全文获取类型
收费全文 | 147篇 |
免费 | 1篇 |
国内免费 | 3篇 |
专业分类
安全科学 | 5篇 |
废物处理 | 3篇 |
环保管理 | 17篇 |
综合类 | 30篇 |
基础理论 | 27篇 |
污染及防治 | 48篇 |
评价与监测 | 10篇 |
社会与环境 | 9篇 |
灾害及防治 | 2篇 |
出版年
2023年 | 1篇 |
2022年 | 2篇 |
2021年 | 1篇 |
2020年 | 2篇 |
2019年 | 2篇 |
2018年 | 2篇 |
2017年 | 2篇 |
2016年 | 9篇 |
2015年 | 9篇 |
2014年 | 3篇 |
2013年 | 6篇 |
2012年 | 8篇 |
2011年 | 12篇 |
2010年 | 7篇 |
2009年 | 9篇 |
2008年 | 15篇 |
2007年 | 12篇 |
2006年 | 6篇 |
2005年 | 4篇 |
2004年 | 4篇 |
2003年 | 7篇 |
2002年 | 6篇 |
2001年 | 2篇 |
1999年 | 1篇 |
1998年 | 1篇 |
1995年 | 1篇 |
1994年 | 1篇 |
1992年 | 3篇 |
1991年 | 1篇 |
1990年 | 3篇 |
1987年 | 2篇 |
1986年 | 1篇 |
1985年 | 1篇 |
1984年 | 2篇 |
1983年 | 3篇 |
排序方式: 共有151条查询结果,搜索用时 375 毫秒
101.
Gilles Billen Vincent Thieu Josette Garnier Marie Silvestre 《Agriculture, ecosystems & environment》2009,133(3-4):234
The watersheds of the Seine, Somme and Scheldt rivers (France, Belgium, the Netherlands), flowing into the continental coastal zone of the English Channel and Southern North Sea, are among the regions of the world with the highest anthropogenic inputs of reactive nitrogen through fertilizer use, legume fixation and deposition of atmospheric nitrogen. They also represent examples of widely open systems, either exporting a large fraction of their N inputs under the form of agricultural products (case of the Seine basin) or importing high amounts of nitrogen as feed for livestock nutrition (case of the Scheldt basin), and delivering up to 2000 kg N km−2 yr−1 at river outlet into the sea. Taking these three watersheds as a case study, we review the different approaches developed so far for describing and predicting the fate of reactive nitrogen inputs to regional systems and its cascade from soils to sea. These approaches range from simple lumped input–output budget, to detailed process-based, spatially distributed models of nutrient transfers. The merits and the limits of these approaches are discussed. Their combination allows to establish a reasonably consistent budget for the three basins, emphasizing the various ‘retention’ terms linked to both landscape and in-stream processes, including storage in long residence time compartments (soil organic matter, vadose zone, aquifers, etc.), denitrification (in soil, riparian zones or river benthos) or sediment burial. Root-zone and riparian denitrification processes appear as major terms of landscape retention in all three investigated watersheds. Retention of nitrogen associated with collection and treatment of urban wastewater is also a major term in the two most populated watersheds. 相似文献
102.
The accumulation of cadmium chloride by a living, by an ethanol or potassium cyanide treated marine pseudomonad was studied. The metal uptake by the living strain was linear during the experiment and the amount of accumulated metal was high. The uptake by the treated strain was very fast during the first hours, but the amount of accumulated cadmium was lower. 相似文献
103.
Vincent Thieu Gilles Billen Josette Garnier Marc Benoît 《Regional Environmental Change》2011,11(2):359-370
Nitrogen contamination of ground and surface water in the Seine, Somme and Scheldt watersheds, as well as in the receiving
coastal marine zones, results in severe ecological problems. Previous modelling results showed that the implementation of
classical management measures involving improvement of wastewater purification and “good agricultural practices” are not sufficient
to obviate these problems. A more radical scenario was therefore established, consisting of a generalised shift to organic
agriculture of all agricultural areas in the three basins, with the additional constraints that livestock is fed only on local
fodder production. This scenario involves an increased livestock density in the Seine and Somme and a decrease in livestock
in the Scheldt basin. It leads to a significant reduction of agricultural production that finally brings the three basins
closer to autotrophy/heterotrophy equilibrium. Nitrate concentrations in most of the drainage network would drop below the
threshold of 2.25 mgN/l in the most optimistic hypothesis. The excess of nitrogen over silica (with respect to the requirements
of marine diatoms) delivered into the coastal zones would be decreased by a factor from 2 to 5, thus strongly reducing, but
not entirely eliminating the potential for marine eutrophication. 相似文献
104.
The behaviour of 4,4′-bis(2-sulfostyryl)biphenyl (DSBP), a fluorescent whitening agent, was investigated in the presence of Fe(III) aquacomplexes at room temperature. In the dark, a two-step reaction was observed when adding Fe(III) to a solution of DSBP: an initial fast redox reaction between DSBP and the monomeric species Fe(OH)2+ and a slower reaction leading to the coagulation of oxidised DSBP and iron. This phenomenon is due to the formation of a complex or an ion-pair between Fe(II) and/or Fe(III) with oxidised DSBP and it probably occurs by charge neutralisation in our experimental conditions. The precipitation of DSBP depends on the initial concentration in Fe(OH)2+ and is achieved for a ratio [Fe(OH) 2+]/[DSBP] of 5 approximately. Under irradiation at 365 nm, a complicated behaviour was observed: a complexation of iron by oxidised DSBP favoured by irradiation and a degradation of DSBP induced by an intramolecular electron transfer in the complex or by a photoredox of Fe(OH)2+ species generating OH radicals in the supernatant. The complete degradation of DSBP is reached four times faster in the presence of Fe(III) with respect to the direct photolysis of DSBP alone. Moreover, the total mineralization of DSBP obtained in less than 120 h upon irradiation at 365 nm is only observed in the presence of the ferric ions, enlightening the efficiency of the method involving Fe(III) and UV irradiation. 相似文献
105.
Gaseous nitrogen emissions and forage nitrogen uptake on soils fertilized with raw and treated swine manure 总被引:1,自引:0,他引:1
Chantigny MH Angers DA Rochette P Bélanger G Massé D Côté D 《Journal of environmental quality》2007,36(6):1864-1872
Treatments to reduce solids content in liquid manure have been developed, but little information is available on gaseous N emissions and plant N uptake after application of treated liquid swine manure (LSM). We measured crop yield, N uptake, and NH3 and N2O losses after the application of mineral fertilizer (NH4 NO3), raw LSM, and LSM that was decanted, filtered, anaerobically digested, or chemically flocculated. The experiment was conducted from 2001 to 2003 on a loam and a sandy loam cropped to timothy (Phleum pratense L.) with annual applications equivalent to 80 kg N ha(-1) in spring and 60 kg N ha(-1) after the first harvest. Raw LSM resulted in NH3 emissions three to six times larger (P < 0.05) than mineral fertilizer. The LSM treatments reduced NH3 emissions by an average of 25% compared with raw LSM (P < 0.05). The N2O emissions tended to be higher with raw LSM than with mineral fertilizer. The LSM treatments had little effect on N2O emissions, except for anaerobic digestion, which reduced emissions by >50% compared with raw LSM (P < 0.05). Forage yield with raw LSM was >90% of that with mineral fertilizer. The LSM treatments tended to increase forage yield and N uptake relative to raw LSM. We conclude that treated or untreated LSM offers an alternative to mineral fertilizers for forage grass production but care must be taken to minimize NH3 volatilization. Removing solids from LSM by mechanical, chemical, and biological means reduced NH3 losses from LSM applied to perennial grass. 相似文献
106.
Parent G Bélanger G Ziadi N Deland JP Laperrière J 《Journal of environmental quality》2007,36(2):557-567
Swine manure contains considerable amounts of total (P) and soluble phosphorus (PO(4)-P) which may increase the soil P content when applied in excess to crop requirements and, consequently, risk water eutrophication. The feasibility of using magnesium (Mg) from the by-product of electrolysis and foundries (BPEF) for the removal of P from liquid swine manure was studied by adding up to 3 g of Mg as BPEF per liter of nursery (NU) and grower-finisher (GF) swine manure in 25-L plastic buckets. Changes in P and other elements were monitored for up to 360 h. Small amounts of Mg as BPEF (0.5 and 1.0 g Mg L(-1) manure) reduced the total P concentration of the liquid fraction by 70 to 95% of both manure types with respect to the control treatment of mixed raw manure. A settling period of 8 h or more was necessary to significantly reduce the liquid fraction's total P concentration for both manure types. Reduction of PO(4)-P varied from 96 to 100% in the liquid fractions for both manure types, which along with natural settling, explains most of the total P reduction in that fraction. The addition of BPEF did not influence the N content of manure. The low P liquid fraction can be safely applied to saturated P soils whereas the high P solid fraction offers the opportunity of transporting manure to agricultural soils deficient in P. Since N is conserved, both liquid and solid fractions could be valuable fertilizer manure by-products. 相似文献
107.
108.
Residual soil nitrate after potato harvest 总被引:1,自引:0,他引:1
Bélanger G Ziadi N Walsh JR Richards JE Milburn PH 《Journal of environmental quality》2003,32(2):607-612
Nitrogen loss by leaching is a major problem, particularly with crops requiring large amounts of N fertilizer. We evaluated the effect of N fertilization and irrigation on residual soil nitrate following potato (Solanum tuberosum L.) harvests in the upper St-John River valley of New Brunswick, Canada. Soil nitrate contents were measured to a 0.90-m depth in three treatments of N fertilization (0, 100, and 250 kg N ha(-1)) at two on-farm sites in 1995, and in four treatments of N fertilization (0, 50, 100, and 250 kg N ha(-1)) at four sites for each of two years (1996 and 1997) with and without supplemental irrigation. Residual soil NO3-N content increased from 33 kg NO3-N ha(-1) in the unfertilized check plots to 160 kg NO3-N ha(-1) when 250 kg N ha(-1) was applied. Across N treatments, residual soil NO3-N contents ranged from 30 to 105 kg NO3-N ha(-1) with irrigation and from 30 to 202 kg NO3-N ha(-1) without irrigation. Residual soil NO3-N content within the surface 0.30 m was related (R2 = 0.94) to the NO3-N content to a 0.90-m depth. Estimates of residual soil NO3-N content at the economically optimum nitrogen fertilizer application (Nop) ranged from 46 to 99 kg NO3-N ha(-1) under irrigated conditions and from 62 to 260 kg NO3-N ha(-1) under nonirrigated conditions, and were lower than the soil NO3-N content measured with 250 kg N ha(-1). We conclude that residual soil NO3-N after harvest can be maintained at a reasonable level (<70 kg NO3-N ha(-1)) when N fertilization is based on the economically optimum N application. 相似文献
109.
110.