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461.
基于ReaxFF力场利用LAMMPS软件建立毕兹分子(QNB)的模型,模拟微观条件下等离子体降解毕兹的反应机理.通过模拟考察300 K恒温条件下毕兹在活性粒子作用下的行为.研究表明毕兹在O自由基作用下降解主要通过苯环活化开环、羟基夺氢反应以及奎宁环中N-O键的形成3个过程,·HO2、O2、NO、NO2这4种活性粒子在模拟中基本未对毕兹分子造成任何破坏.利用ReaxFF MD分子模拟方法对常温环境下等离子体降解毕兹反应机理研究的一个尝试,可为相关的毒剂降解试验机理分析、理论研究提供一定的参考. 相似文献
462.
SMBR-IVCW系统处理高浓度综合污水 总被引:1,自引:0,他引:1
为了提高污水处理的质量和效率,将高效的生物处理技术--膜.生物反应器(SMBR)与生态净化技术--复合垂直流人工湿地(IVCW)进行有效复合而成的SMBR-IVCW复合系统应用于高浓度综合污水的高效处理与回用中.通过对不同水力负荷组合条件下SMBR-IVCW系统对污染物净化效果的比较,得到了该复合系统的较好水力组合条件.结果表明,SMBR-IVCW具有良好的净化功效及稳定性,SMBR单元在有机物的去除、硝化作用中起到主要贡献,而IVCW单元在反硝化脱氮、深度除磷等方面进一步补充,两者的有机结合能充分发挥各自的优势,并得到了较优的水力负荷组合条件:SMBR为1000L·d-1,IVCW为375mm·d~;在该条件下.SMBR-IVCW系统总停留时问为19.22h.处理后出水中CODcr、TP、NH 4-N浓度分别为11.0、0.086、0.44mg·L-1,均可达地表水环境质量Ⅲ类标准(GB 3838.2002).SMBR-IVCW系统在此类污水处理方面具有良好的潜力. 相似文献
463.
Nowadays, intensive breeding of poultry and livestock of large scale has made the treatment of its waste and wastewater an urgent
environmental issue, which motivated this study. A wetland of 688 m2 was constructed on an egg duck farm, and water hyacinth
(Eichhornia crassipes) was chosen as an aquatic plant for the wetland and used as food for duck production. The objectives of this
study were to test the role of water hyacinth in purifying nutrient-rich wastewater and its effects on the ducks’ feed intake, egg laying
performance and egg quality. This paper shows that the constructed wetland removed as much as 64.44% of chemical oxygen demand
(COD), 21.78% of total nitrogen (TN) and 23.02% of total phosphorus (TP). Both dissolved oxygen (DO) and the transparency of the
wastewater were remarkably improved, with its transparency 2.5 times higher than that of the untreated wastewater. After the ducks
were fed with water hyacinth, the average daily feed intake and the egg-laying ratio in the test group were 5.86% and 9.79% higher,
respectively, than in the control group; the di erences were both significant at the 0.01 probability level. The egg weight in the test group
was 2.36% higher than in the control group (P < 0.05), but the feed conversion ratios were almost the same. The eggshell thickness
and strength were among the egg qualities significantly increased in ducks fed with water hyacinth.We concluded that a water hyacinth
system was e ective for purifying wastewater from an intensive duck farm during the water hyacinth growing season, as harvested
water hyacinth had an excellent performance as duck feed. We also discussed the limitations of the experiment. 相似文献
464.
Bacterial diversity in activated sludge from a consecutively aerated submerged
membrane bioreactor treating domestic wastewater 总被引:1,自引:0,他引:1
DU Cheng WU Zhenbin XIAO Enrong ZHOU Qiaohong CHENG Shuiping LIANG Wei HE Feng 《环境科学学报(英文版)》2008,20(10):1210-1217
The bacterial diversity of activated sludge from submerged membrane bioreactor (SMBR) was investigated. A 16S rDNA clone library was generated, and 150 clones were screened using restriction fragment length polymorphism (RFLP). Of the screened clones, almost full-length 16S rDNA sequences of 64 clones were sequenced. Phylogenetic tree was constructed with a database containing clone sequences from this study and bacterial rDNA sequences from NCBI for identification purposes. The 90.6% of the clones were a?l... 相似文献
465.
Profiling of microbial communities in a bioreactor for treating
hydrocarbon-sulfide-containing wastewater 总被引:2,自引:0,他引:2
A technology of polymerase chain reaction-denaturing gradient gel electrophoresis(PCR-DGGE)was used to profile the structure and dynamic changes of microbial communities in a bioreactor for treating hydrocarbon-sulfide-containing(HSC)wastewater.The results showed that the heterotrophic genus of Acinetobacter and the autotrophic genera of Thiobacillus and Thiomonas could survive well in all of three operating conditions.Some special genera were also observed with changes of micro-ecoenvironment in the rea... 相似文献
466.
467.
468.
人工湿地污水处理系统中植物体系的构建与展望 总被引:2,自引:0,他引:2
植物是人工湿地系统中的重要组成成分之一,它不仅可以起到净化污水的作用,而且还为微生物提供生存环境,同时具有景观价值。因此要选择适应性强、生物量大、根系发达、具有抗逆性的植物作为湿地植物。由于陆生植物受季节影响小且易于管理,超富集植物和转基因植物具有较高的吸收、吸附和富集的作用的特点相继成为湿地系统中植物研究的热点。而且通过合理配置植物系统可以提高湿地系统净化效果。湿地植物仍存在受季节变化的影响,植物的衰退,植物收割的后续处理等问题,仍有待研究。随着对湿地植物研究的深入,人工湿地系统一定会获得更加广阔的应用前景。 相似文献
469.
Xiao WANG Fanghua HAO Xuan ZHANG Wen SUN Hongguang CHENG 《Frontiers of Environmental Science & Engineering in China》2008,2(3):318-325
Environmental risk of high sulfur gas field exploitation has become one of the hot spots of environmental management studies.
Severe gas H2S blowout accidents in recent years have shown that poor understanding and estimates of the poisonous gas movement could lead
to dangerous evacuation delays. It is important to evaluate the real concentration of H2S, especially in complex terrain. Traditional experiential models are not valid in the case of rough terrain, especially in
low-lying areas where the gas accumulates. This study, using high sulfur content gas field of Sichuan “Pu Guang gas field”
as study object and adopting objective diagnosis of wind field of land following coordinate three dimensions, applied Lagrangian
Puff Model and breaking up technique of puffs to simulate the H2S diffusion condition of blowout accidents produced in the high sulfur content gas field of complex terrain area. The results
showed that the H2S distribution did not occur mainly in low wind direction, and due to the obstruction of the mountain’s body, it accumulated
in front of mountain on produced turn over, flowed around submitted jumping type distribution. The mountain waist near the
hilltop and low hollow river valley site rapture points simulating contrast showed that the higher the rapture point, the
better the diffusing condition of pollutant, the distribution of risk sensitive point decided piping rupture environmental
risk size combining the H2S diffusion result and residential area dispersing in the study area, synthetic judge located in the high rapture point environmental
risk was smaller than the low hollow point, thus it was suggested to carryout laying of lining build of equal high line of
higher terrain. According to simulation results, the environmental risk management measures aimed at putting down adverse
effects were worked out. 相似文献
470.
Rong CHENG Jianlong WANG Weixian ZHANG 《Frontiers of Environmental Science & Engineering in China》2008,2(1):103-108
Chlorophenols (CPs), as important contaminants in groundwater, are toxic and difficult to biodegrade. Recently nanoscale zero-valent
iron received a great deal of attention because of its excellent performance in treating recalcitrant compounds. In this study,
nanoscale zero-valent iron particles were prepared using chemical reduction, and the reductive transformations of three kinds
of chlorinated phenols (2-CP, 3-CP, and 4-CP) by nanoscale zero-valent iron under different conditions were investigated.
The transformation process of the CPs was shown to be dechlorination first, then cleavage of the benzene ring. The removal
efficiency of the CPs varied as follows: 2-CP > 3-CP > 4-CP. The reactivity of CPs was associated with their energy of lowest
unoccupied molecular orbit (E
LUMO). With the increase in initial concentrations of CPs, removal efficiency decreased a little. But the quantities of CPs reduced
increased evidently. Temperature had influence on not only the removal efficiency, but also the transformation pathway. At
higher temperatures, dechlorination occurred prior to benzene ring cleavage. At lower temperatures, however, the oxidation
product was formed more easily.
__________
Translated from China Environmental Science, 2006, 26(6): 698–702 [译自: 中国环境科学] 相似文献