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931.
Historical changes of anthropogenic Pb pollution were reconstructed based on Pb concentrations and isotope ratios in lake and peat sediment profiles from Ny-?lesund of Arctic. The calculated excess Pb isotope ratios showed that Pb pollution largely came from west Europe and Russia. The peat profile clearly reflected the historical changes of atmospheric deposition of anthropogenic Pb into Ny-?lesund, and the result showed that anthropogenic Pb peaked at 1960s-1970s, and thereafter a significant recovery was observed by a rapid increase of (206)Pb/(207)Pb ratios and a remarkable decrease in anthropogenic Pb contents. In contrast to the peat record, the longer lake record showed relatively high anthropogenic Pb contents and a persistent decrease of (206)Pb/(207)Pb ratios within the uppermost samples, suggesting that climate-sensitive processes such as catchment erosion and meltwater runoff might have influenced the recent change of Pb pollution record in the High Arctic lake sediments. 相似文献
932.
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935.
从长期被石油污染的土壤中筛选得到一株以蒽为惟一碳源的混合菌T2,在接种量为1%,pH为7,温度为30℃,摇床转速为120r/min,蒽的初始浓度为100mg/L的条件下培养5d后,其对蒽的降解率可以达到56.6%。通过单因素实验和正交实验对菌种T2的培养条件进行研究,得到菌种T2的最佳培养条件为:接种量为5%,pH为6,温度为35℃,蒽的初始浓度为40mg/L时,最适合菌种生长。另外,菌种T2对蒽的降解动力学实验的结果表明,蒽的残留浓度Y(mg/L)与时间t(h)符合方程y=2.544e(-0.00275)t. 相似文献
936.
Zhan-Yong Wang Fan Li Zi-Qi Guo Yan Wang Shan Chen 《Journal of Polymers and the Environment》2011,19(4):827-833
A gene encoding a poly(l-lactic acid) (PLA) depolymerase from Pseudomonas sp. strain DS04-T was cloned and overexpressed in Escherichia coli. The recombinant PLA depolymerase with a molecular weight of 19.2 kDa was purified to homogeneity. The optimum pH and temperature
of the PLA depolymerase are 8.5 and 60 °C, respectively. K+, Ca2+ and Ni2+ enhance the enzyme activity, while Na+, Zn2+, Mg2+, Cu2+, Fe2+, Mn2+ and Co2+ inhibit it. The inhibition of different chemicals on the PLA depolymerase activity were examined, in which EDTA was found
to have a significantly inhibitory effect. The main degradation product of the depolymerase is identified as lactic acid monomer
by mass spectrometric analysis. Physicochemical properties, substrate specificity and sequence analysis indicated that PME
is a new type of PLA depolymerase. 相似文献
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938.
建立了2015年乌昌石区域化石燃料固定燃烧点源大气污染物(NO_x、SO_2、PM_(2.5)和PM_(10))的排放清单,并对污染物的时空分布特征进行了分析。结果表明,2015年乌昌石区域化石燃料固定燃烧点源NO_x、SO_2、PM_(2.5)和PM_(10)的年排放量分别为2.10×10~5、1.52×10~5、4.28×10~4、8.35×10~4 t。从行业上来看,电力生产与供应行业对NO_x、SO_2、PM_(2.5)和PM_(10)的贡献率最大,分别为70.78%、66.56%、51.10%、49.98%;从化石燃料上来看,煤炭对NO_x、SO_2、PM_(2.5)和PM_(10)的贡献率最大,分别为95.63%、99.84%、99.70%、99.84%;从锅炉类型上来看,煤粉炉对NO_x、SO_2、PM_(2.5)和PM_(10)的贡献率最大,分别为84.20%、85.09%、83.43%、84.06%。固定燃烧点源污染物排放呈现出明显的时间变化特征,采暖季污染物排放量明显高于非采暖季,一天中白天的污染物排放量高于夜晚。空间分布显示,大气污染物的排放源主要集中在乌鲁木齐市、五家渠市和昌吉市。 相似文献
939.
Surface ozone and some meteorological parameters were continuously measured from June 2003 to May 2004 at urban Jinan, China. The levels and variations of surface ozone were studied and the influences of meteorological parameters on ozone were analyzed. Annual and diurnal ozone variation patterns in Jinan both show a typical pattern for polluted urban areas. Daytime ozone concentrations in summer were the highest in the four seasons. However, during nighttime from 2100 to 0600 hours ozone concentrations in spring was higher than that in summer. Daily averaged ozone showed negative correlation with pressure and relative humidity and positive correlation with temperature, total solar radiation, sunshine duration and wind speed during the study period. Further studies show that, solar radiation is a primary influence factor for the daytime variations of ozone concentrations at this site; transport of pollutants by wind could enhance the pollution at this site; precipitation has a significant influence on decreasing surface ozone. A multi-day ozone episode from 16 to 21 June 2003 was observed at this site. Surface meteorological data analysis and backward trajectory computation show that the episode is associated with the influence of typhoon Soudelor, attributing to both local photochemical processes and transport of air pollutants from southeastern coastal region, especially Yangtze River Delta region. 相似文献
940.
Wenpo Shan Haixia Lu Shuying Huo Zhixin Huang Lina You 《Environmental monitoring and assessment》2010,163(1-4):337-345
A high PM10 episode observed at a coastal site nearby Shanghai during 18–19 January 2007 was analyzed in this study. The maximum hourly averaged PM10 concentrations for the 2 days were 0.58 and 0.62 mg/m3, respectively. The meteorological condition during the episode was favorable for air pollution with large-scale stagnation. There was no dispersing effect by high wind, no scavenging function by precipitation, and no diluting process by clean marine air during the episode. The trajectories for 16–19 January all came from the northern region and kept in low levels, and during the episode peak time, from the morning of 18 to the morning of 19 January, trajectories all came from the northern inland areas and had passed over the coastal region of Jiangsu province before arriving at the site. The variation of the air pollution indexes (APIs) in the cities located in the upwind direction of the site during the episode days clearly shows a process of large-scale air pollution from north to south. The liner correlation coefficient for PM10 and SO2 concentrations is 0.774 during the episode, while for PM10 and CO, it even reaches 0.995, which indicated that the high PM10 was mainly emitted from the coal burning for domestic heating in winter. Therefore, the observed episode was caused by the transport of domestic heating pollutants accumulated in the boundary layer from northern continental areas. 相似文献