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881.
An interactive dual-circulating fluidized bed system has been proposed in which the pyrolysis of sewage sludge(SS) and incineration of biomass proceed simultaneously, and alumina is used as the bed material and heat carrier. The alumina coated with biomass ash would mix with sewage sludge in the pyrolysis reactor of this device. It is important to know the influence of composite alumina(CA) on the pyrolysis progress. Sewage sludge was pyrolyzed in a fixed bed reactor from 400 to 600°C using CA as catalyst. The effects of temperature and CA additive ratio on the products were investigated. The product yields and component distribution of non-condensable gas were more sensitive to the change of temperature, and the maximum liquid yield of 48.44 wt.% and maximum Useable Energy of Liquid of 3871 k J/kg sludge were observed at 500°C with 1/5 CA/SS(mass ratio). The gas chromatography–mass spectrometry results showed that the increase of temperature enhanced devolatilization of organic matter and promoted cyclization and aromatization of aliphatics. The presence of CA could strengthen secondary cracking and interaction among primary products from different organic compounds, such as acid–amine condensation,and reduce the content of oxygenated compounds. When the CA additive amount exceeded a certain proportion, the aromatization was clearly strengthened. The effects of CA on decomposition of fatty acids and formation of aromatics were similar to that of temperature. This means that the reaction temperature could be lowered by introducing CA, which has a positive effect on reducing energy consumption. 相似文献
882.
应用SEM-EDS结合XRF法测定了2013年8月-2014年5月昆山市7个不同地区大气PM2.5中无机元素的污染水平。研究发现,昆山地区一共可检出40种无机元素,其中主要的22种元素浓度范围在3.02~1113 ng/m3之间,合计为3784 ng/m3;PM2.5中无机元素季节变化明显,呈现春秋季高,夏冬季低的变化特点。无机元素的空间变化不大。通过富集因子的研究,Sc、Ni、Cu、Zn、As、Br、Cd、Pb、Se、Ag、Sn、Sb和Tl等13种元素EF>10,富集程度非常高,说明人类活动对这些元素的贡献较大。 相似文献
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To utilize visible light more effectively in photocatalytic reactions, a fly ash cenosphere (FAC)-supported CeO2-BiV04 (CeO2-BiVO4/FAC) composite photocatalyst was prepared by modified metalorganic decomposition and impregnation methods. The physical and photophysical properties of the composite have been characterized by X-ray diffraction (XRD), scanning electron microscope (SEM) and energy dispersive X-ray spectroscopy (EDX), X-ray photoelectron spectroscopy (XPS), and UV-Visible diffuse reflectance spectra. The XRD patterns exhibited characteristic diffraction peaks of both BiVO4 and Ce02 crystalline phases. The XPS results showed that Ce was present as both Ce4+ and Ce3+ oxidation states in Ce02 and dispersed on the surface of BiV04 to constitute a p-n heterojunction composite. The absorption threshold of the CeO2-BiVO4/FAC composite shifted to a longer wavelength in the UV-Vis absorption spectrum compared to the pure Ce02 and pure BiV04. The composites exhibited enhanced photocatalytic activity for Methylene Blue (MB) degradation under visible light irradiation. It was found that the 7.5 wt.% CeO2-BiVO4/FAC composite showed the highest photocatalytic activity for MB dye wastewater treatment. 相似文献
884.
Xue Fei Xi Lei Wang Jia Jun Hu Yu Shu Tang Yu Hu Xiao Hua Fu Ying Sun Yiu Fai Tsang Yan Nan Zhang Jin Hai Chen 《环境科学学报(英文版)》2014,26(12):2562-2570
Estuarine wetland, where freshwater mixes with salt water, comprises different regions(rivers and marine ecosystems) with significantly varying tidal salinities. Two sampling areas, ZXS and JS, were selected to investigate the effect of tidal salinity on soil respiration(SR). ZXS and JS were located in Zhongxia Shoal and Jiangyanan Shoal of Jiuduansha Wetland respectively, with similar elevation and plant species, but significantly different in salinity. The results showed that with almost identical plant biomass, the SR and soil microbial respiration(SMR) of the tidal wetland with lower salinity(JS) were significantly higher than those of the tidal wetland with higher salinity(ZXS)(p 〈 0.05). However, unlike SMR and SR, the difference in the soil microbial biomass(SMB) was not significant(p 〉 0.05)with the SMB of ZXS a little higher than that of JS. The higher SMR and SR of JS may be closely connected to the soil microbial community structures and amount of dominant bacteria. Abundant β- and γ-Proteobacteria and Actinobacteria in JS soil, which have strong heterotrophic metabolic capabilities, could be the main reason for higher SMR and SR,whereas a high number of ε-Proteobacteria in ZXS, some of which have carbon fixation ability, could be responsible for relatively lower carbon output. Path analysis indicated that soil salinity had the maximum negative total influencing coefficient with SMR among the various soil physical and chemical factors, suggesting that higher soil salinity, restricting highly heterotrophic bacteria, is the principle reason for lower SMR and SR in the ZXS. 相似文献
885.
大力发展低碳经济,是山西省转变经济发展方式、实现可持续发展的必由之路.本文从产业结构、能源结构、碳排放强度、以及山西省在全国的碳排放水平等方面分析了山西省的碳排放特征,在此基础上提出山西省的低碳发展策略. 相似文献
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河蚬(Corbicula fluminea)扰动对表层沉积物中氨氧化菌群落结构和丰度的影响 总被引:1,自引:1,他引:0
为研究不同生物量河蚬(Corbicula fluminea)的生物扰动对表层沉积物中氨氧化菌群落结构和丰度的影响,本研究设计了沉积物-水微宇宙的模拟体系,通过构建克隆文库、实时荧光定量PCR(real-time qPCR)等分子生物学方法比较不同密度河蚬扰动的沉积物中氨氧化古菌(ammonia-oxidizing archaea,AOA)和氨氧化细菌(ammonia-oxidizing bacteria,AOB)群落结构和丰度差异.结果表明,河蚬的生物扰动作用对表层沉积物氮素释放有明显的促进作用.氨氧化菌(AOA和AOB)amoA基因克隆文库中,AOA的amoA基因序列包含了已知的海洋和土壤环境中的两个分支,AOB的amoA基因绝大部分序列都属于变形菌门β亚纲(β-Proteobacteria)中的亚硝化单细胞菌属(Nitrosomonas).3个处理组表层沉积物中细菌amoA基因丰度均高于古菌amoA基因丰度,且河蚬密度越高则细菌amoA的丰度越低.同时,河蚬的添加使得微宇宙体系中氨氧化菌(AOA和AOB)的多样性降低.综上,河蚬的生物扰动对表层沉积物中氨氧化菌群落结构和丰度产生了一定的影响. 相似文献
890.
在分析1991-2002武汉市三废产生量的时间变化特征基础上,运用灰色关联度方法,定量分析了武汉市城市三废产生量的主要因子。利用灰色系统理论建立了城市三废产生量的GM(1,1)模型,模型经精度检验合格,预测了2010年武汉市三废产生量,预测结果为:武汉市三废产生量到2010年将达到432.63百万吨、3998.08亿标准立方米和678.10万吨。 相似文献