全文获取类型
收费全文 | 940篇 |
免费 | 44篇 |
国内免费 | 372篇 |
专业分类
安全科学 | 58篇 |
废物处理 | 55篇 |
环保管理 | 87篇 |
综合类 | 509篇 |
基础理论 | 197篇 |
污染及防治 | 311篇 |
评价与监测 | 28篇 |
社会与环境 | 34篇 |
灾害及防治 | 77篇 |
出版年
2023年 | 15篇 |
2022年 | 52篇 |
2021年 | 40篇 |
2020年 | 28篇 |
2019年 | 27篇 |
2018年 | 44篇 |
2017年 | 48篇 |
2016年 | 48篇 |
2015年 | 75篇 |
2014年 | 83篇 |
2013年 | 97篇 |
2012年 | 97篇 |
2011年 | 94篇 |
2010年 | 66篇 |
2009年 | 59篇 |
2008年 | 65篇 |
2007年 | 59篇 |
2006年 | 38篇 |
2005年 | 37篇 |
2004年 | 19篇 |
2003年 | 25篇 |
2002年 | 27篇 |
2001年 | 26篇 |
2000年 | 23篇 |
1999年 | 25篇 |
1998年 | 22篇 |
1997年 | 20篇 |
1996年 | 21篇 |
1995年 | 21篇 |
1994年 | 10篇 |
1993年 | 8篇 |
1992年 | 8篇 |
1991年 | 7篇 |
1990年 | 8篇 |
1989年 | 3篇 |
1988年 | 6篇 |
1987年 | 1篇 |
1986年 | 3篇 |
1985年 | 1篇 |
排序方式: 共有1356条查询结果,搜索用时 0 毫秒
101.
Rothenberg SE Du X Zhu YG Jay JA 《Environmental pollution (Barking, Essex : 1987)》2007,149(2):246-251
The impact of sewage irrigation on the uptake and translocation of mercury (Hg) in corn plants (Zea mays) was investigated. Corn plants were harvested the same day from two nearby fields in suburban Beijing, one irrigated historically with sewage effluent, and one irrigated solely with groundwater. Hg content was analyzed in the soil, roots and stems, while percent moisture and soil organic content were analyzed in the soil samples. The concentration of Hg in the soil and roots, and the soil organic content were not significantly different between the two fields, despite the historic practice of sewage irrigation. Hg content in roots was positively correlated with soil Hg concentration (r=0.95, n=6). The transfer coefficients between roots and stems were significantly higher in the control site (control: 2.06, sewage-irrigated: 0.44, p<0.05), indicating that the barrier effect of the roots was not consistent between the two fields. 相似文献
102.
A novel method was developed to suppress membrane fouling in submerged membrane bioreactors. The method is based on the dielectrophoretic (DEP) motion of particles in an inhomogeneous electrical field. Using a real sample of biomass as feed, the fouling-suppression performance using DEP with different electrical field intensities (60–160 V) and different frequencies (50–1000 Hz) was investigated. The fouling-suppression performance was found to relate closely with the intensity and frequency of the electrical field. A stronger electrical field was found to better recover the filtrate flux. This is because of a stronger DEP force acting on the biomass particles close to the membrane's surface. Above an intensity and frequency value of 130 V and 1 kHz, respectively the permeate flux was reduced due to an electrothermal effect. 相似文献
103.
Xinhua Wang Jingmei Li Xiufen Li Guocheng Du 《Frontiers of Environmental Science & Engineering in China》2011,5(4):615-622
Among the numerous parameters affecting the membrane bioreactor (MBR) performance, the aeration intensity is one of the most
important factors. In the present investigation, an anoxic/aerobic-type (A/O-type) sequencing batch MBR system, added anoxic
process as a pretreatment to improve the biodegradability of azo dye wastewater, was investigated under different aeration
intensities and the impact of the aeration intensity on effluent quantity, sludge properties, extracellular polymeric substances
(EPS) amount generated as well as the change of permeation flux were examined. Neither lower nor higher aeration intensities
could improve A/O-type sequencing batch MBR performances. The results showed 0.15 m3·h−1 aeration intensity was promising for treatment of azo dye wastewater under the conditions examined. Under this aeration intensity,
chemical oxygen demand (COD), ammonium nitrogen and color removal as well as membrane flux amounted to 97.8%, 96.5%, 98.7%
and 6.21 L·m−2·h−1, respectively. The effluent quality, with 25.0 mg·L−1COD, 0.84 mg·L−1 ammonium nitrogen and 8 chroma, could directly meet the reuse standard in China. In the meantime, the sludge relative hydrophobicity,
the bound EPS, soluble EPS and EPS amounts contained in the membrane fouling layer were 70.3%, 52.0 mg·g−1VSS, 38.8 mg·g−1VSS and 90.8 mg·g−1VSS, respectively, which showed close relationships to both pollutant removals and membrane flux. 相似文献
104.
105.
某湿地生态保护区水体中铜的生态风险评价及管理限值研究 总被引:1,自引:0,他引:1
铜是生物必需的微量元素,但过量暴露会对生物产生毒害效应。针对我国南方城市某湿地生态保护区水体重金属污染问题,参照《澳大利亚和新西兰淡水和海水水质指南》,应用物种敏感度分布(speeies sensitivity distribution,SSD)方法和联合概率曲线(joint probability curve,JPC)方法评价水体中铜的生态风险评价,在此基础上提出水体中铜浓度的管理限值。根据该湿地生态保护区生物调查历史数据以及其他文献数据,整理了415个本地物种的清单,通过美国环境保护署ECOTOX数据库以及其他文献共获取了13个物种的毒性数据,构建了Weibull分布、对数正态分布、正态分布、对数Logistic分布、Logistic分布、BurrⅢ型分布和Gumbel分布等7个SSD模型。结果表明,利用13个本地物种铜毒性数据构建的SSD模型具有合理性,不同模型计算得到的湿地生态保护区水体中铜的总体风险期望值为0.054~0.121。其中,BurrⅢ型分布模型的拟合效果最好,据此推导得到以保护水生生态系统为目标的铜的高可靠性与中等可靠性触发值分别为2.55μg·L~(-1)和1.41μg·L~(-1)。考虑到管理目标的可达性和现状的生态风险水平,提出该湿地生态保护区水体中铜浓度的管理限值为3μg·L~(-1)。 相似文献
106.
Dan Du 《中国人口.资源与环境(英文版)》2017,15(3):226-238
The present study aims to better understand the relationship between energy intensity and its determinants including energy price, technological progress, economic structure, and energy mix using the autoregressive distributed lag(ARDL) bounds approach and vector error correction model technique. Based on China's time series over 1985-2014, the ARDL bounds approach yields empirical evidence that confirms the existence of long run relationship between energy price, technological progress, economic structure, energy mix, and energy intensity. The results show that technological progress is an important driver for the declining energy intensity in short and long run. Energy price has not been demonstrated as an important role in decreasing energy intensity in the short run. The high share of coal use in total energy use may be responsible for China's high energy intensity.However, the relative change in economic sectors plays a minor role in energy intensity reduction during the past years. In the long run, technological progress, energy mix and energy prices Granger cause energy intensity, but not vice versa except for the energy mix. 相似文献
107.
中国大部分污水处理厂目前均采用二级处理工艺,主要去除碳源污染物,而消解氮、磷类污染物的效果较差.在传统二级处理工艺基础上,对中水进行三级深度处理,BOD5、SS以及COD类污染物去除效果明显,但运行成本较高,处理量受限.人工构造湿地利用基质-植物-微生物复合生态系统的物理、化学和生物的三重协同作用,通过过滤、吸附与沉淀等作用,以及微生物同化分解和植物吸收转化等途径,可有效去除污水中的氮、磷、SS、有机物及重金属等污染物,且具有低投资、低运转费、低维持成本等特点. 相似文献
108.
109.
The presence of Bacillus thuringiensis (Bt) protein in earthworms Eisenia fetida has no deleterious effects on their growth and reproduction 总被引:1,自引:0,他引:1
Earthworms Eisenia fetida, bred in substances with stover of two genetically-engineered Bacillus thuringiensis (Bt) corns (5422Bt1 (Event Bt11) and 5422CBCL (MON810)) expressing Cry1Ab and their near-isogenic non-Bt corn (5422), were used to investigate the non-target effects of Bt corn on soil-dwelling organisms. Cry1Ab concentrations in substances, casts and guts of E. fetida were also investigated by Enzyme-linked immunosorbent assay (ELISA). More than 90% individuals of E. fetida survived over a period of 30 d, irrespective of whether they received Bt corn or non-Bt corn. Compared to 5422 treatments, significantly higher relative growth rate and more number of new offspring and cocoons of E. fetida were found in 5422Bt1 and 5422CBCL treatments. These results were unlikely to be directly caused by Cry1Ab released from Bt corns but rather by differences in other factors of plants such as plant components (soluble sugar, total organic carbon, total protein and available phosphorus of Bt corns were more than 5422). ELISA results indicated immunoreactive Cry1Ab was detectable in substances, and the casts, guts of E. fetida from Bt corns treatments, of which the highest levels were detected in substances under the corresponding experimental conditions. With the increase of treated time, a strong decline was observed in Cry1Ab from substances and casts of E. fetida, whereas Cry1Ab in guts of E. fetida from 5422Bt1 treatments gradually increased and that from 5422CBCL treatments increased between 14 and 30 d. Therefore, the presence of Cry1Ab in E. fetida had no deleterious effects on their growth and reproduction. 相似文献
110.
Du?ica Ili? Ivan S. Risti? Ljubi?a Nikoli? Mihajlo Stankovi? Goran Nikoli? Ljiljana Stanojevi? Vesna Nikoli? 《Journal of Polymers and the Environment》2012,20(1):80-87
In this work was described poly(d,l-lactide) microwave synthesis using tin(II) 2-ethylhexanoate initiated ring-opening polymerization. Polymerization was performed
at 100 °C with monomer to initiator molar ratio ([M]/[I]) of 5,000 in 30 min. The achieved number average molar mass of obtained
polymers (determined by gel permeation chromatography) was 102,320 g/mol, with the polydispersion index, Q, 2.80. Structural characterization was performed by FT-IR spectroscopy followed characteristic bands. For applicative purposes
the obtained polymer was purified during the procedure of microsphere preparation. Biodegradable microspheres prepared from
poly(d,l-lactide) have been widely studied in recent years and have become well established controlled drug delivery systems. In this
work microspheres were loaded with allyl thiosulfinate (allicin) and its transforments products (ajoene and vinyldithiine),
as pharmacological active substances. The morphology of the microspheres was analyzed using a scanning electron microscope.
Allicin was synthesized by acid oxidation of allyl disufide and purification of obtained products by liquid–liquid extraction
with diethyl ether. Obtained allicin, purity 73%, was transformed using microwave in acetone solution, at solvent boiling
temperature, for 5 min. For the quality and quantity analysis of allicin and its transformation process was used LC/MS chromatography.
(E)- and (Z)-ajoene were detected at retention time 3.1 and 3.3 min, respectively, whence 3-vynil-4H-1,2-dithiine and 2-vynil-4H-1,3-dithiine
were detected at 4.3 and 4.8 min, respectively. Retention time of allicin was 2.93 min, according to liquid chromatography
results. HPLC method was used for assessment of pharmaceutical substances (alicine and alicine transforments) releasing from
microspheres at room temperature in solutions with different pH (pH = 3 and pH = 8) for 24 h. 相似文献