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12.
Ning Zong Peili Shi Minghua Song Xianzhou Zhang Jing Jiang Xi Chai 《Environmental management》2016,57(3):531-542
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Guanglong Pang Donghui Wang Yunhong Zhang Chunyan Ma Zhengping Hao 《Frontiers of Environmental Science & Engineering》2016,10(3):447-457
MnO2 microspheres with various surface structures were prepared using the hydrothermal method, and Au/MnO2 catalysts were synthesized using the sol-gel method. We obtained three MnO2 microspheres and Au/MnO2 samples: coherent solid spheres covered with wire-like nanostructures, solid spheres with nanosheets, and hierarchical hollow microspheres with nanoplatelets and nanorods. We investigated the properties and catalytic activities of formaldehyde oxidation at room temperature. Crystalline structures of MnO2 are the main factor affecting the catalytic activities of these samples, and γ-MnO2 shows high catalytic performance. The excellent redox properties are responsible for the catalytic ability of γ-MnO2. The gold-supported interaction can change the redox properties of catalysts and accelerate surface oxygen species transition, which can account for the catalytic activity enhancement of Au/MnO2. We also studied intermediate species. The dioxymethylene (DOM) and formate species formed on the catalyst surface were considered intermediates, and were ultimately transformed into hydrocarbonate and carbonate and then decomposed into CO2. A proposed mechanism of formaldehyde oxidation over Au/MnO2 catalysts was also obtained. 相似文献
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Ambient volatile organic compounds pollution in China 总被引:1,自引:0,他引:1
Xinmin Zhang Zhigang Xue Hong Li Li Yan Yuan Yang Yi Wang Jingchun Duan Lei Li Fahe Chai Miaomiao Cheng Weiqi Zhang 《环境科学学报(英文版)》2017,29(5):69-75
Owing to rapid economic and industrial development, China has been suffering from degraded air quality and visibility. Volatile organic compounds (VOCs) are important precursors to the formation of ground-level ozone and hence photochemical smog. Some VOCs adversely affect human health. Therefore, VOCs have recently elicited public concern and given new impetus to scientific interest. China is now implementing a series of polices to control VOCs pollution. The key to formulating policy is understanding the ambient VOCs pollution status. This paper mainly analyzes the species, levels, sources, and spatial distributions of VOCs in ambient air. The results show that the concentrations of ambient VOCs in China are much higher than those of developed countries such as the United States and Japan, especial benzene, which exceeds available standards. At the same time, the ozone formation potential (OFP) and secondary organic aerosol formation potential (SOAFP) of various VOCs are calculated. Aromatics and alkenes have much higher OFPs, while aromatics have higher SOAFP. The OFPs of ambient VOCs in the cities of Beijing, Guangzhou and Changchun are very high, and the SOAFP of ambient VOCs in the cities of Hangzhou, Guangzhou and Changchun are higher. 相似文献
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建筑行业作为一个高危险行业,由于作业条件、人员素质、管理水平等原因而事故频发并具有自身的事故特点.从国内外建筑行业事故类型、事故发生时间规律特点分析,探究建筑行业事故发生的内因和外因,从而为行业主管部门、安全监管部门提供一定依据以促进建筑企业生产的本质安全化. 相似文献
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浅析电子废弃物回收利用及危害解决办法 总被引:1,自引:0,他引:1
随着高科技的发展和人们需求的增长,电子产品不断推陈出新,电子废弃物成为世界上数量增长最快的垃圾."电子垃圾",主要包括各种使用后废弃的电脑、通信设备、电视机、电冰箱、洗衣机等电子电器产品.电子废弃物不规范回收处理易造成污染.电子废弃物中含有很多可回收再利用的有色金属、黑色金属、玻璃等物质.严格意义上讲,这些电子废弃物,不应称其为电子垃圾,而应称作电子旧货.伴随着电子工业的高速发展,电子废弃物污染不可避免地摆在了我们面前.电子废弃物具有危害性和可利用性. 相似文献
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Chunyan Liu Kai Wang Shixie Meng Xunhua Zheng Zaixing Zhou Shenghui Han Deli Chen Zhiping Yang 《Agriculture, ecosystems & environment》2011,140(1-2):226-233
One-year winter wheat–summer maize rotation is the most popular double cropping system in north-central China, and this highly productive system is an important source of nitrous oxide (N2O) and nitric oxide (NO) emissions due to the high fertilizer N and irrigation water inputs. To sustain the high crop production and mitigate the detrimental impacts of N2O and NO emissions, improved management practices are extensively applied. The aim of this study is therefore to evaluate the effects of an improved management practice of irrigation, fertilization and crop straw on grain yield and N2O and NO emissions for a wheat–maize rotation field in northern China. Using automated and manual chamber measuring systems, we monitored N2O and NO fluxes for the conventional (CT, 2007–2008), improved (IT, 2007–2008), straw-amended (WS, 2008–2009), straw-not-amended (NS, 2008–2009), and no N-fertilizer treatments (WS–NN, 2008–2009), respectively, for one rotation-year. The grain yields were determined for CT and IT for three rotation-years (2005–2008) and for WS, NS and WS–NN for one rotation-year (2008–2009). The improved management of irrigation and fertilization reduced the annual N fertilization rate and irrigation amount by 17% and 30%, respectively; increased the maize yield by 7–14%; and significantly decreased the N2O and NO emissions by 7% (p < 0.05) and 29% (p < 0.01), respectively. The incorporation of wheat straw increased the cumulative N2O and NO emissions in the following maize season by 58% (p < 0.01) and 13%, respectively, whereas the effects of maize straw application were not remarkable. The N2O and NO emission factors of applied N were 2.32 ± 2.32% and 0.42 ± 1.69% for wheat straw and 0.67 ± 0.23% and 0.54 ± 0.15% for chemical N-fertilizers, respectively. Compared to conventional management practices using high application rates of irrigation water and chemical N-fertilizer as well as the field burning of crop straw, the improved management strategy presented here has obvious environmentally positive effects on grain yield and mitigation of N2O and NO emissions. 相似文献
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