全文获取类型
收费全文 | 89617篇 |
免费 | 1222篇 |
国内免费 | 1087篇 |
专业分类
安全科学 | 3706篇 |
废物处理 | 3254篇 |
环保管理 | 13752篇 |
综合类 | 21234篇 |
基础理论 | 26061篇 |
环境理论 | 72篇 |
污染及防治 | 14238篇 |
评价与监测 | 5399篇 |
社会与环境 | 3709篇 |
灾害及防治 | 501篇 |
出版年
2022年 | 810篇 |
2021年 | 802篇 |
2020年 | 647篇 |
2019年 | 871篇 |
2018年 | 1113篇 |
2017年 | 1159篇 |
2016年 | 2168篇 |
2015年 | 1839篇 |
2014年 | 2591篇 |
2013年 | 9260篇 |
2012年 | 2105篇 |
2011年 | 2311篇 |
2010年 | 3238篇 |
2009年 | 3386篇 |
2008年 | 1886篇 |
2007年 | 1748篇 |
2006年 | 2185篇 |
2005年 | 2211篇 |
2004年 | 2516篇 |
2003年 | 2346篇 |
2002年 | 1908篇 |
2001年 | 2209篇 |
2000年 | 1935篇 |
1999年 | 1495篇 |
1998年 | 1367篇 |
1997年 | 1353篇 |
1996年 | 1474篇 |
1995年 | 1570篇 |
1994年 | 1477篇 |
1993年 | 1318篇 |
1992年 | 1301篇 |
1991年 | 1287篇 |
1990年 | 1233篇 |
1989年 | 1191篇 |
1988年 | 1040篇 |
1987年 | 975篇 |
1986年 | 988篇 |
1985年 | 1057篇 |
1984年 | 1157篇 |
1983年 | 1164篇 |
1982年 | 1172篇 |
1981年 | 1094篇 |
1980年 | 943篇 |
1979年 | 920篇 |
1978年 | 823篇 |
1977年 | 718篇 |
1976年 | 640篇 |
1974年 | 607篇 |
1973年 | 630篇 |
1972年 | 629篇 |
排序方式: 共有10000条查询结果,搜索用时 15 毫秒
801.
The Ria Formosa lagoon, Portugal, receives organic matter from many natural and anthropogenic sources. This paper presents an overview of the contribution these sources made through the use of lipid biomarkers. Sixty-one surface sediment samples were collected and analysed for a range of lipids. Sewage materials were confined to regions within 2 km of discharge points; phytoplankton biomarkers (sterols and fatty acids) suggest production was greatest in the inner parts of the lagoon that also have greatest inorganic nutrient enrichment; terrestrial organic matter was present in relatively low concentrations as shown by both sterol and fatty alcohols; bacteria were widespread although the Sulphate Reducing Bacteria (SRBs, shown by the presence of 3-OH fatty acids) were located near but not adjacent to sewage discharge points. 相似文献
802.
L. Axelsson 《Marine Biology》1988,97(2):287-294
An automatically operated method for high precision measurements of steady-state photosynthesis by macroalgae was developed. Changes in pH and oxygen content of seawater passing the algae in a flowthrough system, could be measured with extremely high accuracy over very long periods of time. The method is especially suitable for measurements on flowthrough systems with high rates of water exchanges (i.e. short retention time), and can be used to study exchange processes for marine plants, animals and small ecosystems. Since the same measuring unit is used for several flowthrough chambers, the method is very suitable for comparisons between different species, or between differently pretreated specimens of the same species (e.g. in toxicological studies). The method was used to study the ratio: [oxygen production] to [CO2+H+ uptake] at different light intensities for several macroalgae belonging to different systematic groups and from different habitats. At lower photosynthetic rates this ratio was similar for all of the algae studied (1.17±0.02). For brown algae of the fucacean family, the ratio increased by 0.08 units at higher photosynthetic rates. This increase was thought to be related to the crassulacean acid metabolism (CAM)-like strategies connected to these algae. For all other algae studied, the ratio remained constant or decreased slightly (at most by 0.04 units) at higher photosynthetic rates. The relations between the abovementioned ratio and the photosynthetic quotient are discussed on a theoretical basis. 相似文献
803.
H. J. Cranfield 《Marine Biology》1973,22(3):211-223
The use during settlement of secretions of the 9 different types of gland in the foot of the pediveliger of Ostrea edulis L. was examined experimentally. During settlement, there is a progressive decrease in the crawling speed of the larva and a strengthening of its bond with the substratum. Both changes are related to (a) a change from ciliary to muscular pedal locomotion; (b) the increasing acidity and viscosity of the mucoid secretions used; (c) the secretion of a byssus thread by the glands of the byssus duet; (d) changes in the form and composition of this byssus. At the termination of settlement, the entire contents of 2 types of gland are discharged. Their secretions give rise to the cement which permanently fixes the larva to the substratum. The 9 types of gland are utilised sequentially in a manner closely related to the 6 phases recognised in settlement behaviour. 相似文献
804.
Behavioral aspects of sperm competition in cuttlefish, Sepia officinalis (Sepioidea: Cephalopoda) 总被引:6,自引:0,他引:6
Sexual selection studies in cephalopods indicate that sperm competition is a central feature of their mating systems, yet
this has not been studied experimentally in any detail. In 1998 we staged 20 matings of the cuttlefish, Sepia officinalis L., in the laboratory. Males rapidly initiated mating in the “head-to-head” position, with no apparent courtship. Mating
lasted an average of 10 min (range 7 to 14 min). For the first 6 min (on average 63% of the mating duration), the male flushed
strong jets of water directly at the female's buccal membrane, which sometimes resulted in the expulsion of parts of spermatangia
placed there in recent matings. Then, in a single discrete movement that lasted an average of only 14 s, the male's modified
fourth left arm – the hectocotylus – wrapped around a single large bundle of spermatophores (ca. 150 to 300) and transferred
them to the female's buccal membrane. For the remainder of the mating (average 3 min, range 1.5 to 5.0 min), the hectocotylus
repeatedly broke the spermatophores open, and manipulated them, so that sperm were released and many spermatangia were attached
along the ventral buccal membrane, near the paired seminal receptacles. Approximately 140 spermatangia were attached in rows
3 to 5 deep around the ventral buccal membrane in a single mating; the rest were usually discarded during mating. Histology
revealed that each of the seminal receptacles consists of a series of sperm storage bulbs connected by a central duct, which
leads to a single pore at the surface of the buccal membrane. Baseline data on sperm motility were obtained, but the mechanism
by which sperm enter the seminal receptacle remains unknown. Females seemed to initiate termination of mating, then males
guarded their mates temporarily. These results, combined with other recent laboratory experiments, provide evidence that sperm
competition may be a major feature of the mating system of S. officinalis.
Received: 4 January 1999 / Accepted: 18 May 1999 相似文献
805.
Jones GL Willy D Lumsden B Taufa T Lourie J 《Environmental pollution (Barking, Essex : 1987)》1987,48(2):101-115
It has long been known that mining activity can markedly change the level and distribution of certain heavy metals in the adjacent environment. This pollution can be quite widespread and long lasting and often has deleterious effects on the health of local populations. In the present study scalp hair was used as the biopsy material because of its ease of collection and long history of use in this connection. Hair was collected from all the local villages in the vicinity of the mine site, as well as from Papua New Guinean nationals from other provinces, and European expatriates who were employed by the mining company and who were resident in the area. Hair from local people showed a remarkably high iron content by comparison with previously studied populations. The extreme variations in hair iron levels were reflected in the differential distribution of levels according to location, age and sex. Hair cadmium was also high in the population studied. Hair copper, lead, zinc and mercury all appeared to be within 'normal' limits by comparison with other general populations. These results are discussed in the context of the environmental and social impact of the mining operations on the local people. 相似文献
806.
铬渣的热解无害化处理 总被引:1,自引:0,他引:1
采用热解工艺无害化处理铬渣,探讨了稻秆在铬渣无害化处理中的作用.研究了热解温度、稻秆与铬渣质量比、铬渣粒径及保温时间对铬渣热解无害化处理的影响,并分析了热解前后热解产物中铬元素形态的变化.结果表明,热解工艺能有效地将铬渣中Cr(Ⅵ)还原,稻秆热解过程中产生的气相挥发分对Cr(Ⅵ)的还原起核心作用.较为适宜的热解条件:热解温度为400 ℃,稻秆与铬渣质量比为0.10,铬渣粒径<2 000 μm,保温时间为10 min.在该热解条件处理下,热解产物中的Cr(Ⅵ)质量浓度为121 mg/kg,低于热解前铬渣中的Cr(Ⅵ)(3 400 mg/kg).热解后,可交换态及碳酸盐结合态铬含量降低,大部分铬转化成了稳定的有机结合态和残渣态,极大地降低了铬渣的危害.第一作者:张大磊,男,1982生,博士研究生,研究方向为固体废弃物热处理. 相似文献
807.
Larisse Montero Matthew Duane Urbano Manfredi Covadonga Astorga Giorgio Martini Massimo Carriero Alois Krasenbrink B.R. Larsen 《Atmospheric environment (Oxford, England : 1994)》2010,44(18):2167-2175
The present paper presents results from the analysis of 29 individual C2–C9 hydrocarbons (HCs) specified in the European Commission Ozone Directive. The 29 HCs are measured in exhaust from common, contemporary vehicle/engine/fuel technologies for which very little or no data is available in the literature. The obtained HC emission fingerprints are compared with fingerprints deriving from technologies that are being phased out in Europe. Based on the total of 138 emission tests, thirteen type-specific fingerprints are extracted (Mean ± SD percentage contributions from individual HCs to the total mass of the 29 HCs), essential for receptor modelling source apportionment. The different types represent exhaust from Euro3 and Euro4 light-duty (LD) diesel and petrol-vehicles, Euro3 heavy-duty (HD) diesel exhaust, and exhaust from 2-stroke preEuro, Euro1 and Euro2 mopeds. The fuels comprise liquefied petroleum gas, petrol/ethanol blends (0–85% ethanol), and mineral diesel in various blends (0–100%) with fatty acid methyl esters, rapeseed methyl esters palm oil methyl esters, soybean oil methyl or sunflower oil methyl esters. Type-specific tracer compounds (markers) are identified for the various vehicle/engine/fuel technologies.An important finding is an insignificant effect on the HC fingerprints of varying the test driving cycle, indicating that combining HC fingerprints from different emission studies for receptor modelling purposes would be a robust approach.The obtained results are discussed in the context of atmospheric ozone formation and health implications from emissions (mg km?1 for LD and mopeds and mg kW h?1 for HD, all normalised to fuel consumption: mg dm?3 fuel) of the harmful HCs, benzene and 1,3-butadiene.Another important finding is a strong linear correlation of the regulated “total” hydrocarbon emissions (tot-HC) with the ozone formation potential of the 29 HCs (ΣPO3 = (1.66 ± 0.04) × tot-RH; r2 = 0.93). Tot-HC is routinely monitored in emission control laboratories, whereas C2–C9 are not. The revealed strong correlations broadens the usability of data from vehicle emission control laboratories and facilitates the comparison of the ozone formation potential of HCs in exhaust from of old and new vehicle/engine/fuel technologies. 相似文献
808.
Savvas Kleanthous Md. Aynul Bari Guenter Baumbach Leire Sarachage-Ruiz 《Atmospheric environment (Oxford, England : 1994)》2009,43(31):4745-4753
The objective of this study was to describe the ambient levels of particulate matter (PM) and its influence to air quality situation on the dry Mediterranean island of Cyprus. From October 2002 to August 2003 PM10 and PM2.5 samples were collected at 31 different sampling sites in Cyprus. In addition, continuous measurements of PM10 were carried out from 2003 to 2007 at a traffic and a rural site. It can be recognised that at all traffic and at some residential and urban background sites, the actual EU limit values have been exceeded. Special events e.g. long-range transport of Sahara dust storms were recorded over urban as well as rural areas in the order of 6–8 events per year, with a major frequency in summer and spring periods. The comparison of the PM10 concentrations in Cyprus cities with values of other European cities demonstrates the PM10 problem in Cyprus, especially in the dry summer season, when no rain is cleaning the air and the dry surfaces. This underlines the necessity of PM abatement strategies. 相似文献
809.
Baseline soil levels of PCDD/Fs established prior to the construction of municipal solid waste incinerators in China 总被引:1,自引:0,他引:1
In order to determine the baseline contamination by polychlorinated dibenzo-p-dioxins (PCDDs) and polychlorinated dibenzofurans (PCDFs) in different areas in China, prior to the construction of municipal solid waste incinerators (MSWIs), a total of 32 representative soil samples was collected near 16 incinerators and analyzed for their PCDD/F concentrations. The PCDD/F baseline concentrations in the soil samples ranged from 0.32 to 11.4 ng I-TEQ kg−1 (dry matter), with average and median value of 2.73 and 2.24 ng I-TEQ kg−1 (dry matter), respectively, and a span between maximum and minimum recorded value of 36. The PCDD homologues predominated in 26 out of 32 soil samples, with the ratio (PCDDs)/(PCDFs) ranging from 1.1 to 164; however in the other 6 samples, PCDF homologues were larger, with the same ratio varying from 0.04 to 0.8. Principal component analysis (PCA) and hierarchical cluster analysis (HCA) were used to examine PCDD/F amount and profile in these soil samples, and their possible associations with known emission sources: in this process 6 really distinct isomer fingerprints were identified. Background PCDD/F levels and profiles were comparable to those found in soils from China and other countries and indicate a rather low baseline PCDD/F contamination of soils. The present data provide the tools for future assessment of a possible impact of these MSWIs. 相似文献
810.
Bacteria transport and deposition under unsaturated conditions: the role of the matrix grain size and the bacteria surface protein 总被引:1,自引:0,他引:1
Gargiulo G Bradford S Simůnek J Ustohal P Vereecken H Klumpp E 《Journal of contaminant hydrology》2007,92(3-4):255-273
Unsaturated (80% water saturated) packed column experiments were conducted to investigate the influence of grain size distribution and bacteria surface macromolecules on bacteria (Rhodococcus rhodochrous) transport and deposition mechanisms. Three sizes of silica sands were used in these transport experiments, and their median grain sizes were 607, 567, and 330 microm. The amount of retained bacteria increased with decreasing sand size, and most of the deposited bacteria were found adjacent to the column inlet. The deposition profiles were not consistent with predictions based on classical filtration theory. The experimental data could be accurately characterized using a mathematical model that accounted for first-order attachment, detachment, and time and depth-dependent straining processes. Visual observations of the bacteria deposition as well as mathematical modelling indicated that straining was the dominant mechanism of deposition in these sands (78-99.6% of the deposited bacteria), which may have been enhanced due to the tendency of this bacterium to form aggregates. An additional unsaturated experiment was conducted to better deduce the role of bacteria surface macromolecules on attachment and straining processes. In this case, the bacteria surface was treated using a proteolitic enzyme. This technique was assessed by examining the Fourier-transform infrared spectrum and hydrophobicity of untreated and enzyme treated cells. Both of these analytical procedures demonstrated that this enzymatic treatment removed the surface proteins and/or associated macromolecules. Transport and modelling studies conducted with the enzyme treated bacteria, revealed a decrease in attachment, but that straining was not significantly affected by this treatment. 相似文献