全文获取类型
收费全文 | 743篇 |
免费 | 1篇 |
国内免费 | 29篇 |
专业分类
安全科学 | 14篇 |
废物处理 | 56篇 |
环保管理 | 57篇 |
综合类 | 89篇 |
基础理论 | 130篇 |
污染及防治 | 293篇 |
评价与监测 | 85篇 |
社会与环境 | 41篇 |
灾害及防治 | 8篇 |
出版年
2023年 | 52篇 |
2022年 | 99篇 |
2021年 | 89篇 |
2020年 | 22篇 |
2019年 | 30篇 |
2018年 | 36篇 |
2017年 | 28篇 |
2016年 | 43篇 |
2015年 | 20篇 |
2014年 | 35篇 |
2013年 | 72篇 |
2012年 | 24篇 |
2011年 | 27篇 |
2010年 | 23篇 |
2009年 | 12篇 |
2008年 | 24篇 |
2007年 | 25篇 |
2006年 | 17篇 |
2005年 | 14篇 |
2004年 | 12篇 |
2003年 | 7篇 |
2002年 | 5篇 |
2001年 | 4篇 |
2000年 | 9篇 |
1999年 | 2篇 |
1998年 | 1篇 |
1995年 | 1篇 |
1994年 | 1篇 |
1993年 | 3篇 |
1992年 | 1篇 |
1991年 | 2篇 |
1989年 | 1篇 |
1988年 | 1篇 |
1986年 | 1篇 |
1984年 | 2篇 |
1983年 | 5篇 |
1982年 | 5篇 |
1981年 | 2篇 |
1979年 | 2篇 |
1978年 | 1篇 |
1977年 | 2篇 |
1976年 | 2篇 |
1975年 | 2篇 |
1974年 | 1篇 |
1970年 | 1篇 |
1969年 | 1篇 |
1967年 | 1篇 |
1966年 | 1篇 |
1964年 | 2篇 |
排序方式: 共有773条查询结果,搜索用时 203 毫秒
711.
Ahmed O. Maslat Raad Al-Hamdany Zacharia Fataftah Alaa. J. Mahrath Mahmoud J. Abussaud 《毒物与环境化学》2013,95(4-6):149-157
A number of newly synthesized phthalidylamines and o-benzoylbenzamide derivatives were evaluated for some biological activities. Synthesis was established by condensation of 3-acetoxyphthalide 1 with morpholine, piperidine, N,N-diisobutyl-N,N-dibenzylamines and piperazine, which afforded N-(3-phthalidyl)amines 3a–d, and 4 respectively, while with N,N-diisopropylamine, o-formyl-N,N-diisopropyl benzamide 5a is formed exclusively. On the other hand, the reaction of 3-acetoxy-3-phenylphthalide 2 with secondary amines afforded o-benzoylbenzamide derivatives 5b–c, 6 in a high yield. The structure of the reaction products was established from their spectral data. These products were screened for antifungal, antibacterial and genotoxic effect. It was found that all tested compounds have antifungal activity. Compounds 1, 2, 3d and 5b were found to be active against Escherichia coli, Bacillus subtilis and Staphylococcus aureus. Genotoxic effects using Ames test showed that Compounds 1 and 2 have a weak base-pair substitution mutagenicity while a clear base-pair substitution mutagenic activity was shown by 3a using TA100-strain of Salmonella typhimurium. Compound 4 showed a frameshift mutgenicity while a weak oxidative mutagenic action was revealed by 6. No change on the mutagenicity of the tested chemicals was observed after using the S9 metabolic activation system. 相似文献
712.
Seaweeds belonging to 14 different genera of Chlorophyta, Phaeophyta and Rhodophyta were analyzed to determine the levels of heavy metals in two areas of the Egyptian Red Sea coast. Among the trace metals analyzed, Mn and Zn showed the highest mass concentrations in the surface seawaters of the two studied areas. However, algae obtained from Suez area had the highest concentrations of the investigated heavy metals than those collected from Mars Alam area. Nevertheless, a high variability of the metal levels occurs among the studied algae and also between the investigated areas. Moreover, Zn was the most abundant metal in the seaweeds of the Suez area, while Pb was predominant in Mars Alam area in red and brown algae. L. farinosa had the highest average concentration factor of Zn in Suez (29161 fold), while it was 20091 fold in E. intestinalis at Mars Alam. The highest value of metal pollution index (MPI) was recoded in L. farinosa (22.0) at Suez. It represents 4.6 fold of that value recorded in L. farinosa at Mars Alam. Among green, brown and red algae in Suez, the highest values of MPI were recorded in Cladophora (mixed sub-species) and H. comuto (18.2 and 18.3), P. pavonia (16.2) and L. farinosa (22.1), respectively; while at Mars Alam, they were recorded in Cladophora (mixed sub-species) (6.6), P. pavonia (3.4) and L. farinosa (4.8), respectively. 相似文献
713.
Neeta A. Salvi Ahmed S. U. Choughuley Tulsi K. Shetty Rathin K. Bhattacharya 《毒物与环境化学》2013,95(2-4):123-131
Nitration of pyridoindoles (β‐carbolines) was carried out using different nitration methods and structural assignments of these nitro compounds were made using different spectroscopic techniques. The mutagenic activity of these nitro derivatives was studied using Salmonella typhimurium strains TA 98 NR and TA 100 NR in the absence as well as in the presence of S‐9 mix. Only trinitro derivatives were found to be highly mutagenic to strain TA 98 NR. 相似文献
714.
Residues of acenaphthylene, fluorene, anthracene, pyrene, chrysene, benzo(b)fluoranthene and benzo(k)fluoranthene were monitored in rain, soil and groundwater around Ismailia, in northeast Egypt. Residues detected in rain water in 1995 and 1996 were mainly of relatively low molecular weight. Both acenaphthylene and fluorene were detected in rain for the two consecutive years. Top soil has shown a wider spectrum and higher concentrations of (PAHs) than those detected in deep soil, rain and ground water. Only three compounds, acenaphthylene, fluorene and anthracene were detected in samples collected at 50 cm depth. While no traces of PAHs were detected at 1 m depth detectable concentrations of fluorene and anthracene were monitored in groundwater. 相似文献
715.
Zafar Fatmi Imran Naeem Abbasi Mubashir Ahmed Ambreen Kazi Fujio Kayama 《Environmental geochemistry and health》2013,35(3):341-346
Prior surveys conducted have found higher proportion of arsenic-contaminated wells in villages along river Indus in Pakistan. This study aims to determine the prevalence of arsenicosis skin lesions among population exposed to higher exposure in taluka Gambat district Khairpur in Sindh. The cross-sectional survey was conducted from August 2008 to January 2009 among 610 households. A total of 707 water sources (hand pumps/wells) were tested from the villages of union councils of Agra and Jado Wahan for arsenic levels with Quick rapid arsenic field test kits. A total of 110 households exposed to arsenic levels >50 ppb were identified. Case screening for arsenic skin lesions was performed for 610 individuals residing in these 110 high-risk households. Information regarding household and socio-demographic characteristics, height and weight measurements and arsenic exposure assessment were collected. Physical examinations by trained physicians were carried out to diagnose the arsenic skin lesions. After data cleaning, 534 individuals from all age groups were included in the final analysis which had complete exposure and outcome information. Overall prevalence of arsenicosis skin lesions was 13.5 % (72 cases). Of the 534 individuals, 490 (91.8 %) were exposed to arsenic levels of ≥100 ppb in drinking water (8.2 % to >50–99 ppb, 58.6 % to 100–299 ppb, 14.6 % to 300–399 ppb and 18 % to ≥400 ppb). Prevalence rate (per 100 population) of arsenicosis was highest at arsenic levels of 100–199 ppb (15.2 cases) followed by ≥400 ppb (13.5 cases) and 300–399 (12.8 cases). Prevalence rate was higher among females (15.2) compared to males (11.3). Our study reports arsenicosis burden due to exposure to higher arsenic levels in drinking water in Pakistan. Exposure to very high levels of arsenic in drinking water calls for urgent action along river Indus. Prevalence of skin lesions increases with increasing arsenic levels in drinking groundwater. Provision of arsenic-free drinking water is essential to avoid current and future burden of arsenicosis in Pakistan. 相似文献
716.
717.
The Chambal river, subjected to industrial and sewage pollution, was studied with reference to the benthic fauna. Twenty seven taxa of benthic fauna of four main groups were observed at the stretch of the river: Oligochaeta, Diptera, Mollusca and Insecta (“others”). It was noted that the pollution input zone shows less fauna. The analysis of various physicochemical parameters showed an increase in pollution where domestic and industrial effluent were added. Changes in the benthic community have been explained with the help of the Diversity Index. The species diversity values showed a decrease from the prepollution point to the effluent discharge channel with an increase at the posteffluent point, indicating it to be a recovery zone. The coefficient of correlation was assessed between different physicochemical and different groups of benthic fauna. 相似文献
718.
719.
Kinetic studies on the NADP-linked glutamate dehydrogenase (GDH) activity in 8 species of marine phytoplankton have been carried out. The pH optima, linearity of reactions, apparent energies of activation, and apparent K
m values for NADPH, NH
4
>+
and -ketoglutarate were determined. Based on these data, an accurate, sensitive enzyme assay procedure is presented which was successfully tested on shipboard during a recent cruise in an upwelling region. Preliminary studies on inhibition and activation of the NADP-linked GDH activity have also been carried out. In addition to NADP-linked GDH activity, NAD-linked GDH activity was discovered in certain species of phytoplankton. The possible physiological roles of NAD-and NADP-linked GDH enzymes are discussed.Contribution No. 911 from the Department of Oceanography, University of Washington. This research was supported by the National Science Foundation Grants GA-34165 and GX-33502. 相似文献
720.
Auristela Mueses Ahmed Said Mark Ross 《Journal of the American Water Resources Association》2007,43(2):473-481
Abstract: A discharge rating is a relationship between stage and discharge at a specific point in a river stream or lake outlet structure. Rating curves are useful for interpolating and perhaps extrapolating flow measurements and for use directly in storage routing models. However, rating data and stations are limited. A generalized nondimensional mathematical expression that describes the rating relation of depth and discharge has been developed and tested against observations from 46 stations in West‐Central Florida. Three approaches were tested in sequence to select the best fit. The proposed model is a log‐linear equation with zero intercept and a slope that fits more than 50% of the stations were analyzed. The model is normalized by the depth and discharge values at 10% exceedance from data published by the U.S. Geological Survey. For ungauged applications, Q10 and d10 were derived from a relationship shown to be reasonably well correlated to the watershed drainage area. The average relative error for this parameter set shows that for the flow range up to the Q10 discharge, better than 30% agreement with the USGS rating data can be expected for about 50% of the stations. Further analysis is required to determine why so many stations exhibit such similar behavior and to identify the criteria or parameters governing the differences. 相似文献