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281.
Formation of chlorinated and brominated dioxins and other organohalogen compounds at the pilot incineration plant VERONA 总被引:5,自引:0,他引:5
Experiments were conducted at the VERONA pilot plant, an incineration plant with stationary grate and separate post-combustion chamber, using wood and propane as basic combustible materials and with controlled dosage of various bromine-, chlorine- and copper-containing compounds. The behaviour of the following compounds was studied in the combustion chamber, after the post-combustion chamber and after the heat exchanger: polychlorinated phenols (PCPh), polybrominated phenols (PBrPh), polychlorinated benzenes (PCBz), polybrominated benzenes (PBrBz), polychlorinated dioxins and furans (PCDD/F) and polybrominated dioxins and furans (PBDD/F). The bromine co-incineration leaded to very high bromophenol concentrations after the post-combustion chamber. The formation of brominated and mixed-halogenated phenols and the further reaction to halogenated dioxins is apparently a relevant reaction mechanism for dioxin formation in processes involving bromine. This assumption is supported by the high formation rates of PBDD/F found in the heat exchanger, which were 4-20 times higher than those of PCDD/F. Moreover, the strong correlations found between the formation rates of PCPh, PCBz and PCDD/F in the heat exchanger indicate that in addition considerable new formation of dioxins takes place through de novo synthesis. Experiments involving the variation of primary operational parameters and fuel properties have shown that the quality of post-combustion plays a much greater role than the other parameters. Furthermore, it became apparent that the congeners of the chlorophenols and of the chlorobenzenes, measured in various incineration stages, do not correlate closely with the dioxin concentrations after the heat exchanger. 相似文献
282.
Oettl D Sturm PJ Pretterhofer G Bacher M Rodler J Almbauer RA 《Journal of the Air & Waste Management Association (1995)》2003,53(10):1233-1240
Transit traffic through the Austrian Alps is of major concern in government policy. Pollutant burdens resulting from such traffic are discussed widely in Austrian politics and have already led to measures to restrict traffic on transit routes. In the course of an environmental assessment study, comprehensive measurements were performed. These included air quality observations using passive samplers, a differential optical absorption spectroscopy system, a mobile and a fixed air quality monitoring station, and meteorological observations. As was evident from several previous studies, dispersion modeling in such areas of complex terrain and, moreover, with frequent calm wind conditions, is difficult to handle. Further, in the case presented here, different pollutant sources had to be treated simultaneously (e.g., road networks, exhaust chimneys from road tunnels, and road tunnel portals). No appropriate system for modeling all these factors has so far appeared in the literature. A prognostic wind field model coupled with a Lagrangian dispersion model is thus presented here and is designed to treat all these factors. A comparison of the modeling system with results from passive samplers and from a fixed air quality monitoring station proved the ability of the model to provide reasonable figures for concentration distributions along the A10. 相似文献
283.
Andreani-Aksoyoglu Sebnem Keller Johannes Dommen Josef Prévôt André S. H. 《Water, Air, & Soil Pollution: Focus》2003,3(5-6):289-305
The three-dimensional Eulerian model CAMx (Comprehensive Air QualityModel with Extensions) was applied for the first time to simulate bothgaseous and particulate photochemical air pollution in Switzerland during July 28–30, 1993. The meteorological input data were prepared using the Systems Applications International Mesoscale Model (SAIMM). The CAMx model results were compared with the measurements carried out at ground level andfrom airborne measuring platforms within the frame of the Swiss POLLUMET research programme. In general, the CAMx performance for gaseous species wasfound to be better than that of the previously used Urban Airshed Model (UAM)and the Variable Grid Urban Airshed Model (UAM-V). The most significant improvement for the gaseous species is in the prediction of HNO3 concentrations, due to the inclusion of aerosol chemistry. Aerosol species such as NO3
-, NH4
+, SO4
2-, and secondary organic aerosols were calculated in one particle size range (0.04–2.5 m) and compared with a few measurements available. Although July 29 was reasonably well simulated, overestimated wind speeds by SAIMM for July 30 caused a too fast transport of pollutants. Similarly to measurements, significant spatial correlation of the secondarily formed aerosols with ozone and formaldehyde is found in the afternoon. 相似文献
284.
285.
J. Scott Turner Johannes R. Henschel Yael D. Lubin 《Behavioral ecology and sociobiology》1993,33(1):35-43
Summary
Seothyra henscheli (Eresidae) is a burrowing spider that lives in the dune sea of the southern Namib Desert, Namibia. Prey capture by these spiders involves a foray from a cool subterranean retreat to the undersurface of a capture web that can be lethally hot. Striking, disentangling and retrieving prey from the capture web typically involves several short trips to the capture web, alternating with retreats to the cool burrow. It has been suggested that this behavior limits the increase of body temperature a spider must experience while working at the hot capture web. We used biophysical models in conjunction with direct observations of prey-capture behavior and distributions of sand temperature to estimate body temperatures experienced by S. henscheli during prey capture. In the circumstances we observed, only the relatively long post-strike retreat from the capture web is important in keeping spiders' body temperatures from exceeding their lethal limits. After the post-strike retreat, shuttling appreciably limits the increase in body temperature of small individuals, but may have little effect on body temperature increase in larger spiders.
Correspondence to: J.S. Turner at the present address 相似文献
286.
287.
Johannes Fresner Jürgen Jantschgi Stefan Birkel Josef Bärnthaler Christina Krenn 《Journal of Cleaner Production》2010,18(2):128-136
Cleaner Production is an organized approach to minimize industrial waste and emissions by increasing the efficiency of the use of materials and energy. It is propagated especially by UNIDO and UNEP as an approach to identify preventive measures to cut on waste and emissions from industrial activities. Case studies conducted by the authors in the last 10 years demonstrate, that in a number of cases water consumption per production unit of industries from the surface treatment sector, from food processing and from the textile industry could be reduced by 30–90%, auxiliary materials consumption could be reduced by 30–50%, and energy consumption of processes could be reduced by 15–25%. All these measures were actually economically beneficial for the companies, most of these measures paid back in less than one year [1].The standard approach to apply Cleaner Production originates from chemical engineering. It follows the steps of: Drawing a process flow sheet – collecting input/output data – doing mass and energy balances – identify sources for waste and emissions – set priorities – identify options. In the process of option generation one generally relies on expert knowledge or on checklists which are available in different manuals or in the best available technology reference (BREF) notes.1 This approach is strong with teams with an (chemical) engineering background.The authors wanted to develop a generic approach for option identification especially for teams with little formal engineering background or teams which have to go beyond their professional experience by using elements of the so-called TRIZ method (Theory of inventive problem solving, or originally Russian: “” (Teoria reschenija isobretatjelskich sadatsch)). TRIZ offers very strong tools for developing process improvement options on a generic level without specific technological knowledge about the process which shall be improved. The authors have found from their research that especially the concept of the Ideal Final Result, and the Laws of Evolution form a conceptual framework which can aid effectively in the identification of improvement options in a systematic way. 相似文献
288.
Bumblebee detection of a flat circular disc (two-dimensional (2D) presentation) and a disc which was presented 10 cm in front
of a structured background (and thus provided three-dimensional (3D) cues) was compared. A dual choice test using a Y-maze
apparatus was conducted to estimate the minimum visual angle at which the bees were able to detect the disc. At large visual
angles of 15, 10 and 5° bees’ performance between the 2D and the 3D presentation did not differ. However, when the disc subtended
3° at the bee’s eye, the bees performed significantly better when 3D information was available. Overall, bees were able to
detect a target subtending a 40% smaller visual angle when it was presented in front of the structured background compared
to a 2D presentation. This suggests that previous reports on the limits of target detection in bees using flat stimuli might
have underestimated the bees’ ability to locate small flowers under natural conditions. Bees use motion parallax, i.e. the
apparent relative motion of a stationary object against a background, for perceiving the third dimension. Our data suggest
that bumblebees can integrate information from at least two types of feature detectors, motion and area, to improve single
target detection. 相似文献
289.
Georg Steinhauser Johannes H. Sterba Eliezer Oren Michaela Foster Max Bichler 《Die Naturwissenschaften》2010,97(4):403-410
Seven pumice samples from excavations in North Sinai have been investigated with respect to their geochemical composition.
This type of volcanic rock has been used as an abrasive and thus has been an object of trade since antiquity. With the help
of Instrumental Neutron Activation Analysis, six of these Bronze Age samples could be correlated to their volcanic sources
on the islands of Santorini, Nisyros and Giali (Greece) using the typical element concentrations (“chemical fingerprint”).
The source of one pumice sample remains unidentified excluding, however, the Santorini eruption as a possible source. The
concluding section of this article discusses the possible contribution, however indirect, of the pumice from Sinai and elsewhere
in the Eastern Mediterranean to the controversial issue of the accurate date of the “Minoan” eruption of Santorini. 相似文献
290.
Abandoned landfills and dumps, where untreated waste materials were deposited in the past, are a main anthropogenic source of relevant gaseous emissions. The determination of stability is a crucial target in the context of landfill risk assessment. FTIR spectroscopy and simultaneous thermal analysis in association with multivariate statistical methods were applied to landfill materials in order to get information on the kind of waste and its reactivity. The spectral and thermal patterns are fingerprints of the material. Industrial waste and the material from a 5-year-old reactor landfill were distinguished from the defined classes of mechanically-biologically treated ("MBT") waste and 30 to 40-year-old stable landfills containing municipal solid waste and construction waste ("LF") by a classification model based on soft independent modeling of class analogy (SIMCA). Degradation experiments were carried out with the fresh material originating from one MBT plant that was subjected to aerobic and anaerobic conditions in lab-scale reactors. These samples were compared to samples of one reactor landfill and to the landfill fraction from the MBT plant to demonstrate the efficiency of the biological pretreatment before final disposal. Prediction models that are based on spectral or thermal characteristics and the corresponding reference analyses were calculated by means of a partial least squares regression (PLS-R). The developed models of the biological oxygen demand (BOD) and the dissolved organic carbon (DOC) were based on spectral data, the models of the total organic carbon (TOC) and total nitrogen (TN) were based on thermal data (heat flow profiles and mass spectra of combustion gases). Preliminary results are discussed. The enthalpy of the materials decreases with progressing mineralization, whereas the enthalpy of the remaining organic matter increases. The ratio of the enthalpies was used as an indicator of stability. Selected samples comprising old landfills, a recent reactor landfill, MBT landfills and MBT materials were classified according to the calculated ratios. 相似文献