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731.
Occurrence and removal of endocrine-disrupting chemicals in wastewater treatment plants in the Three Gorges Reservoir area, Chongqing, China 总被引:1,自引:0,他引:1
Ye X Guo X Cui X Zhang X Zhang H Wang MK Qiu L Chen S 《Journal of environmental monitoring : JEM》2012,14(8):2204-2211
Concentrations of six endocrine-disrupting compounds (EDCs), bisphenol A (BPA), estrone (E(1)), 17β-estradiol (E(2)), estriol (E(3)), 17α-ethynylestradiol (EE(2)) and diethylstilbestrol (DES), were assessed in influents, effluents and excess sludge in ten municipal wastewater treatment plants (WWTPs) in the Three Gorges Reservoir (TGR) area, Chongqing, China. Three types of activated sludge treatment processes, oxidation ditch (OD), reversed anaerobic-anoxic-oxic (rA(2)/O) technology and sequential batch reactor (SBR), were used in the surveyed WWTPs. These WWTPs were all combined landfill leachate-sewage treatment plants. All analytes were extracted by solid-phase extraction (SPE) in the dissolved phase and by accelerated solvent-based extraction (ASE) in sludge. Gas chromatography-mass spectrometry (GC-MS) was employed for the analysis of EDCs. Among these EDCs, BPA was the most frequently detected and abundant compound (100.0-10566.7 ng L(-1), 15.5-1210.7 ng L(-1) and 85.0-2470.4 ng g(-1) with respect to the influents, effluents and excess sludge samples). The greatest levels of steroidal estrogens in municipal influents were observed in E(3) which were all >100 ng L(-1), followed by E(1) (42.2-110.7 ng L(-1)) and E(2) (7.4-32.7 ng L(-1)), and in the effluents and sludge were E(1) > E(3) > E(2) which were all <31 ng L(-1) and 105 ng g(-1), respectively. Regarding synthetic estrogens, EE(2) was frequently detected in the influents, occurring below 50 ng L(-1), while DES was not detected at all. A high correlation coefficient was observed between the leachate-sludge ratio and concentrations of influent EDCs, and it was statistically significant (i.e., R > 0.65, P < 0.05), but removal efficiency of the EDCs did not show significant differences with OD, rA(2)/O and SBR processes. Furthermore, modification of treatment technology as well as operational parameters, such as hydraulic retention time (HRT), sludge retention time (SRT) and disinfection process (DP), were recommended to further eliminate the residual EDCs. 相似文献
732.
Xiaomin Gu Yong Xiao Shiyang Yin Xingyao Pan Yong Niu Jingli Shao Yali Cui Qiulan Zhang Qichen Hao 《Environmental monitoring and assessment》2017,189(10):514
In this study, the hydrochemical characteristics of shallow groundwater were analyzed to get insight into the factors affecting groundwater quality in a typical agricultural dominated area of the North China Plain. Forty-four shallow groundwater samples were collected for chemical analysis. The water type changes from Ca·Na-HCO3 type in grass land to Ca·Na-Cl (+NO3) type and Na (Ca)-Cl (+NO3+SO4) type in construction and facility agricultural land, indicating the influence of human activities. The factor analysis and geostatistical analysis revealed that the two major factors contributing to the groundwater hydrochemical compositions were the water-rock interaction and contamination from sewage discharge and agricultural fertilizers. The major ions (F, HCO3) and trace element (As) in the shallow groundwater represented the natural origin, while the nitrate and sulfate concentrations were related to the application of fertilizer and sewage discharge in the facility agricultural area, which was mainly affected by the human activities. The values of pH, total dissolved solids, electric conductivity, and conventional component (K, Ca, Na, Mg, Cl) in shallow groundwater increased from grass land and cultivated land, to construction land and to facility agriculture which were originated from the combination sources of natural processes (e.g., water-rock interaction) and human activities (e.g., domestic effluents). The study indicated that both natural processes and human activities had influences on the groundwater hydrochemical compositions in shallow groundwater, while anthropogenic processes had more contribution, especially in the reclaimed water irrigation area. 相似文献
733.
Zhihui Xiao Tingyu Cui Zhenbei Wang Yan Dang Meijie Zheng Yixinfei Lin Zilong Song Yiping Wang Chao Liu Bingbing Xu Amir Ikhlaq Jolanta Kumirska Ewa Maria Siedlecka Fei Qi 《环境科学学报(英文版)》2022,34(5):88-102
In this study,carbamazepine(CBZ) decay in solution has been studied by coupling electrocoagulation with electro-Fenton(EC-EF) with a novel P-rGO/carbon felt(CF) cathode,aiming to accelerate the in-situ generation of ·OH,instead of adding Fe2+ and H2 O2.Firstly,the fabricated P-rGO and its derived cathode were characterized by XRD,SEM,AFM,XPS and electrochemical test(EIS,CV and LSV).Secondly,it was confirmed that the performance in removal efficiency and electric ... 相似文献
734.
用同位素示踪法测定微生物的葡萄糖摄入量,可能检测废水中有毒物质的生物毒性。实验结果显示:TCC/TCS对废水处理系统中厌氧菌的葡萄糖摄入有抑制作用,其抑制率与接触剂量的对数呈线性关系,但与接触时间却没有明显的线性关系。由此可见,TCC/TCS对微生物葡萄糖摄入的影响是复杂的。当生物处理系统中的微生物未接触TCC/TCS时,10%有作用浓度(EC10)和50%有作用浓度(EC50)分别为1.71mg 相似文献
735.
福建省沿海地区海盐和大气污染物反应的致酸作用 总被引:4,自引:0,他引:4
本文着重研究福建省沿海地区盐和大气污染物反应的致酸作用,从源排放估算、致酸前体物观测、大气气溶胶组成分析、降水离子特征分析四个层次进行讨论,结果表明HCl人为排放源仅占SO2,NOs的4%;大气中活性氯;HCl最大浓度为4.23μg/m^-3,Cl2最大浓度为3.97μg.m^-3,气溶胶中Cl^-/Na^+比和降水中Cl/Na^+比背离,降水中过量氯与H浓度呈现正相关,过量氯对H浓度最大贡献达3 相似文献
736.
As human populations expand and nonhuman animals decline, understanding the interactions between people and wildlife is essential.
For endangered species, appreciating the effect of human disturbance can be important for their conservation. However, a human
disturbance angle is often absent from ecological research, despite growing evidence of the negative impact of nonfatal human
interference. Here, we monitored Hainan Eld’s deer living within a reserve and translocated animals living amongst villagers.
We show that translocated deer deviated from a crepuscular activity pattern and became increasingly nocturnal, and most active
when villagers were not. It appears that translocated deer adapted over time to human disturbance and this pattern is similar
to that of other species during periods of hunting. People do not pose an actual threat to Eld’s deer, but their presence
triggered a response akin to predator avoidance and may be interfering with broader aspects of their biology and conservation. 相似文献
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738.
739.
740.
Luo SL Chen L Chen JL Xiao X Xu TY Wan Y Rao C Liu CB Liu YT Lai C Zeng GM 《Chemosphere》2011,85(7):1130-1138
This study investigates the heavy metal-resistant bacterial endophytes of Cd-hyperaccumulator Solanum nigrum L. grown on a mine tailing by using cultivation-dependent technique. Thirty Cd-tolerant bacterial endophytes were isolated from roots, stems, and leaves of S. nigrum L. and classified by amplified ribosomal DNA-restriction analysis into 18 different types. Phylogenetic analysis based on 16S rDNA sequences showed that these isolates belonged to four groups: Actinobacteria (43%), Proteobacteria (23%), Bacteroidetes (27%) and Firmicutes (7%). All the isolates were then characterized for their plant growth promoting traits as well as their resistances to different heavy metals; and the actual plant growth promotion and colonization ability were also assessed. Four isolates were re-introduced into S. nigrum L. under Cd stress and resulted in Cd phytotoxicity decrease, as dry weights of roots increased from 55% to 143% and dry weights of above-ground from 64% to 100% compared to the uninoculated ones. The total Cd accumulation of inoculated plants increased from 66% to 135% (roots) and from 22% to 64% (above-ground) compared to the uninoculated ones. Our research suggests that bacterial endophytes are a most promising resource and may be the excellent candidates of bio-inoculants for enhancing the phytoremediation efficiency. 相似文献