全文获取类型
收费全文 | 4231篇 |
免费 | 34篇 |
国内免费 | 17篇 |
专业分类
安全科学 | 49篇 |
废物处理 | 279篇 |
环保管理 | 258篇 |
综合类 | 686篇 |
基础理论 | 873篇 |
环境理论 | 4篇 |
污染及防治 | 1475篇 |
评价与监测 | 400篇 |
社会与环境 | 248篇 |
灾害及防治 | 10篇 |
出版年
2023年 | 49篇 |
2022年 | 134篇 |
2021年 | 129篇 |
2020年 | 53篇 |
2019年 | 55篇 |
2018年 | 153篇 |
2017年 | 108篇 |
2016年 | 216篇 |
2015年 | 117篇 |
2014年 | 235篇 |
2013年 | 411篇 |
2012年 | 264篇 |
2011年 | 263篇 |
2010年 | 193篇 |
2009年 | 155篇 |
2008年 | 236篇 |
2007年 | 241篇 |
2006年 | 229篇 |
2005年 | 152篇 |
2004年 | 124篇 |
2003年 | 113篇 |
2002年 | 99篇 |
2001年 | 59篇 |
2000年 | 47篇 |
1999年 | 36篇 |
1998年 | 15篇 |
1997年 | 14篇 |
1996年 | 9篇 |
1995年 | 23篇 |
1994年 | 16篇 |
1993年 | 12篇 |
1992年 | 8篇 |
1991年 | 7篇 |
1990年 | 10篇 |
1989年 | 9篇 |
1970年 | 6篇 |
1967年 | 7篇 |
1966年 | 11篇 |
1965年 | 15篇 |
1964年 | 28篇 |
1963年 | 12篇 |
1962年 | 17篇 |
1961年 | 11篇 |
1960年 | 9篇 |
1959年 | 26篇 |
1958年 | 25篇 |
1957年 | 17篇 |
1956年 | 13篇 |
1955年 | 18篇 |
1954年 | 7篇 |
排序方式: 共有4282条查询结果,搜索用时 20 毫秒
781.
The assessment of the particulate matter (PM) levels and its constituents presented in the atmosphere is an important requirement of the air quality management and air pollution abatement. The heavy metal levels in PM10 are commonly evaluated by experimental measurements; nevertheless, the EC Directives also allow the Regional Governments to estimate the regulated metal levels (Pb in Directive 2008/50/EC and As, Ni and Cd in Directive 2004/107/EC) by objective estimation and modelling techniques. These techniques are proper alternatives to the experimental determination because the required analysis and/or the number of required sampling sites are reduced. The present work aims to estimate the annual levels of regulated heavy metals by means of multivariate linear regression (MLR) and principal component regression (PCR) at four sites in the Cantabria region (Northern Spain). Since the objective estimation techniques may only be applied when the regulated metal concentrations are below to the lower assessment threshold, a previous evaluation of the determined annual levels of heavy metals is conducted to test the fulfilment of the EC Directives requirements. At the four studied sites, the results show that the objective estimations are allowed alternatives to the experimental determination. The annual average metal concentrations are well estimated by the MLR technique in all the studied sites; furthermore, the EC quality requirements for the objective estimations are fulfilled by the developed statistical MLR models. Hence these estimations may be used by Regional Governments as a proper alternative to the experimental measurements for the regulated metal levels assessment. 相似文献
782.
Galante-Oliveira S Oliveira I Ferreira N Santos JA Pacheco M Barroso C 《Journal of environmental monitoring : JEM》2011,13(2):304-312
Nucella lapillus (dog whelk) imposex levels were assessed along the mainland Portuguese coast in 2006 and 2008 and were compared with available data from 2003 for the same area. Given that specimen size has been described as a factor inducing variation in some of the imposex assessment indices, and thus resulting in less reliable results, new monitoring and data analysis procedures are described and applied to study change of imposex levels from 2003 to 2008. A significant decline in imposex intensity was observed in the study area during the study period, and the Portuguese coast ecological status (under the terms defined by the OSPAR Commission) notably improved after 2003, confirming the effectiveness of the Regulation (EC) No. 782/2003 in reducing TBT pollution. Nevertheless, N. lapillus populations are still extensively affected by imposex, and fresh TBT inputs were detected in seawater throughout the coast in 2006. These recent inputs are attributed to vessels still carrying TBT antifoulants applied before 2003, as their presence in vessels was only forbidden in 2008. Considering that Regulation (EC) No. 782/2003 is an anticipation of the IMO global ban entered into force in September 2008, a worldwide-scale decrease in TBT pollution can be expected in the near future. 相似文献
783.
Corada-Fernández C Lara-Martín PA Candela L González-Mazo E 《Journal of environmental monitoring : JEM》2011,13(7):2010-2017
A study has been made of the presence and reactivity of the most commonly used surfactants, both anionic (linear alkylbenzene sulfonates, LAS, and alkyl ethoxysulfates, AES) and non-ionic (alcohol polyethoxylates, AEOs, and nonylphenol polyethoxylates, NPEOs), in water and surface sediments from the middle stretch of the Guadalete River in SW Spain (12 stations). Average values were between 0.1 and 3.7 mg kg(-1) in sediment, and between 0.2 and 37 μg L(-1) in water. The sorption of surfactants was dominated by hydrophobic mechanisms, so those homologues having longer alkyl chains (e.g. C(18)AEO) showed higher relative percentages and concentrations in sediments compared with water. Local and sharply higher concentrations of these compounds were observed at three sampling stations (7, 9 and 12), indicating the occurrence of wastewater discharges into the river. By analysing the distributions of different surfactant homologues and their metabolites we were able to distinguish between sewage contamination from sources discharging treated and untreated wastewaters. Upstream (stations 1-2), LAS concentrations were below 30 μg L(-1) and the composition of their degradation intermediates (sulfophenyl carboxylic acids, SPCs) (160 μg L(-1)) was dominated by short-chain homologues (C(6)-C(9)SPCs), indicating that the degradation of this surfactant is at an advanced stage. The highest concentration (487 μg L(-1)) of SPCs was detected near the effluent outlet of a sewage treatment plant (STP) (station 12). Sampling stations (7 and 9) affected by untreated wastewater discharges were the only ones showing the presence of the most reactive and biodegradable SPC isomers and homologues (e.g. C(11)SPC). Here, LAS reached the highest concentration values measured (>2 mg L(-1)), and showed a homologue distribution closer to that of commercial mixtures than LAS found at the other stations. 相似文献
784.
We report a fetus with hydrops, congenital heart disease and bilateral radioulnar synostosis caused by a novel pathogenic MECOM variant. The female fetus was referred for post-mortem examination after fetal hydrops and intrauterine death was diagnosed at 20 weeks gestation. Post-mortem examination confirmed fetal hydrops, pallor, truncus arteriosus and bilateral radioulnar synostosis. Trio whole genome sequencing analysis detected a novel de novo heterozygous pathogenic loss-of-function variant in MECOM (NM_004991), associated with a diagnosis of Radioulnar Synostosis with Amegakaryocytic Thrombocytopenia 2 (RUSAT-2). RUSAT-2 is a variable condition associated postnatally with bone marrow failure, radioulnar synostosis and congenital anomalies. RUSAT-2 is not currently associated with a prenatal phenotype or fetal demise, and was not present on diagnostic NHS prenatal gene panels at time of diagnosis. This case highlights the diagnostic value of detailed phenotyping with post-mortem examination, and of using a broad sequencing approach. 相似文献
785.
786.
Fumian Tulio Machado Ferreira Fernando César de Andrade Juliana da Silva Ribeiro Canal Natália Silva Gomes Gabriela Teixeira Lilian Borges Miagostovich Marize Pereira 《Food and environmental virology》2021,13(4):553-559
Food and Environmental Virology - Norovirus is a major cause of foodborne-associated acute gastroenteritis (AGE) outbreaks worldwide. Usually, food products are contaminated either during... 相似文献
787.
Silva Marcio Roberto Ferreira Fernando César Maranhão Adriana Gonçalves Lanzarini Natália Maria de Carvalho Castro Karina Neboo Miagostovich Marize Pereira 《Food and environmental virology》2021,13(4):528-534
Food and Environmental Virology - Enteric viruses have been described as important contaminants in fresh and ready-to-eat foods such as sandwiches, deli meat and dairy products. This is a... 相似文献
788.
The leachability of some metals (Al, As, Ba, Ca, Cr, Cu, Fe, K, Mg, Mn, Ti, Zn) from fly ashes was studied in the presence of ethylenediamine tetraacetic acid (EDTA) and naturally occurring complexing agents-humic acids (HAs). Secondary complex-forming equilibria taking place in the leachates increase significantly the leached amounts of most metals. Kinetic experiments showed that almost the whole "available" amounts of metals are leached from fly ash within a time period of several hours (mostly within 20 h), with exceptions of matrix constituents (typically aluminium), which are released more slowly. 相似文献
789.
Quantification of mass fluxes and natural attenuation rates at an industrial site with a limited monitoring network: a case study 总被引:3,自引:0,他引:3
Bockelmann A Zamfirescu D Ptak T Grathwohl P Teutsch G 《Journal of contaminant hydrology》2003,60(1-2):97-121
At many "real world" field sites, the number of available monitoring wells is limited due to economic or geological reasons. Under such restricted conditions, it is difficult to perform a reliable field investigation and to quantify primary lines of evidence for natural attenuation (NA), like the documentation of a decrease of contaminant mass flux in flow direction. This study reports the results of a groundwater investigation at a former manufactured gas plant situated in a Quaternary river valley in southwest Germany. The location, infrastructure and aquifer setting are typical of many industrial sites in Germany. Due to difficult drilling conditions (coarse glaciofluvial gravel deposits and an anthropogenic fill above the aquifer), only 12 monitoring wells were available for the investigation and localisation of the contaminant plume. These wells were situated along three control planes (CP) downgradient from the contaminant source, with four wells along each plane. Based on the sparse set of monitoring wells, field scale mass fluxes and first-order natural attenuation rate constants of benzene, toluene, ethylbenzene, and o-xylene and p-xylene (BTEX) and low molecular weight polycyclic aromatic hydrocarbons (PAH) were estimated utilizing different point scale and also a new integral investigation method. The results show that even at a heterogeneous site with a sparse monitoring network point scale investigation methods can provide reliable information on field scale natural attenuation rates, if a dependable flow model or tracer test data is available. If this information is not available, only the new integral investigation method presented can yield adequate results for the quantification of contaminant mass fluxes under sparse monitoring conditions. 相似文献
790.
Schirmer Waldir Nagel Stroparo Erivelton César Gueri Matheus Vitor Diniz Capanema Marlon André Mazur Douglas Luiz Jucá José Fernando Thomé Martins Kelly Geronazzo 《Journal of Material Cycles and Waste Management》2022,24(5):2041-2053
Journal of Material Cycles and Waste Management - Biofilters have been recognized as a key technology in the mitigation of greenhouse gases (GHG) emitted by landfills. This study aimed to evaluate... 相似文献