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Adriana Gregorova Vladimir Sedlarik Miroslav Pastorek Hari Jachandra Franz Stelzer 《Journal of Polymers and the Environment》2011,19(2):372-381
This article contains a concept of the mechanical properties improvement of the highly crystalline poly(lactic acid) (PLA)
and filled composites. PLA as a semi-crystalline thermoplastic polymer was plasticized with poly(ethylene glycol) and filled
with 30 vol% of organic and/or inorganic filler. The degree of crytallinity was intentionally increased by annealing. The
filler/polymer matrix interphase was modified with the addition of 4, 4′-Methylenediphenyl diisocyanate (MDI). The effect
of compatibilizing as well as plasticizing agent on the thermal and mechanical properties, the water-absorption behaviour
and crystallization characteristics were studied. The results indicated that high content of filler and crystallites have
a strong influence on the composite′s mechanical properties despite of the plasticizer content, showing a high Young modulus.
The MDI seems to react in preference easy with plasticizing agent and then alternatively with filler due to the low functionality
of commercial PLA grade. 相似文献
109.
Hartmut Koehler Jürgen Warrelmann Peter Behrend Ingo Dobner Tobias Frische Wolfgang Heyser Bernd Jastorff Ulrich Walter 《Environmental Sciences Europe》2001,13(6):359-368
The final article of a series of three evaluates the in situ-remediation of TNT(trinitrotoluene)-contaminated soil from ‘Werk Tanne’. The multidisciplinary approach allows a differentiated assessment. Grading with large-scale machinery leads to a depletion of TNT for almost 90% within the first 6 months, while ADNT(amino-dinitrotoluene)-content decreases more or less steadily over 1,5 years. Grading reduces the heterogenous distribution of the contamination only slightly. Results from field-monitoring and biotest-battery indicate residual toxicities of ecotoxicological relevance and a reduced capacity for biological regeneration, in comparison with the uncontamined site. Mycorrhized plants safe-guard the site and improve the soilecological conditions. Their role in reducing lower level residual toxicity requires further investigation. There is need for future research (1) on the dynamics and mechanisms of the initial decrease of TNT followed by stagnation, (2) on the fate of the primary metabolites, (3) on long-term effects of the phytoremediation, and (4) on the establishment of the complex monitoring for routine work. 相似文献
110.
Vetterlein D Szegedi K Ackermann J Mattusch J Neue HU Tanneberg H Jahn R 《Journal of environmental quality》2007,36(6):1811-1820
Arsenate (As V) is the predominant form of arsenic in soils under aerobic conditions and competes with the major plant nutrient phosphorus (P) in the form of phosphate (PV) not only for sorption sites on mineral surfaces in soil but also for root membrane transporters. Plants have evolved several mechanisms for the mobilization of PV in soils in response to P deficiency, such as the release of organic anions and protons. The aim of the present study was to test whether these mechanisms result in a simultaneous mobilization of arsenate and what would be the consequences for As transfer from soil to plant. The compartment system approach with Zea mays as model crop was chosen as an experimental setup. The system is equipped with micro suction cups and allowed us to investigate processes occurring in the vicinity of roots. As a case study, an artificial quartz substrate with well defined soil physical properties was fertilized, spiked with As V, and amended with increasing amounts of goethite (0, 1, and 4 g kg(-1) in treatments G-0, G-1, and G-4, respectively). The addition of goethite alleviated the As V-induced growth reduction and reduced As V transfer from the substrate to the plant but induced P deficiency at the same time. When low amounts of goethite (1 g kg(-1)) were added, plants mobilized PV but not As V, which might be related to differences in surface complexation reported for PV and As V. No mobilization of PV or As V was observed with the addition of higher amounts of goethite, probably because of decreasing competition between organic anions, PV, and As V for binding sites. 相似文献