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251.
The layered laurylsulfonate intercalated green rust (lauryl-S GR) was synthesized to evaluate the influence of synthesis parameters and aqueous conditions on the adsorption of CeIV. The maximum adsorption capacity of 305.58 mg/g by lauryl-S GR was predictably obtained. The pseudo-first-order kinetic model was appropriate in fitting the whole uptake process in a weak acid environment. Three isotherm models including Langmuir, Freundlich, and Tempkin were all reliable in depicting the isotherm adsorption process. The maximum monolayer adsorption capacity of lauryl-S GR towards CeIV was 315.46 mg/g. Ce species including CeO and Ce2O3 besides CeO2 were matched in the XPS distribution, directly indicating the reduction reaction brought by FeII in the GR occurred to hydrated CeIV ions during the adsorption. Nano-sized Ce particles attached to the lauryl-S GRs after the adsorption experiments were observed in the morphological characterization. Flocculated materials were formed on the surface of the lauryl-S GR at a pH of 7, which further reduced the active sites and disrupted the continuous uptake of CeIV to the lauryl-S GR. This study expands the application of GRs and supplies an ideal iron-based material for the construction of the affiliated recovery pathway to the traditional separation of Ce. 相似文献
252.
单一重金属污染对水稻叶片光合特性的影响 总被引:14,自引:0,他引:14
以杂交稻协优818为材料,研究了Cu^2+、Hg^2+、Cd^2+ 3种重金属离子对水稻叶片光合特性的影响。试验结果表明:(1)Cu^2+在低浓度时BI起叶片叶绿素含量降低。而Hg^2+、Cd^2+在低浓度时。则导致叶绿素含量增加:高浓度时,3种重金属均BI起叶绿素含量降低。同时,低浓度时3种重金属离子均导致叶绿素a/b值升高:高浓度时则均引起叶绿素a/b值下降。(2)Cu^2+、Hg^2+、Cd^2+对水稻叶片叶绿素的吸收光谱均无明显影响,在活体条件下并未发生卟啉环中Mg^2+的置换。(3)Cu^2+、Hg^2+、Cd^2+均引起叶片希尔反应活力降低,即重金属污染明显影响光合作用。 相似文献
253.
254.
Commercial available zero valent aluminum under air-equilibrated acidic conditions (ZVAl/H+/air system) demonstrated an excellent capacity to remove aqueous organic compounds. Acetaminophen (ACTM), the active ingredient of the over-the-counter drug Tylenol®, is widely present in the aquatic environment and therefore the treatment of ACTM-contaminated water calls for further research. Herein we investigated the oxidative removal of ACTM by ZVAl/H+/air system and the reaction mechanism. In acidic solutions (pH < 3.5), ZVAl displayed an excellent capacity to remove ACTM. More than 99% of ACTM was eliminated within 16 hr in pH 1.5 reaction solutions initially containing 2.0 g/L aluminum and 2.0 mg/L ACTM at 25 ± 1\textcelsius. Higher temperature and lower pH facilitated ACTM removal. The addition of different iron species Fe0, Fe2+ and Fe3+ into ZVAl/H+/air system dramatically accelerated the reaction likely due to the enhancing transformation of H2O2 to HO. via Fenton's reaction. Furthermore, the primary intermediate hydroquinone and the anions formate, acetate and nitrate, were identified and a possible reaction scheme was proposed. This work suggested that ZVAl/H+/air system may be potentially employed to treat ACTM-contaminated water. 相似文献
255.
通过对污染源普查工作的探索,在实践中进行验证,现实的思考如何能更好的开展污染普查的工作方法,努力把国情调查工作做的更细致、更全面、更有效,全面实现国情调查的目的.本文根据实践经验对存在问题和解决措施进行归纳总结,并针对性的提出了一些建议和设想,以期为再次的污染源普查工作积累经验. 相似文献
256.
The characteristics of Pb2+ adsorption on the surface of birnessites with different average oxidation states (AOS) of Mn, synthesized under acidic and alkali conditions, were investigated. The results indicated that the amount of adsorbed Pb2+ increased with the increase of Mn AOS in birnessites. The amount of Pb2+ adsorbed positively correlated with the amount of released Mn2+, H+, and K+ (r = 0.9962 > 0.6614, n = 14, α = 0.01). The released Mn2+, H+, and K+ were derived mostly from the corresponding catio... 相似文献
257.
258.
刘会建 《中国环境管理干部学院学报》2013,(1):14-17
根据2006年以来的环境空气质量监测数据,对侯马市空气质量状况进行了月际浓度趋势和年际浓度趋势分析评价,指出了燃料燃烧、交通运输、城市建设、气象因素、外来污染等大气污染物的来源及特征,提出了深入治理煤烟污染、积极推广新能源使用、控制机动车尾气污染、加大治理城市扬尘污染、强化工业污染源治理等改善大气环境质量的对策建议。 相似文献
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260.
环境是公共的,环境利益具有公众性。在环境执法中积极吸纳公众意见,是国家民主管理社会的体现。公众参与环境执法的角色定位即:政府在环境执法中处于核心地位,拥有最终裁量权;企业是环境执法的对象;公众是环境执法的最终受益者。政府、企业与公众的沟通协调是公众参与环境执法的有效机制。 相似文献