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171.
The effects of biofilm growth and methane gas generation on water flow in porous media were investigated in an anaerobic two-dimensional sand-filled cell. Inoculation of the lower portion of the cell with a methanogenic culture and addition of methanol to the bottom of the cell led to biomass growth and formation of a gas phase. Biomass distributions in the water and on the sand in the cell were measured by protein analysis. The biofilm distribution on sand was observed by confocal laser scanning microscopy. The formation, migration, distribution and saturation of gases in the cell were visualized by the charge-coupled device (CCD) camera. The effects of biofilm and gas generation on water flow were separated by performing one tracer test in the presence of both biofilm and a gas phase and a second tracer test after removal of the gas phase through water flushing. The results of tracer tests demonstrated that flow and transport in the two-dimensional cell were significantly affected by both gas generation and biofilm growth. Gas generated at the bottom of the cell in the biologically active zone moved upwards in discrete fingers, so that gas phase saturations (gas-filled fraction of void space) in the biologically active zone at the bottom of the cell did not exceed 40-50%, while gas accumulation at the top of the cell produced gas phase saturations as high as 80%. The greatest reductions in water phase permeability, based on measurements of reductions in water phase saturations, occurred near the top of the box as a result of the gas accumulation. In contrast the greatest reductions in permeability due to biofilm growth, based on measurements of biofilm thickness, occurred in the most biologically active zone at the bottom of the cell, where gas phase saturations were approximately 40-50%, but permeability reductions due to biofilm growth were estimated to be 80-95%. 相似文献
172.
173.
Ionic composition of TSP and PM2.5 during dust storms and air pollution episodes at Xi'an,China 总被引:1,自引:0,他引:1
Zhenxing Shen Junji Cao Richard Arimoto Zhiwei Han Renjian Zhang Yuemei Han Suixin Liu Tomoaki Okuda Shunsuke Nakao Shigeru Tanaka 《Atmospheric environment (Oxford, England : 1994)》2009,43(18):2911-2918
TSP and PM2.5 samples were collected at Xi'an, China during dust storms (DSs) and several types of pollution events, including haze, biomass burning, and firework displays. Aerosol mass concentrations were up to 2 times higher during the particulate matter (PM) events than on normal days (NDs), and all types of PM led to decreased visibility. Water-soluble ions (Na+, NH4+, K+, Mg2+, Ca2+, F?, Cl?, NO3?, and SO42?). were major aerosol components during the pollution episodes, but their concentrations were lower during DSs. NH4+, K+, F?, Cl?, NO3?, and SO42? were more abundant in PM2.5 than TSP but the opposite was true for Mg2+ and Ca2+. PM collected on hazy days was enriched with secondary species (NH4+, NO3?, and SO42) while PM from straw combustion showed high K+ and Cl?. Firework displays caused increases in K+ and also enrichments of NO3? relative to SO42?. During DSs, the concentrations of secondary aerosol components were low, but Ca2+ was abundant. Ion balance calculations indicate that PM from haze and straw combustion was acidic while the DSs samples were alkaline and the fireworks' PM was close to neutral. Ion ratios (SO42?/K+, NO3?/SO42?, and Cl?/K+) proved effective as indicators for different pollution episodes. 相似文献
174.
Jun-Ji Cao Bai-Qing Xu Jian-Qiao He Xian-Qin Liu Yong-Ming Han Ge-hui Wang Chong-shu Zhu 《Atmospheric environment (Oxford, England : 1994)》2009,43(29):4444-4452
Carbonaceous aerosol concentrations were determined for total suspended particle samples collected from Muztagh Ata Mountain in western China from December 2003 to February 2006. Elemental carbon (EC) varied from 0.004 to 0.174 μg m?3 (average = 0.055 μg m?3) while organic carbon (OC) ranged from 0.12 to 2.17 μg m?3 and carbonate carbon (CC) from below detection to 3.57 μg m?3. Overall, EC was the least abundant fraction of carbonaceous species, and the EC concentrations approached those in some remote polar areas, possibly representing a regional background. Low EC and OC concentrations occurred in winter and spring while high CC in spring and summer was presumably due to dust from the Taklimakan desert, China. OC/EC ratios averaged 10.0, and strong correlations between OC and EC in spring–winter suggest their cycles are coupled, but lower correlations in summer–autumn suggest influences from biogenic OC emissions and secondary OC formation. Trajectory analyses indicate that air transported from outside of China brings ~0.05 μg m?3 EC, ~0.42 μg m?3 OC, and ~0.10 μg m?3 CC to the site, with higher levels coming from inside China. The observed EC was within the range of loadings estimated from a glacial ice core, and implications of EC-induced warming for regional climate and glacial ice dynamics are discussed. 相似文献
175.
Incorporating layer- and local-scale heterogeneities in numerical simulation of unsaturated flow and tracer transport 总被引:1,自引:0,他引:1
Feng Pan Ming Ye Jianting Zhu Yu-Shu Wu Bill X. Hu Zhongbo Yu 《Journal of contaminant hydrology》2009,103(3-4):194-205
This study characterizes layer- and local-scale heterogeneities in hydraulic parameters (i.e., matrix permeability and porosity) and investigates the relative effect of layer- and local-scale heterogeneities on the uncertainty assessment of unsaturated flow and tracer transport in the unsaturated zone of Yucca Mountain, USA. The layer-scale heterogeneity is specific to hydrogeologic layers with layerwise properties, while the local-scale heterogeneity refers to the spatial variation of hydraulic properties within a layer. A Monte Carlo method is used to estimate mean, variance, and 5th, and 95th percentiles for the quantities of interest (e.g., matrix saturation and normalized cumulative mass arrival). Model simulations of unsaturated flow are evaluated by comparing the simulated and observed matrix saturations. Local-scale heterogeneity is examined by comparing the results of this study with those of the previous study that only considers layer-scale heterogeneity. We find that local-scale heterogeneity significantly increases predictive uncertainty in the percolation fluxes and tracer plumes, whereas the mean predictions are only slightly affected by the local-scale heterogeneity. The mean travel time of the conservative and reactive tracers to the water table in the early stage increases significantly due to the local-scale heterogeneity, while the influence of local-scale heterogeneity on travel time gradually decreases over time. Layer-scale heterogeneity is more important than local-scale heterogeneity for simulating overall tracer travel time, suggesting that it would be more cost-effective to reduce the layer-scale parameter uncertainty in order to reduce predictive uncertainty in tracer transport. 相似文献
176.
微生物絮凝剂改善城市污水厂浓缩污泥脱水性能的研究 总被引:7,自引:2,他引:5
采用酱油曲霉(Aspergillus sojae)产生的微生物絮凝剂(MBF)作为污泥絮凝脱水剂,对城市污水处理厂浓缩污泥进行调理,确定该絮凝剂对浓缩污泥脱水的处理工艺参数为:微生物絮凝液最佳投加体积为6%~8%(体积比),发挥絮凝作用的最适污泥温度为28~32℃,最适pH为6~7。经微生物絮凝剂调理的污泥在3 000 r/min离心9 min,污泥脱水率高达82.7%,滤饼含水率降低至77.3%,污泥脱水后体积减至原来的1/5左右。 相似文献
177.
178.
脉冲电晕反应器结构对乙硫醇消除效果的影响 总被引:2,自引:1,他引:1
研究了脉冲电晕等离子体反应器结构的变化对乙硫醇消除效果的影响规律。结果表明,在反应器内设置折流板,可以增加气流的湍动程度,有利于活性粒子与污染物的充分接触,从而提高消除率。高压电极间距对电晕区范围及消毒效果有较大影响,间距较小将导致各电极产生的电场相互干扰明显,消除率减小;而电极间距过大,虽然电极间电场分布相互干扰小,但是反应器内可排布的电极数减少,总电晕区减少,消除率也减小。根据实验结果,电极间距设置为50 mm比较合理。另外,在相同的电场强度和脉冲频率下,毛刺形高压电极比线电极结构能耗低,能量利用率高。 相似文献
179.
竹林土壤中甲基对硫磷降解菌的降解效果及其与土壤物理特性的关系 总被引:1,自引:0,他引:1
采用实验室控制试验研究了甲基对硫磷降解菌在竹林土壤生态系统中的降解效果及其与土壤物理特性的关系。试验结果表明,邻单胞菌(DLL-1)具有高效性,甲基对硫磷初始浓度为15 mg/kg干土,第5 d竹林土壤上、中和下层的降解率分别为88.6%、85.9%和79.2%,相应的半衰期为2.5、2.84与3.79 d。甲基对硫磷在土壤中的不同粒径范围吸附情况是不同的,从而影响DLL-1菌的降解效果,表现为土壤中粘粒含量与降解率呈显著正相关。孔隙度也是影响降解效果的一个因素,上中下3层的降解率随着孔隙度的减小而降低。 相似文献
180.
1,4-二氯苯降解菌的分离及其降解特性研究 总被引:2,自引:1,他引:1
从某污水处理曝气池的活性污泥中分离出一株能够以1,4-二氯苯为唯一碳源和能源生长的菌株DEB-1,通过形态特征和生理生化试验初步鉴定为黄杆菌属(Flavobacterium sp.)。实验结果表明,该菌株最适降解温度为32℃、最适降解pH为7.8,24 h对100 mg/L的1,4-二氯苯的降解率达94.5%。菌株DEB-1的降解谱较广,对5种氯苯类物质具有较高的降解率。并进一步研究了DEB-1的1,4-二氯苯降解酶粗酶液的性质,其最适反应温度和pH分别为30℃和8.5。对处理含氯代芳香化合物的有机废水具有一定的意义。 相似文献