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511.
以硫脲为硫的源物质,以钛酸四丁酯为TiO2的前驱体,采用溶胶-凝胶法制备了掺硫改性TiO2光催化剂.以活性艳红X-3B为目标污染物,研究了该催化剂的光催化降解性能,对硫掺杂量、催化剂焙烧温度、溶液pH值以及催化剂添加量等影响因素进行了研究,并采用XRD分析手法对光催化剂进行表征.结果表明,经掺硫改性后的TiO2的催化活性有了很大提高,且硫的掺杂有一个最佳值,即Ti:S的摩尔比为1:1.经掺硫改性的TiO2在可见光区具备一定的催化活性,180 min内对活性艳红X-3B的去除率可达35.1%,且在紫外光区的催化活性优于纯TiO2. 相似文献
512.
Reconstructing long-term vegetation buffers along streams in agricultural landscapes has become a common environmental restoration strategy for improving water quality and wildlife habitat connectivity. This article developed a linear weighted model to rank the priority of agricultural sub-basins for the establishment of vegetative buffers. The method was applied to an agricultural watershed of 146 km2 in Ontario, Canada. The watershed was divided into 11 sub-basins as basic decision units. In each sub-basin, four stream buffer schemes with widths of 5, 10, 15 and 20m were generated. For each buffer, three benefit-cost attributes of reconstructing vegetation cover were estimated, which include acreage per dollar, sediment abatement per dollar and habitat benefit per dollar. These attributes were first normalized using a linear normalization approach to eliminate the effects across different units. The normalized attributes were then integrated using a simple additive weighting method to rank the 11 sub-basins for prioritizing spatial restoration action. A sensitivity analysis was also conducted to observe the impact of a change in attribute weights on the management decisions. The results suggest that vegetation buffers reconstructed for achieving the water quality goal are not effective in improving habitat connectivity and vice versa. 相似文献
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Hanlon EA Fan XH Gu B Migliaccio KW Li YC Dreschel TW 《Journal of environmental quality》2010,39(5):1724-1733
Restoration of the Florida Everglades is important for the health of the natural system, including both the "River of Grass" and its downstream estuaries. Water quality improvement is one indicator of successful restoration in this complex ecosystem. Using the period of record of 1977 through 2005, we evaluated data from seven inflow sites to the Everglades National Park (ENP) for temporal trends of various forms of phosphorus (P) and nitrogen (N) and analyzed them using principal component analysis and factor analysis without flow adjustments. Locally estimated scatter plot smoothing (LOESS) trend lines identified two inflection points (three time periods) of changing trend in total P (TP) concentration at the seven sites. Results indicated that overall water quality in ENP inflow improved from 1977 to 2005, with significant downward trends in TP concentration. The overall trend ofTP is probably mediated by hydrology, which is evident by a negative relationship between flow and annual average TP concentration at the majority of stations within the available data, although additional changes in vegetation due to hydroperiod may have some effects. Total N (TN), total Kjeldahl N, and total organic N concentrations also generally decreased at inflow sites. Water quality standards for TP, TN, and NH4+ -N were exceeded at selected sites during the study period. Principle component analysis and factor analysis detected a grouping of sampling sites related to the water delivery system that could be used as indicators to better manage monitoring resources. Study results suggest that water quality data analyses could provide additional insight into the success of a restoration management plan and on how monitoring may be modified for more efficient use ofresources. 相似文献
515.
Liu GD Gu B Miao SL Li YC Migliaccio KW Qian Y 《Journal of environmental quality》2010,39(5):1585-1593
Dead plant tissues and ash from a prescribed fire play an important role in nutrient balance and cycling in the Florida Everglades ecosystem. The objective of this study was to assess the dynamic changes in total phosphorus release (TPr) from ash or tissues of either cattail (Typha domingensis Pers.) or sawgrass (Cladium jamaicense Crantz) to water. Natural-dead (senesced-dead) and burning-dead (standing-dead due to a prescribed fire) cattail and sawgrass were collected from highly (H) and moderately (M) impacted zones in the Florida Everglades. This experiment was conducted by incubation and water-extraction of the materials in plastic bottles for 65 d at room temperature (24 +/- 1 degrees C). Results showed that 63 to 88%, 17 to 48%, 9 to 20%, and 13 to 28% of total P (TPp) were released as TPr from cattail and sawgrass ash, cattail tissues from the H zone, cattail tissues, and sawgrass tissues from the M zone, respectively. TPp means total P of plant tissues, whereas TPr is total P release from the tissues or ash. Most of the TPr was released within 24 h after burning. The quick release of TPr observed in this experiment may help explain the P surge in the surface water immediately following a fire in the marsh. These findings suggest that prescribed burning accelerates P release from cattail and sawgrass. They also imply that it is very important to keep the water stagnant in the first 24 h to maximize the benefits of a prescribed fire in the Everglades. 相似文献
516.
Sven D. Jelaska Toni Nikolić Lucija Šerić Jelaska Vladimir Kušan Hrvoje Peternel Goran Gužvica Zoran Major 《Environmental management》2010,45(3):616-625
Here we present the methodology used for terrestrial biodiversity analysis and site selection in Phase B of the UNDP/GEF COAST
project. The analysis was focused on the problem of biodiversity evaluation in four Croatian counties stretching from sea
level to the highest mountain in Croatia. Data on habitats, vascular flora, and fauna (mammals, birds, reptiles, amphibians,
butterflies, ground beetles, and underground invertebrates) were collected and analyzed for each of the four counties. Emphasis
was given to the richness of endangered species and the rarity of endemic species. Based on the spatial analyses of habitat,
fauna, and flora data, four to six areas were selected from each county and ranked according to their biodiversity importance.
Overlap between areas important for richness and those important for rarity was highest for data on flora (65.5%) and lowest
for data on fauna (16.7%). When different data sets were compared, the lowest overlap was between flora and fauna (17.1%)
and largest between fauna and habitats (23.9%). Simultaneous overlap among all three data sets was found in just 6.5% of the
overall selected areas. These results suggest that less specific data, with respect to taxa threat status, could better serve
as surrogate data in estimating overall biodiversity. In summary, this analysis has demonstrated that Dalmatia is a region
with a high overall biodiversity that is important in a broader European context. 相似文献
517.
以水体异味物质2-甲基异莰醇(2-methylisoborneol,2-MIB)为研究对象,在紫外光(λ<380 nm)照射下,探讨TiO2(P25)对2-MIB的光催化降解特性及光化学作用机理。结果表明,UV/TiO2光催化体系可以有效去除水体异味物质2-MIB,紫外光照射60 min,对2-MIB的降解率达95%。同时研究了光催化降解体系介质pH,共存腐殖酸(HA)和过硫酸钾(K2S2O8)对UV/TiO2光催化体系降解2-MIB的影响,发现低浓度HA([HA]≤0.5 mg/L)可以提高2-MIB降解速率,当HA浓度高于0.5 mg/L,2-MIB降解反应受到抑制;同时当加入电子受体K2S2O8后,降解体系中活性物种羟基自由基(.OH)明显增加,提高了TiO2对2-MIB的降解能力。利用苯甲酸荧光光度法和POD-DPD显色法跟踪测定降解过程中羟基自由基(·OH)和过氧化氢(H2O2)的变化,表明光催化反应涉及·OH机理。 相似文献
518.
污染场地不同深度土壤有机-矿质复合体中有机氯农药的分布 总被引:2,自引:0,他引:2
采用物理方法将某农药厂土壤分成4种粒径的有机-矿质复合体组分,粘粒、粉粒、细砂和粗砂,研究有机氯农药在土壤不同有机-矿质复合体组分中的分布特征及有机质含量对污染物质赋存分布的影响。结果表明,粉粒组分中污染物质六六六含量较高,粘粒组分中滴滴涕含量较高。粘粒和粉粒组分中污染物质的含量与相应的有机质含量间呈现显著相关关系,而在细砂和粗砂中这种相关性不显著。lgKoc值与污染物质含量的相关性分析结果与有机质的相关性分析结果相似。有机质可能是影响场地土壤有机氯农药分布的重要因素之一。本研究的结果可为污染场地的风险控制和环境修复提供基础依据。 相似文献
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