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In this study, the content and speciation of arsenic in coal waste and gas condensates from coal waste fires were investigated,
respectively, using the digestion and sequential extraction methods. The fresh and fired-coal waste samples were collected
from Yangquan, which is one of the major coal production regions in northern China. High-performance liquid chromatography-inductively
coupled plasma-mass spectrometry (HPLC-ICP-MS) was used to determine the concentrations of four major arsenic species [As(III),
As(V), monomethylarsonic acid (MMA) and dimethylarsenic acid (DMA)] in the extracts, while ICP-MS was used to measure total
As content. Arsenic content in the investigated coal wastes and the condensate ranges between 23.3 and 69.3 mg/kg, which are
higher than its reported average content in soils. Arsenic in coal waste exists primarily in the residual fraction; this is
followed in decreasing order by the organic matter-bound, Fe–Mn oxides-bound, exchangeable, carbonates-bound, and water-soluble
fractions. The high content of arsenic in the condensates indicates that combustion or spontaneous combustion is one of the
major ways for arsenic release into the environment from coal waste. About 15% of the arsenic in the condensate sample is
labile and can release into the environment under leaching processes. The water extractable arsenic (WEA) in the fresh coal
waste, fired coal wastes, and the condensate varied between 14.6 and 341 μg/kg, with As(V) as the major species. Furthermore,
both MMA and DMA were found in fresh coal wastes, fired coal wastes, and the condensate. 相似文献
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Fan Xiaoshan Gao Jixi 《中国人口.资源与环境(英文版)》2007,5(3):63-75
China has won the name of the world factory being famous for exporting a great deal of and various kinds of low-price merchandise. However, most of Chinese exports are primary goods or manufactured products that create heavy pollution and require intensive use of resources. Chinese products go abroad, but their following harms stay behind. The article analyzes many obvious low-price facts in China and their concomitant terrible environmental results in detail, and points out that there are huge hidden troubles in the way of China's sustainable development behind her seemingly flourishing economy. 相似文献
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以流域为单元进行水资源综合规划和管理是实现水环境改善的重要途径。本文以太湖流域第二大省界湖泊—淀山湖为例,在综合分析流域水环境质量基础上,利用GIS 分析工具划分流域治理片区并制定分区管控策略。根据流域所含骨干河流流向、骨干河流与淀山湖交汇特点、上中下游不同河段及镇域行政边界,将淀山湖流域分为吴淞江流域、千灯浦- 淀山湖流域、昆南湖荡流域、元荡湖荡流域、太浦河流域五大片区138 个子评价单元。通过水环境容量与压力两类空间叠加分析,构建形成污染重点减排区、污染综合治理区、产业绿色化提升区、生态环境保育区等四个类型区域,并提出差异化的产业准入和环境治理措施。本研究不仅为以流域为治理单元的水环境治理规划提供了较为可行的技术体系,而且为太湖流域水环境综合整治思路创新提供了可借鉴的案例。 相似文献