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831.
Jing L Steinberg SM Johnson BJ 《Journal of the Air & Waste Management Association (1995)》2001,51(9):1359-1366
Oxidation of benzene, toluene, ethylbenzene, and xylenes (BTEX) in air, of significance due to, for example, the potential for O3 formation, is believed to be initiated by OH attack on the ring (addition) or on the alkyl side chain (H abstraction). A series of ring-breaking reactions follows, with major products predicted to be alpha-dicarbonyls, simple aldehydes, and organic acids. To test this prediction, ambient air mixing ratios of aldehydes (formaldehyde, acetaldehyde, benzaldehyde, glyoxal, and pyruvaldehyde), along with some supporting BTEX data, were measured at an urban site in Las Vegas, NV. Samples were collected on sorbents and determined by chromatographic methods; mixing ratios were compared to ambient levels of CO, O3, and NOx. A meteorological analysis (temperature, wind speed, and wind direction) was also included. Statistically significant relationships were noted among the BTEX hydrocarbons (HCs) and among the photochemically derived species (e.g., O3, NO2, and some of the aldehydes), although there was seasonal variation. The observations are consistent with a common primary source (i.e., vehicular exhaust or fuel evaporation) for the BTEX compounds and a common secondary source (e.g., OH attack) for glyoxal and pyruvaldehyde. 相似文献
832.
Pilkington MG Caporn SJ Carroll JA Cresswell N Lee JA Emmett BA Johnson D 《Environmental pollution (Barking, Essex : 1987)》2005,135(3):469-480
This study determined the effects of increased N deposition on rates of N and P transformations in an upland moor. The litter layer and the surface of the organic Oh horizon were taken from plots that had received long-term additions of ammonium nitrate at rates of 40, 80 and 120 kg N ha(-1) yr(-1). Net mineralisation processes were measured in both field and laboratory incubations. Soil phosphomonoesterase (PME) activity and rates of N(2)O release were measured in laboratory incubations and root-surface PME activity measured in laboratory microcosms using Calluna vulgaris bioassay seedlings. Net mineralisation rates were relatively slow, with net ammonification consistently stimulated by N addition. Net nitrification was marginally stimulated by N addition in the laboratory incubation. N additions also increased soil and root-surface (PME) activity and rates of N(2)O release. Linear correlations were found between litter C:N ratio and all the above processes except net nitrification in field incubations. When compared with data from a survey of European forest sites, values of litter C:N ratio were greater than a threshold below which substantial, N input-related increases in net nitrification rates occurred. The maintenance of high C:N ratios with negligible rates of net nitrification was associated with the common presence of ericaceous litter and a mor humus layer in both this moorland as well as the forest sites. 相似文献
833.
D. W. Johnson R. B. Susfalk T. G. Caldwell J. D. Murphy W. W. Miller R. F. Walker 《Water, Air, & Soil Pollution: Focus》2004,4(2-3):263-275
Estimates of C and N loss by gasification during a wildfire in a Jeffrey pine (Pinus Jeffreyii [Grev. and Balf.]) forest in Little Valley, Nevada are compared to potential losses in more mesic forests in the Integrated Forest Study (IFS). In Little Valley, the fire consumed the forest floor, foliage, and an unknown amount of soil organic matter, but little standing large woody material. On an ecosystem level, the fire consumed approximately equal percentages of C and N (12 and 9%, respectively), but a considerably greater proportion of aboveground N (71%) than C (21%). Salvage logging was the major factor in loss, and C lost from the site will not be replenished until forest vegetation is established and succeeds the current shrub vegetation. N2 fixation by Ceanothus velutinus [Dougl.] in the post-fire shrub vegetation appears to have more than made up for N lost by gasification in the fire over the first 16 yr, and may result in long-term increases in C stocks once forest vegetation takes over the site. N loss from the fire equaled > 1,000 years of atmospheric N deposition and > 10,000 years of N leaching at current rates. Calculations of C and N losses from theoretical wildfires in the IFS sites show similar patterns to those in Little Valley. Calculated losses of N in most of the IFS sites would equal many centuries of leaching. Conceptual models of biogeochemical cycling in forests need to include episodic events such as fire. 相似文献
834.
Increasing land applications of biosolid wastes as soil amendments have raised concerns about potential toxic effects of associated metals on the environment. This study investigated the ability of biosolid colloids to transport metals associated with organic waste amendments through subsurface soil environments with leaching experiments involving undisturbed soil monoliths. Biosolid colloids were fractionated from a lime-stabilized, an aerobically digested, and a poultry manure organic waste and applied onto the monoliths at a rate of 0.7 cm/h. Eluents were monitored for Cu, Zn, Pb, and colloid concentrations over 16 to 24 pore volumes of leaching. Mass-balance calculations indicated significantly higher (up to 77 times) metal elutions in association with the biosolid colloids in both total and soluble fractions over the control treatments. Eluted metal loads varied with metal, colloid, and soil type, following the sequences Zn = Cu > Pb, and ADB > PMB > LSB colloids. Colloid and metal elution was enhanced by decreasing pH and colloid size, and increasing soil macroporosity and organic matter content. Breakthrough curves were mostly irregular, showing several maxima and minima as a result of preferential macropore flow and multiple clogging and flushing cycles. Soil- and colloid-metal sorption affinities were not reliable predictors of metal attenuation/elution loads, underscoring the dynamic nature of transport processes. The findings demonstrate the important role of biosolid colloids as contaminant carriers and the significant risk they pose, if unaccounted, for soil and ground water contamination in areas receiving heavy applications of biosolid waste amendments. 相似文献
835.
TEMPORAL VARIATION IN THE NUTRIENT EXPORT OF RIVERS DRAINING INTO THE BAY OF QUINTE,ONTARIO, CANADA1
ABSTRACT: Annual exports of total phosphorus, soluble reactive phosphorus, and total nitrogen are presented for the period 1965–1974, for five rivers draining into the Bay of Quinte, Lake Ontario. The export values are typical for the physiography and land use though the results indicate that soluble reactive phosphorus exports for the four largest rivers have been declining. Also the variation in export of total phosphorus and total nitrogen is highly correlated with variation in annual runoff. This is noted as being a factor deserving more attention in future efforts to classify nutrient export values in relation to land use and geology. 相似文献
836.
Alan R. Johnson 《Environmental management》1988,12(4):515-523
The state of an ecosystem may be represented by a multidemensional state vector,x. The goal of ecosystem management is to insure that the ecosystem remains within some setX of acceptable states, such thatx X. Since ecosystem management decisions must be based on limited knowledge, a small number of diagnostic variables must be found which accurately reflect ecosystem state. If the vector of diagnostic variables, , is found to be within a specified set , the state vectorx is predicted to be withinX. The selection and use of such diagnostic variables is examined in the context of an aquatic ecosystem simulation model. Techniques used in searching for diagnostic criteria include multiple linear regression, discriminant analysis, and visual inspection of graphical data displays. The adequacy of a diagnostic criterion as a predictor of ecological risk is demonstrated to be a function of the associated rates of type I and type II statistical errors. A simple cost-benefit analysis is undertaken to illustrate one approach for choosing an optimal balance between these error rates. 相似文献
837.
Feng Peng David L. Johnson Steven W. Effler 《Journal of the American Water Resources Association》2002,38(5):1453-1465
ABSTRACT: The technique of i ndividual p article a nalysis conducted by s canning electron microscopy interfaced with a utomated X ‐ray microanalysis (IPA/SAX) was used to characterize suspended particulate matter in New York City's drinking water reservoirs and their tributaries. The study covered a two year period and involved analyses of more than 300 samples. The particle cross sectional area per unit volume (PAV), or area concentration, was measured to account for the observed turbidity, a representation of light scattering property of the studied medium. A simple linear model with a nearly zero intercept was able to explain more than 85 percent of the variation in the measured turbidity. Moreover, the particle assemblage was categorized into generic particle types with distinctive geochemical or geological origins. Thus, PAV compositions in terms of particle types could be apportioned into turbidity components based on the model. Inorganic tripton, dominated by aluminosilicate (clay) and silicate of nonbiological nature, was found to be the major turbidity causing constituent in most cases. With the exception of one reservoir where organic detritus was significant, the predicted inorganic particle turbidity agreed with the measured turbidity within experimental error. 相似文献
838.
Karen L. Bushaw‐Newton David D. Hart James E. Pizzuto James R. Thomson Jennifer Egan Jeffrey T. Ashley Thomas E. Johnson Richard J. Horwitz Melissa Keeley Joy Lawrence Don Charles Catherine Gatenby Daniel A. Kreeger Tim Nightengale Roger L. Thomas David J. Velinsky 《Journal of the American Water Resources Association》2002,38(6):1581-1599
ABSTRACT: Dam removal has been proposed as an effective method of river restoration, but few integrative studies have examined ecological responses to the removal of dams. In 1999, we initiated an interdisciplinary study to determine ecological responses to the removal of a 2 m high dam on lower Manatawny Creek in southeastern Pennsylvania. We used an integrative monitoring program to assess the physical, chemical, and biological responses to dam removal. Following removal in 2000, increased sediment transport has led to major changes in channel form in the former impoundment and downstream reaches. Water quality did not change markedly following removal, probably because of the impoundment's short hydraulic residence time (less than two hours at base flow) and infrequent temperature stratification. When the impoundment was converted to a free flowing reach, the composition of the benthic macroinvertebrate and fish assemblages in this portion of Manatawny Creek shifted dramatically from lentic to lotic taxa. Some fish species inhabiting the free flowing reach downstream from the dam were negatively affected by large scale sediment transport and habitat alteration following dam removal, but this appears to be a short term response. Based on our observations and experiences in this study, we provide a list of issues to evaluate when considering future dam removals. 相似文献
839.
Pete Bettinger K. Norman Johnson John Sessions 《Journal of the American Water Resources Association》1998,34(4):891-907
ABSTRACT: A land management activity scheduling model that can perform a multi-period, simultaneous evaluation of aquatic habitat quality and commodity production goals was used to identify alternatives which would allow the improvement of aquatic habitat conditions over time, while producing wood products. The scheduling model has the ability to use stream sediment index levels, stream temperature index levels, and equivalent clearcut acres (ECA) levels as primary goals. A secondary goal imbedded in the model is the achievement of an even-flow of timber harvest volume, and a tertiary goal is the achievement of maximum efficiency (maximum net present value). The scheduling model utilizes a heuristic programming technique (Tabu search) to guide the selection of timber harvests and road standards. A 14,643 acre case study watershed in eastern Oregon is used to illustrate several policy scenarios. Activities considered include: clearcutting and partial cutting; cable, skyline, ground-based, and helicopter logging; road obliteration; requiring lower truck tire pressures on forest roads; and tree planting in riparian areas. The scheduling model produced land management plans which were spatially and temporally feasible over ten ten-year time periods. Stream temperature was shown to be dramatically reduced if tree planting is performed in all riparian areas, regardless of whether harvesting activities occurred, and including meadows and forested areas where shade density is low. Timber harvest volume levels decreased 31 to 43 percent, and net present value levels decreased 36 to 46 percent, from an unconstrained case, when any of the following occurred: ECA was constrained to 15 percent, sediment index levels were required to decrease by 1 percent per decade, or temperature levels were constrained to “no harvest” levels. The use of a heuristic programming technique is a departure from traditional techniques that are commonly used in management plan development. Yet the heuristic technique allows the inclusion of complex management goals, many of which may be prohibited when using more traditional mathematical programming techniques. In addition, decision variables which require spatial information, requiring them to take on integer or non-linear representations, can be accounted for without realizing the limitations of the traditional techniques. 相似文献
840.
Johnson U. Kitheka George S. Ongwenyi Kenneth M. Mavuti 《Ambio-人类环境杂志》2002,31(7):580-587
本文主要研究了肯尼亚姆瓦彻湾(属于浅潮滩红树林湿地)泥沙交换的动力机制.该港湾属于半日潮,大、小潮的潮差分别为.2m和1.4m,大潮高水位的水面面积为17km2. 相似文献