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201.
Investigations concerning the measurement and evaluation of mineral oil hydrocarbons using Fourier-transform-infrared (FT/IR-)-spectroscopy,1H-Nuclear magnetic resonance (1H-NMR)-spectroscopy and Capillary gas chromatography — Flame ionisation detection (GC-FID) are presented. By means of various mineral oils and three certified reference materials (CRM) all tested methods were within a ±7%-range to the mineral oil nominal value and the 95% confidence intervals of the CRM’s, respectively. The GC-FID evaluation could be done without calibration using an relative response ratio of mineral oil to an internal standard (n-tetracontane). A1H-NMR-method was developed for the quantitative determination of mineral oil hydrocarbons, successfully applied down to 0.2 mg/ml. Due to the determination limit achieved, the1H-NMR-spectroscopy gain in importance as a reference method for the analysis of mineral oils. 相似文献
202.
203.
Permeable reactive barriers (PRBs) are widely applied for in-situ remediation of contaminant plumes transported by groundwater. Besides the goal of a sufficient contaminant remediation inside the reactive cell (residence time) the width of plume intercepted by a PRB is of critical concern. A 2-dimensional analytical approach is applied to determine the flow fields towards rectangular PRBs of the continuous wall (CW) configuration with and without impermeable side walls (but yet no funnel). The approach is based on the conformal mapping technique and assumes a homogeneous aquifer with a uniform ambient flow field. The hydraulic conductivity of the reactive material is furthermore assumed to exceed the conductivity of the aquifer by at least one order of magnitude as to neglect the hydraulic gradient across the reactor. The flow fields are analyzed regarding the widths and shapes of the respective capture zones as functions of the dimensions (aspect ratio) of the reactive cell and the ambient groundwater flow direction. Presented are an improved characterization of the advantages of impermeable side walls, a convenient approach to improved hydraulic design (including basic cost-optimization) and new concepts for monitoring CW PRBs. Water level data from a CW PRB at the Seneca Army Depot site, NY, are used for field demonstration. 相似文献
204.
Špela Bavec Mateja Gosar Miloš Miler Harald Biester 《Environmental geochemistry and health》2017,39(3):443-465
A comprehensive geochemical investigation of potentially harmful elements (PHEs) in household dust from the town of Idrija (Slovenia), once a world-famous Hg mining town that is now seriously polluted, was performed for the first time. After aqua regia digestion, the content of mercury (Hg), arsenic (As), cadmium (Cd), cobalt (Co), chromium (Cr), copper (Cu), molybdenum (Mo), nickel (Ni), lead (Pb) and zinc (Zn) was measured. PHE-bearing particles were recognised and observed by scanning electron microscopy and energy-dispersive spectrometry before and after exposure to simulated stomach acid (SSA). Mercury binding forms were identified by Hg thermal desorption technique and gastric bioaccessible Hg was estimated after SSA extraction by ICP-MS. With regard to rural and urban background values for Slovenia, high Hg content (6–120 mg/kg) and slightly elevated As content (1–13 mg/kg) were found. Mercury pollution is a result of past mining and ore processing activities. Arsenic content is potentially associated with As enrichment in local soils. Four Hg binding forms were identified: all samples contained Hg bound to the dust matrix, 14 samples contained cinnabar, two samples contained metallic Hg (Hg0), and one sample assumingly contained mercury oxide. After exposure to SSA, Hg-bearing phases showed no signs of dissolution, while other PHE-bearing phases were significantly morphologically and/or chemically altered. Estimated gastric Hg bioaccessibility was low (<0.006–0.09 %), which is in accordance with identified Hg binding forms and high organic carbon content (15.9–31.5 %) in the dust samples. 相似文献
205.
Harald Geiger Karl H. Becker 《Journal of the Air & Waste Management Association (1995)》2013,63(4):425-433
Abstract Based on exhaust gas analyses from the combustion of five different types of gasoline in a passenger car operated on a chassis dynamometer, box model simulations of the irradiation of exhaust/NOx /air mixtures using an established chemical mechanism for a standardized photo-smog scenario were performed. The fuel matrix used covered wide fractional ranges for paraffinic, olefinic, and aromatic hydrocarbons. Two fuels also contained methyl tertiary butyl ether (MTBE). The different O3 profiles calculated for each run were compared and interpreted. The O3 levels obtained were strongly influenced by the exhaust gas concentrations of aromatic and olefinic hydro-carbons. The higher exhaust content of these compounds caused higher O3 production in the smog system investigated. The conclusion of the present study is that the composition of gasoline cannot be taken directly for the estimation of the emissions’ O3 creation potential from its combustion. Variation of the dilution in the different calculations showed evidence for an additional influence of transport effects. Accordingly, further detailed exhaust gas analyses followed by more complex modeling studies are necessary for a proper characterization of the relationship between fuel blend and gasoline combustion products. 相似文献
206.
Kris Verheyen Margot Vanhellemont Harald Auge Lander Baeten Christopher Baraloto Nadia Barsoum Simon Bilodeau-Gauthier Helge Bruelheide Bastien Castagneyrol Douglas Godbold Josephine Haase Andy Hector Hervé Jactel Julia Koricheva Michel Loreau Simone Mereu Christian Messier Bart Muys Philippe Nolet Alain Paquette John Parker Mike Perring Quentin Ponette Catherine Potvin Peter Reich Andy Smith Martin Weih Michael Scherer-Lorenzen 《Ambio》2016,45(1):29-41
207.
Winfried Schröder Stefan Nickel Simon Schönrock Michaela Meyer Werner Wosniok Harry Harmens Marina V. Frontasyeva Renate Alber Julia Aleksiayenak Lambe Barandovski Alejo Carballeira Helena Danielsson Ludwig de Temmermann Barbara Godzik Zvonka Jeran Gunilla Pihl Karlsson Pranvera Lazo Sebastien Leblond Antti-Jussi Lindroos Siiri Liiv Sigurður H. Magnússon Blanka Mankovska Javier Martínez-Abaigar Juha Piispanen Jarmo Poikolainen Ion V. Popescu Flora Qarri Jesus Miguel Santamaria Mitja Skudnik Zdravko Špirić Trajce Stafilov Eiliv Steinnes Claudia Stihi Lotti Thöni Hilde Thelle Uggerud Harald G. Zechmeister 《Environmental science and pollution research international》2016,23(11):10457-10476
For analysing element input into ecosystems and associated risks due to atmospheric deposition, element concentrations in moss provide complementary and time-integrated data at high spatial resolution every 5 years since 1990. The paper reviews (1) minimum sample sizes needed for reliable, statistical estimation of mean values at four different spatial scales (European and national level as well as landscape-specific level covering Europe and single countries); (2) trends of heavy metal (HM) and nitrogen (N) concentrations in moss in Europe (1990–2010); (3) correlations between concentrations of HM in moss and soil specimens collected across Norway (1990–2010); and (4) canopy drip-induced site-specific variation of N concentration in moss sampled in seven European countries (1990–2013). While the minimum sample sizes on the European and national level were achieved without exception, for some ecological land classes and elements, the coverage with sampling sites should be improved. The decline in emission and subsequent atmospheric deposition of HM across Europe has resulted in decreasing HM concentrations in moss between 1990 and 2010. In contrast, hardly any changes were observed for N in moss between 2005, when N was included into the survey for the first time, and 2010. In Norway, both, the moss and the soil survey data sets, were correlated, indicating a decrease of HM concentrations in moss and soil. At the site level, the average N deposition inside of forests was almost three times higher than the average N deposition outside of forests. 相似文献
208.
This article exemplifies an approach to analyzing political arguments and press deliberation on the issue of climate change and oil policy. I apply political discourse analysis to examine an oil minister's press conference presentation of the key official document on Norway's future oil policy, and evaluate how he attempted to reconcile the country's expansive petroleum policy with its self-proclaimed ambition of being world leading in responsible climate policy. The analysis displays how the minister's argumentation served to legitimate an expansive oil policy by projecting an altruistic motivation and invoking the authority of the tradition of the industry. This is supplemented by an analysis of newspaper editorials and commentaries on the speech, identifying a major split in viewpoints between local and national newspapers. The analyses evaluate arguments in an explicit manner, for example by critically questioning their value premises, thus suggesting an approach that could benefit critical research on environmental communication. 相似文献
209.
Evaluating sustainable forest management strategies with the Analytic Network Process in a Pressure-State-Response framework 总被引:1,自引:0,他引:1
Nowadays forestry faces a complex management situation; the understanding of sustainable forest management (SFM) has gone far beyond the original meaning of sustainable yield of timber. SFM strategies should fulfil ecological, economic and social functions without causing damage to other ecosystems. In this understanding, forest management actions cannot be seen as isolated or mono-causal. In this case study, indicators for SFM are arranged in a Pressure-State-Response (PSR) framework at forest management unit level. This framework links pressures on the environment caused by human activities with changes of environmental state (condition) parameters. Forest management also responds to these changes by instituting environmental and economic measures to reduce pressures and restore natural resources. The Analytic Network Process (ANP) is utilized to evaluate the performance of four management strategies with regard to the PSR framework on SFM. Priorities of indicators and alternatives are modelled with the ANP resulting from the interconnections to other indicators and their respective cumulative importance. The approach allows for more detailed information on the network of human influences and their impacts on forest ecosystems and goes beyond the limitations of flat-dimensioned indicator sets. 相似文献
210.
Criteria and indicators assessment is one of the ways to evaluate management strategies for mountain watersheds. One framework
for this, Integrated Watershed Management (IWM), was employed at Chittagong Hill Tracts region of Bangladesh using a multi-criteria
analysis approach. The IWM framework, consisting of the design and application of principles, criteria, indicators, and verifiers
(PCIV), facilitates active participation by diverse professionals, experts, and interest groups in watershed management, to
explicitly address the demands and problems to measure the complexity of problems in a transparent and understandable way.
Management alternatives are developed to fulfill every key component of IWM considering the developed PCIV set and current
situation of the study area. Different management strategies, each focusing on a different approach (biodiversity conservation,
flood control, soil and water quality conservation, indigenous knowledge conservation, income generation, watershed conservation,
and landscape conservation) were assessed qualitatively on their potential to improve the current situation according to each
verifier of the criteria and indicator set. Analytic Hierarchy Process (AHP), including sensitivity analysis, was employed
to identify an appropriate management strategy according to overall priorities (i.e., different weights of each principle)
of key informants. The AHP process indicated that a strategy focused on conservation of biodiversity provided the best option
to address watershed-related challenges in the Chittagong Hill Tracts, Bangladesh. 相似文献