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901.
Photocatalytic degradation of mixed gaseous carbonyl compounds at low level on adsorptive TiO2/SiO2 photocatalyst using a fluidized bed reactor 总被引:7,自引:0,他引:7
An adsorptive silica-supported titania photocatalyst TiO(2)/SiO(2) was prepared by using nanosized titania (anatase) immobilized on silica gel by the sol-gel technique with the titanium tetra isopropoxide as the main raw material and acetic acid as the acid catalyst. Meanwhile the structure and properties of the TiO(2)/SiO(2) photocatalyst were studied by means of many modern analysis techniques such as TEM, XRD, and BET. Gas-solid heterogeneous photocatalytic decomposition of four carbonyl compounds mixture at low concentration levels over ultraviolet irradiated TiO(2)/SiO(2) photocatalyst were carried out with high degradation efficiencies in a coaxial triple-cylinder-type fluidized bed photocatalytic reactor, which provided efficient continuous contact of ultraviolet photons, silica-supported titania photocatalyst, and gaseous reactants. Experimental results showed that the photocatalyst had a high adsorption performance and a good photocatalytic activity for four carbonyl compounds mixture. Some factors influencing the photocatalytic decomposition of the mixed carbonyl compounds, i.e. the gas flowrate, relative humidity, concentration of oxygen, and illumination time, were discussed in detail. It is found that the photocatalytic reaction rate of four carbonyl compounds decreased in this order: propionaldehyde, acetone, acetaldehyde and formaldehyde. 相似文献
902.
903.
结构建模分析是工程应用领域中应用较为普遍的一种分析设计方法,对于简单的几何模型实体单元不仅能够得到较高的精度而且能够很好地再现结构受力特性,应力云图具有较高的展示度,而对于复杂的几何模型,实体模型不仅消耗大量的建模时间,而且求解时间也相对较长.文中分析了Solid-Shell-Beam(S-S-B)多单元建模及耦合技术原理,建立了铸造起重机S-S-B多单元装配模型,通过S-S-B多单元模型与实体模型的对比分析,验证了S-S-B单元装配模型计算准确性,最后利用S-S-B单元耦合分析方法计算了铸造起重机在空载、满载、偏载等典型工况下的结构受力情况,为铸造起重机的设计、校核及使用维护提供技术支撑. 相似文献
904.
Ding Guanghui Li Xueyao Zhang Jing Zhang Nannan Li Ruijuan Wang Yingying Yang Zhanning Peijnenburg Willie J. G. M. 《Environmental science and pollution research international》2019,26(25):25538-25549
Environmental Science and Pollution Research - Environmental waters cover a range of water quality characteristics which could greatly affect the behavior and fate of C60 in the aquatic... 相似文献
905.
Chen Ziang Ren Gengbo Ma Xiaodong Ding Ye Hui Yunmin Qin Pingping Xu Zhuoqi Gu Xiujun Yuan Fang Liu Yanhai 《Environmental science and pollution research international》2020,27(31):38580-38590
Environmental Science and Pollution Research - In this study, the occurrence, spatial distribution, sources, and ecological risks of perfluoroalkyl substances (PFASs) in the surface waters of the... 相似文献
906.
Binding and detoxification of chlorpyrifos by lactic acid bacteria on rice straw silage fermentation
Yan-Su Wang Tian-Hao Wu Yao Yang Cen-Ling Zhu Cheng-Long Ding 《Journal of environmental science and health. Part. B》2016,51(5):316-325
This investigation examined the reduction of pesticide residues on straw inoculated with lactic acid bacteria (LAB) during ensiling. Lactobacillus casei WYS3 was isolated from rice straw that contained pesticide residues. Non-sterilized rice straw, which was inoculated with L. casei WYS3, showed increased removal of chlorpyrifos after ensiling, compared with rice straw that was not inoculated with L. casei WYS3 or sterilized rice straw. In pure culture, these strains can bind chlorpyrifos as indicated by high-performance liquid chromatography analysis. Viable L. casei WYS3 was shown to bind 33.3–42% of exogenously added chlorpyrifos. These results are similar to those of acid-treated cells but less than those of heat-treated cells, which were found to bind 32.0% and 77.2% of the added chlorpyrifos respectively. Furthermore, gas chromatography–mass spectrometry analysis determined that L. casei WYS3 detoxified chlorpyrifos via P-O-C cleavage. Real-time polymerized chain reaction analysis determined that organophosphorus hydrolase gene expression tripled after the addition of chlorpyrifos to LAB cultures, compared with the control group (without chlorpyrifos). This paper highlights the potential use of LAB starter cultures for the detoxification and removal of chlorpyrifos residues in the environment. 相似文献
907.
抗生素药生产废水处理工艺改进研究 总被引:1,自引:0,他引:1
企业抗生素废水经原有工艺处理后污染物指标偏高,且不稳定。工艺通过采用增加初沉池和二沉池、污泥回用等改进措施,COD、氨氮等排放浓度下降且稳定排放,改进效果明显。 相似文献
908.
You H Ding J Zhao XS Li YF Liu LY Ma WL Qi H Shen JM 《Environmental geochemistry and health》2011,33(3):291-299
The spatial and seasonal variation of polychlorinated biphenyls (PCBs) were investigated in water and sediment samples collected
from Songhua River, China, from 2007 to 2008. The total concentration of PCB congeners ranged from 1.1 to 14 ng/l in water
and 0.26–9.7 ng/g dry weight (dw) in sediment. The results of seasonal variation may suggest an impact to PCB concentration
in water from its atmospheric input, the dilution to PCBs concentrations of high stream in summer, and a general trend towards
increased volatilization in warmer conditions. From PCBs concentrations comparison between upstream and downstream of industrial
urban cities, it was obvious that industrial urban cities reflect an important pollutant source for PCBs in our study, also
with the evidences of high concentrations of PCBs occurring in high development industry and residential areas. Meanwhile,
the homologue profile of PCBs in Songhua was analyzed, whose comparison with published data indicates that the sources of
PCBs accumulated in the sediment may also came from the residue of PCBs production in China. Total five dioxin-like PCBs (CB-77,
81, 105, 114, and 126) and nine (CB-77, 81, 105, 114, 118, 123, 126, 156, and 167) were found in Songhua water and sediment. 相似文献
909.
太子河洛氏鱥幼鱼栖息地适宜度评估 总被引:3,自引:0,他引:3
基于对太子河流域鱼类及栖息地的调查研究,选择该流域的优势种洛氏鱥(Phoxinus lagowskii)作为指示生物,建立洛氏鱥幼鱼对水深、流速、溶解氧、总溶解颗粒物和河岸带植被指数的栖息地适宜度曲线,并借鉴河道内流量增量法计算各采样点河段的洛氏鱥幼鱼栖息地适宜度指数。结果表明:洛氏鱥幼鱼栖息地适宜度指数在太子河上游较高(>0.5),中游次之(0.2-0.5),下游较低(<0.2)。洛氏鱥幼鱼栖息地适宜度指数与10项栖息地调查指标和土地利用类型的相关性分析表明:太子河流域内限制洛氏鱥幼鱼生存的因素不是水文条件,而是河流水质及河岸带等环境因素;洛氏鱥幼鱼栖息地适宜度指数受人类活动影响较大,随着太子河中下游人类开发强度加大,洛氏鱥栖息地质量呈下降趋势。 相似文献
910.
Fu J Ding YH Li L Sheng S Wen T Yu LJ Chen W An SQ Zhu HL 《Journal of environmental monitoring : JEM》2011,13(3):597-604
The distribution, source, ecological risk and ecotoxicity of polycyclic aromatic hydrocarbons (PAHs) of sediments from 7 sampling sites, named as Xinyang (XY), Huainan (HN), Bengbu (BB), Xuyi (XuY), Fuyang (FY), Mengcheng (MC) and Zhengzhou (ZZ), in the Huaihe River basin, China, have been investigated. The total concentrations of 16 USEPA priority PAHs ranged from 62.9 to 2232.4 ng g?1 dry weight (d.w.) with a mean concentration of 1056.8 ng g?1 d.w. Through the assessment of ecological risk, we found that the levels of PAHs in the Huaihe River should not exert adverse biological effects. The total benzo[a]pyrene toxicity equivalent (TEQ) values calculated for samples varied from 0.01 to 194.1 ng g?1 d.w., with an average of 65.9 ng g?1. The toxicity data were accordant with the chemical analysis results in this study. HN, BB and ZZ showed the greatest pollution extent both in the chemical analysis and the study of ecotoxicological effects. 相似文献