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131.
132.
Degradation of pentachlorobiphenyl by a sequential treatment using Pd coated iron and an aerobic bacterium (H1) 总被引:1,自引:0,他引:1
The reductive dechlorination and biodegradation of 2,2′4,5,5′-pentachlorobiphenyl (PCB#101) was investigated in a laboratory-scale. Palladium coated iron (Pd/Fe) was used as a catalytic reductant for the chemical degradation of 2,2′4,5,5′-pentachlorobiphenyl, and an aerobic bacteria was used for biodegradation following the chemical reaction in this study. Dechlorination was affected by several factors such as Pd loading, initial soil pH and the amount of Pd/Fe used. The results showed that higher Pd loading, higher dosage of Pd/Fe and slightly acid condition were beneficial to the catalytic dechlorination of 2,2′,4,5,5′-pentachlorobiphenyl. In laboratory batch experiments, 2,2′4,5,5′-pentachlorobiphenyl was reduced in the presence of Pd/Fe bimetal, which was not further degraded by aerobic bacteria. 2,2′,4-trichlorobiphenyl (PCB#17), a reduction product from 2,2′4,5,5′-pentachlorobiphenyl, was readily biodegraded in the presence of a aerobic bacterial strain. It is suggested that an integrated Pd/Fe catalytic reduction-aerobic biodegradation process may be a feasible option for treating PCB-contaminated soil. 相似文献
133.
通过正交试验,得到了DAT-IAT工艺和A/DAT-IAT工艺处理城市污水的常规指标去除和生态毒理指标削减的最优运行条件。结果表明,在正交试验的同一工艺中,COD去除最优运行条件的出水COD值优于生态毒性削减最优运行条件的出水COD值,但前者出水的生态毒性较大。由于厌氧池的水解酸化作用,A/DAT-IAT工艺对COD和生态毒性的处理效果均优于DAT-IAT工艺,并且回流总能耗低于DAT-IAT工艺,但是出水COD仍不达标。为了降低进入工艺的COD的总量,以絮凝沉淀做为预处理工艺,并采用Al残留量最小的絮凝剂投药量以降低出水中残留Al带来的生态风险。结果表明,在COD去除最优运行条件下,具有絮凝预处理的工艺对COD的去除效果优于没有絮凝预处理的工艺。絮凝-A/DAT-IAT工艺在COD去除最优运行条件下出水COD为104.46 mg/L,满足排放标准。在毒性削减最优运行条件下,具有絮凝预处理的工艺的出水生态毒性有所上升,但是污染物的总量得到了大幅削减。絮凝-A/DAT-IAT工艺与DAT-IAT工艺相比,在污染物去除效率得到大幅增加的同时,生态毒性得到有效控制,生态安全得到了有效的保障。 相似文献
134.
135.
传统的评价方法费时费力,效率低下.将计算机技术与评价方法相结合是评价工作发展的趋势.介绍了为世界各国石油化工企业所广为接受的美国道化学公司(DOW)火灾、爆炸危险性指数评价法,以及根据该法的评价思路所开发的辅助软件的设计思路和功能. 相似文献
136.
137.
Spatial and temporal distribution of polycyclic aromatic hydrocarbons (PAHs) in sediments of the Nansi Lake, China 总被引:2,自引:0,他引:2
Hong-Li Li Hong Gao Chen Zhu Guo-Gang Li Fan Yang Zheng-Yu Gong Jun Lian 《Environmental monitoring and assessment》2009,154(1-4):469-478
Polycyclic aromatic hydrocarbons (PAHs) were measured in surface sediments and dated core sediments from the Nansi Lake of China to investigate the spatial and temporal distribution characteristics. The concentrations of 16 kinds priority PAH compounds were determined by GC-MS method. And 210Pb isotope dating method was used to determine the chronological age of the sediment as well as the deposition rate. The results indicated that the total PAHs concentration ranges in surface and core sediment samples were 160 ~32,600 and 137 ~ 693 ng/g (dry wt.), respectively. The sediment rate and the average mass sedimentation were calculated to be 0.330 cm·year???1 and 0.237 g·cm???2·yr???1 and the sediment time of the collected core sample ranged from 1899 to 2000. The peak of PAH concentrations came at recent years. The source analysis showed PAHs mainly came from the contamination of low temperature pyrogenic processes, such as coal combustion. The PAHs concentrations were lower than ERL and LEL values for most collected samples. However, in several surface sediment samples especially in estuary sites, the PAHs concentrations were not only higher than ERL and LEL values, but also higher than ERM values. 相似文献
138.
Due to the growing concern of highly contaminated landfill leachate problems in Taiwan, an innovative advanced catalytic oxidation (FeGAC/H(2)O(2)) process was developed and employed in this research to treat the landfill leachate from central Taiwan. Experimental results indicated that the FeGAC/H(2)O(2) process could effectively remove organic compounds from landfill leachate. The presence of iron oxide coated granular activated carbon (FeGAC) greatly improved the oxidative ability of H(2)O(2) for the removal of humic acids, fulvic acids and non-humic substance from leachate. For instance, at pH 6, the removal efficiencies of FeGAC/H(2)O(2) and H(2)O(2) processes were 70% and 8%, respectively. FeGAC/H(2)O(2) combined both advantages of FeGAC and H(2)O(2) where FeGAC had good organics adsorption ability and could effectively catalyse the hydrogen peroxide oxidation reaction for organics removal. 相似文献
139.
采用风险分类-要素分析-风险排序的思路,对北京市核与辐射恐怖事件风险进行分析。根据国际上1998—2006年该类恐怖事件的实例,从事件所涉及的材料、场所角度将核与辐射恐怖事件分为6大类。结合北京市的实际情况进行涉核恐怖事件的要素分析,将北京市各类场所划分为4类敏感区并与5类涉核恐怖事件结合起来,得到北京市核与辐射恐怖事件风险构成图。通过风险分析,笔者认为北京市发生核与辐射恐怖事件风险最大的场所为核研究机构,最容易发生的核与辐射恐怖事件类型为涉及放射源的恐怖事件,结合分析结果对从阻止、探测、响应3个层次上提出了奥运核安保工作的反核恐工作建议。 相似文献
140.
本文介绍了炭催化剂吸附剂标准物质的研制过程。对标准物质的制备技术、均匀性检验、稳定性考察及定值和不确定度进行了逐项分析。采用活性炭浸渍、煅烧技术制得炭催化剂吸附剂标准物质。试验结果表明,该标准物质定值结果准确,均匀性、稳定性良好。铜含量的标准值为11.06%,扩展不确定度为0.13%。 相似文献