosporidium oocysts included cattle age class, 24 h precipitation, and cumulative seasonal precipitation, but not percent slope, lot acreage, cattle stocking number, or cattle density. Vegetated buffer strips and straw mulch application significantly reduced the protozoal concentrations and loads in storm runoff, while cattle exclusion and removal of manure did not. The study findings suggest that BMPs such as vegetated buffer strips and straw mulch application, especially when placed near calf areas, will reduce environmental loading of fecal protozoa and improve stormwater quality. These findings are assisting working dairies in their efforts to improve farm and ecosystem health along the California coast. 相似文献
7.
Human exposure to dioxins through the diet in Catalonia,Spain: carcinogenic and non-carcinogenic risk 总被引:2,自引:0,他引:2
The main objectives of this study were to estimate the dietary intake of dioxins by the population of Catalonia, Spain, to determine which food groups showed the greatest contribution to this intake, and to assess the health risks potentially associated with the dietary dioxin intake. From June to August 2000, food samples were randomly acquired in seven cities of Catalonia. Dioxin concentrations were determined in 108 samples belonging to the following groups: vegetables, fruits, pulses, cereals, fish and shellfish, meats and meat products, eggs, milk and dairy products, and oils and fats. Estimates of average daily food consumption were obtained from recent studies. Total dietary intake of dioxins for the general population of Catalonia was estimated to be 95.4 pg WHO-TEQ/day (78.4 pg I-TEQ/day), with fish and shellfish (31%), diary products (25%), cereals (14%) and meat (13%) showing the greatest percentages of contribution to dioxin intake. The contribution of all the rest of food groups to the total dietary intake was under 20%. The non-carcinogenic risk index of dioxin intake through the diet was in the range 0.34-1.36, while the carcinogenic risk level was 1,360 excess cancer over a lifetime of 70 years. Our results corroborate the decreasing tendency in dietary intake of dioxins found in recent studies (2000-2001) from various countries. 相似文献
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Rising demand for product means that the recycling of materials is now more important than ever, saving a lot of energy embedded in materials, thus reducing CO2 emissions. Providing relevant information can raise the recycling efficiency, which is too low at present.A Recycling Information Matrix (RIM) concentrating on Waste Electrical and Electronic Equipment (WEEE) is suggested in order to facilitate and improve materials recycling. Each RIM focuses on a recycling target, and for each type of product a WEEE vector is constructed. The WEEE vector contains nine hexadecimal numbers where core-recycling info is stored.The WEEE vector can provide direct recycling information escorting the product. Another possibility is to individually identify every single product via RFID technology, giving the potential to look for relevant recycling information in databases. This offers the opportunity to add waste-handling information after the product has entered the market. This would be useful, for example, in tracking substances regarded as non-toxic at time of production which might later be proven to be the opposite.This paper is based on study visits at recycling facilities in Sweden and on many student EcoDesign projects including disassembly of consumer products. Research is done on a focused disassembly of dishwashers and on a polymer recycling experiment at a recycling plant for freezers and refrigerators. Possible escort memories are also studied, especially Radio Frequency Identification Devices (RFID). 相似文献