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131.
Carbon isotope fractionation during reductive dechlorination of TCE in batch experiments with iron samples from reactive barriers 总被引:4,自引:0,他引:4
Reductive dechlorination of trichloroethene (TCE) by zero-valent iron produces a systematic enrichment of 13C in the remaining substrate that can be described using a Rayleigh model. In this study, fractionation factors for TCE dechlorination with iron samples from two permeable reactive barriers (PRBs) were established in batch experiments. Samples included original unused iron as well as material from a barrier in Belfast after almost 4 years of operation. Despite the variety of samples, carbon isotope fractionations of TCE were remarkably similar and seemed to be independent of iron origin, reaction rate, and formation of precipitates on the iron surfaces. The average enrichment factor for all experiments was -10.1 per thousand (+/- 0.4 per thousand). These results indicate that the enrichment factor provides a powerful tool to monitor the reaction progress, and thus the performance, of an iron-reactive barrier over time. The strong fractionation observed may also serve as a tool to distinguish between insufficient residence time in the wall and a possible bypassing of the wall by the plume, which should result in an unchanged isotopic signature of the TCE. Although further work is necessary to apply this stable isotope method in the field, it has potential to serve as a unique monitoring tool for PRBs based on zero-valent iron. 相似文献
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He Yuejun Cornelissen Johannes H. C. Wang Pengpeng Dong Ming Ou Jing 《Environmental science and pollution research international》2019,26(9):8828-8837
Environmental Science and Pollution Research - The formation of a common mycorrhizal network (CMN) between roots of different plant species enables nutrient transfers from one plant to another and... 相似文献
135.
Georg Steinhauser Stefan Merz Dieter Hainz Johannes H. Sterba 《Environmental science and pollution research international》2013,20(4):2527-2534
Several environmental media in Austria were monitored for artificial radionuclides released during the Fukushima nuclear accident. Air (up to 1.2 mBq/m3 particulate 131I) and rainwater (up to 5.2 Bq/L 131I) proved to be the media best suited for the environmental monitoring, allowing also a temporal resolution of the activity levels. Significant regional differences in the wet deposition of 131I with rain could be observed within the city of Vienna during the arrival of the contaminated air masses. Forward-trajectory analysis supported the hypothesis that the contaminated air masses coming from the northwest changed direction to northeast over Northern Austria, leading to a strong activity concentration gradient over Vienna. In the course of the environmental monitoring of the Fukushima releases, this phenomenon—significant differences of 131I activity concentrations in rainwater on a narrow local scale (8.1 km)—appears to be unique. Vegetation (grass) was contaminated with 131I and/or 137Cs at a low level. Soil (up to 22 Bq/kg 137Cs) was only affected by previous releases (nuclear weapon tests, Chernobyl). Here, also significant local differences can be observed due to different deposition rates during the Chernobyl accident. The effective ecological half-lives of 137Cs in soil were calculated for four locations in Austria. They range from 7 to 30 years. No Austrian sample investigated herein exceeded the detection limit for 134Cs; hence, the Fukushima nuclear accident did not contribute significantly to the total radiocesium inventory in Austrian environmental media. The levels of detected radioactivity were of no concern for public health. 相似文献
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Tina Heger Anna T. Pahl Zoltan Botta-Dukát Francesca Gherardi Christina Hoppe Ivan Hoste Kurt Jax Leena Lindström Pieter Boets Sylvia Haider Johannes Kollmann Meike J. Wittmann Jonathan M. Jeschke 《Ambio》2013,42(5):527-540
Invasion ecology has much advanced since its early beginnings. Nevertheless, explanation, prediction, and management of biological invasions remain difficult. We argue that progress in invasion research can be accelerated by, first, pointing out difficulties this field is currently facing and, second, looking for measures to overcome them. We see basic and applied research in invasion ecology confronted with difficulties arising from (A) societal issues, e.g., disparate perceptions of invasive species; (B) the peculiarity of the invasion process, e.g., its complexity and context dependency; and (C) the scientific methodology, e.g., imprecise hypotheses. To overcome these difficulties, we propose three key measures: (1) a checklist for definitions to encourage explicit definitions; (2) implementation of a hierarchy of hypotheses (HoH), where general hypotheses branch into specific and precisely testable hypotheses; and (3) platforms for improved communication. These measures may significantly increase conceptual clarity and enhance communication, thus advancing invasion ecology. 相似文献
137.
Globally, policies aiming for conservation of species, free-flowing rivers, and promotion of hydroelectricity as renewable energy and as a means to decarbonize energy systems generate trade-offs between protecting freshwater fauna and development of hydropower. Hydroelectric turbines put fish at risk of severe injury during passage. Therefore, comprehensive, reliable analyses of turbine-induced fish mortality are pivotal to support an informed debate on the sustainability of hydropower (i.e., how much a society is willing to pay in terms of costs incurred on rivers and their biota). We compiled and examined a comprehensive, global data set of turbine fish-mortality assessments involving >275,000 individual fish of 75 species to estimate mortality across turbine types and fish species. Average fish mortality from hydroelectric turbines was 22.3% (95% CI 17.5–26.7%) when accounting for common uncertainties related to empirical estimates (e.g., handling- or catch-related effects). Mortality estimates were highly variable among and within different turbine types, study methods, and taxa. Technical configurations of hydroelectric turbines that successfully reduce fish mortality and fish-protective hydropower operation as a global standard could balance the need for renewable energy with protection of fish biodiversity. 相似文献
138.
Column experiments and model simulations were employed to evaluate the processes involved in multicomponent solute transport in a system with heterogeneous flow. Column experiments were performed with goethite embedded in polyacrylamide gel beads. The gel forms an immobile water region that can be accessed by diffusion. A two-region transport model with diffusion into spheres was combined with a surface complexation model to predict reactive transport in the goethite-gel bead system. Chromate and sulphate breakthrough curves were measured in a set of transport experiments, along with corresponding changes in the pH of the effluent. Sorption and transport of sulphate and chromate in separate columns were predicted from independently measured sorption parameters. The model overestimated the pH changes in the effluent, possibly because of proton buffering by the polyacrylamide gel. The effect of competitive sorption on transport was examined in experiments with both anions present. The model predicted the effect of competition very well in a system initially equilibrated with sulphate, followed by infiltration with chromate. However, when sulphate was infiltrated after equilibration with chromate, chromate desorption and sulphate adsorption were clearly overestimated by the transport model. The exchange between the more strongly bound chromate and the sulphate added subsequently may be too slow to cause a substantial chromate peak in the effluent. This suggests that the local equilibrium assumption was not applicable in this case. 相似文献
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