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191.
Klaus-Michael Wollin Helmut Höring Hermann H. Dieter 《Environmental Sciences Europe》1996,8(5):261-266
Risk assessment of contaminated sites from abandoned ammunition plants follows a multi-stage procedure with its own specific requirements for the toxicological assessment of chemical contaminants. Thus, the 22 explosives and related compounds (STVs) were classified according to carcinogenicity, genotoxicity and evaluation numbers for their toxicological potential (ENs). These characteristics permit a specific toxicological assessment and ranking at the stage of “historical reconnaissance”, independent of an evaluation of the contaminant concentrations. With a view to “orientative site evaluation” for the assessment of explosives and related compounds in groundwater and drinking water, toxicologically related guide values based on the ENs of toxicological potential as well as TDI-based guide values for STVs in soil were derived as based on toxicologically safe body doses and lifelong exposure (TDI=Tolerable Daily Intake). For regulatory purposes, substance related precautionary values are defined for probable carcinogens and contaminants with essential lacks in the toxicological data base. 相似文献
192.
Atmospheric lead and bromine in Germany: post-abatement levels,variabilities and trends 总被引:2,自引:0,他引:2
Lammel G Röhrl A Schreiber H 《Environmental science and pollution research international》2002,9(6):397-404
INTENTION, GOAL, SCOPE, BACKGROUND: Abatement measures since the 1970s have depleted lead and bromine levels in the atmosphere over large parts of Europe. Our knowledge of the atmospheric cycling of these elements while a several decade-long period of intensive mobilization reaches its end is incomplete. OBJECTIVE: We have characterized the trends in the atmospheric levels of Pb and Br and present-day temporal and spatial variabilities. METHODS: This was achieved by short-term (weeks) and long-term (years) measurements of particulate Pb and Br at various sites in Germany. Samples of atmospheric particulate matter were collected on filter membranes and analyzed by x-ray fluorescence. RESULTS AND DISCUSSION: Average Pb levels at rural and urban inland sites did not exceed concentrations in background aerosols, sampled at a Baltic Sea coastal site, by more than a factor of 3. Due to sea salt, bromide inland particulate Br levels are below those at a coastal site. There, non-sea salt Br, however, is significant as well. Urban Pb and Br levels are not necessarily higher than rural levels. The concentration levels have decreased in such a way that the previously common source, local vehicular traffic emissions, is no longer predominant. Regional rather than local sources have been increasingly determining the concentrations since the 1990s. This is more pronounced for Br than for Pb. We found indications for coal burning and long-range transport as significant Pb sources. For particulate Pb species, a range of ages (elapsed time since Pb emission) has been found. This range shows two maxima corresponding to characteristic times of 72 and 24 h. CONCLUSIONS: The (mean) atmospheric residence time of particulate Pb is longer than the residence time of Br, in particular in the wintertime. The chemical species contributing to atmospheric Pb should be addressed in future studies. RECOMMENDATION AND OUTLOOK: Clearly, despite effective abatement measures, atmospheric Pb will continue to be dominated by anthropogenic mobilization. The influence from long-range transport can be expected to decrease with the effectiveness of abatement programmes in neighbouring countries of the region. 相似文献
193.
Sewage sludge ash to phosphorus fertiliser: variables influencing heavy metal removal during thermochemical treatment 总被引:1,自引:0,他引:1
Mattenberger H Fraissler G Brunner T Herk P Hermann L Obernberger I 《Waste management (New York, N.Y.)》2008,28(12):2709-2722
The aim of this study was to improve the removal of heavy metals from sewage sludge ash by a thermochemical process. The resulting detoxified ash was intended for use as a raw material rich in phosphorus (P) for inorganic fertiliser production. The thermochemical treatment was performed in a rotary kiln where the evaporation of relevant heavy metals was enhanced by additives. The four variables investigated for process optimisation were treatment temperature, type of additive (KCl, MgCl(2)) and its amount, as well as type of reactor (directly or indirectly heated rotary kiln). The removal rates of Cd, Cr, Cu, Ni, Pb, Zn and of Ca, P and Cl were investigated. The best overall removal efficiency for Cd, Cu, Pb and Zn could be found for the indirectly heated system. The type of additive was critical, since MgCl(2) favours Zn- over Cu-removal, while KCl acts conversely. The use of MgCl(2) caused less particle abrasion from the pellets in the kiln than KCl. In the case of the additive KCl, liquid KCl - temporarily formed in the pellets - acted as a barrier to heavy metal evaporation as long as treatment temperatures were not sufficiently high to enhance its reaction or evaporation. 相似文献
194.
Oliver Wiche Balázs Székely Christin Moschner Hermann Heilmeier 《Environmental science and pollution research international》2018,25(32):31938-31956
Germanium (Ge) is widespread in the Earth’s crust. As a cognate element to silicon (Si), Ge shows very similar chemical characteristics. Recent use of Ge/Si to trace Si cycles and changes in weathering over time, growing demand for Ge as raw material, and consequently an increasing interest in Ge phytomining have contributed to a growing interest in this previously rather scarcely considered element in geochemical studies. This review deals with the distribution of Ge in primary minerals and surface soils as well as the factors influencing the mobility of Ge in soils including the sequestration of Ge in secondary mineral phases and soil organic matter. Furthermore, the uptake and accumulation of Ge in plants and effects of plant-soil relationships on the availability of Ge in soils and the biogeochemical cycling of Ge are discussed. The formation of secondary soil minerals and soil organic matter are of particular importance for the concentration of Ge in plant-available forms. The transfer from soil to plant is usually low and shows clear differences between species belonging to the functional groups of grasses and forbs. Possible uptake mechanisms in the rhizosphere are discussed. However, the processes that are involved in the formation of plant-available Ge pools in soils and consequently its biogeochemical cycling are not yet well understood. There is, therefore, a need for future studies on the uptake mechanisms and stoichiometry of Ge uptake under field conditions and plant-soil-microbe interactions in the rhizosphere as well as the chemical speciation in different plant parts. 相似文献
195.
Monitoring global change: Comparison of forest cover estimates using remote sensing and inventory approaches 总被引:2,自引:0,他引:2
David P. Turner Greg Koerper Hermann Gucinski Charles Peterson Robert K. Dixon 《Environmental monitoring and assessment》1993,26(2-3):295-305
Satellite-based remote sensing offers great potential for frequent assessment of forest cover over broad spatial scales, however, calibration and validation using ground-based surveys are needed. In this study, forest cover estimates for the United States from a recently developed land surface cover map generated from satellite remote sensing data were compared to state-level inventory data from the U.S. National Resources Planning Act Timber Database. The land cover map was produced at the U.S. Geological Survey EROS Data Center and is based on imagery from the AVHRR sensor (spatial resolution 1.1 km). Vegetation type was classified using the temporal signal in the Normalized Difference Vegetation Index derived from AVHRR data. Comparisons revealed close agreement in the estimate of forest cover for extensively forested states with large polygons of relatively similar vegetation such as Oregon. Larger forest cover differences were observed in other states with some regional patterns in the level of agreement apparent.Comparisons in inventory- and remote sensing-based estimates of current forested area with potential vegetation maps indicated the magnitude of past land use change and the potential for future changes. The remote sensing approach appears to hold promise for conducting surveys of forest cover where inventory data are limited or where rates of vegetation change, due to human or climatic factors, are rapid. 相似文献
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