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64.
Degradation of the pharmaceutical metronidazole via UV, Fenton and photo-Fenton processes 总被引:12,自引:0,他引:12
Degradation rates and removal efficiencies of Metronidazole using UV, UV/H2O2, H2O2/Fe2+, and UV/H2O2/Fe2+ were studied in de-ionized water. The four different oxidation processes were compared for the removal kinetics of the antimicrobial pharmaceutical Metronidazole. It was found that the degradation of Metronidazole by UV and UV/H2O2 exhibited pseudo-first order reaction kinetics. By applying H2O2/Fe2+, and UV/H2O2/Fe2+ the degradation kinetics followed a second order behavior. The quantum yields for direct photolysis, measured at 254 nm and 200-400 nm, were 0.0033 and 0.0080 mol E(-1), respectively. Increasing the concentrations of hydrogen peroxide promoted the oxidation rate by UV/ H2O2. Adding more ferrous ions enhanced the oxidation rate for the H2O2/Fe2+ and UV/H2O2/Fe2+ processes. The major advantages and disadvantages of each process and the complexity of comparing the various advanced oxidation processes on an equal basis are discussed. 相似文献
65.
Endocrine disrupting compounds (EDCs) are exogenous environmental chemicals that can interfere with normal hormone function and present a potential threat to both environmental and human health. The fate, distribution and degradation of EDCs is a subject of considerable investigation. To date, several studies have demonstrated that conventional water treatment processes are ineffective for removal of most EDCs and in some instances produce multiple unknown transformation products. In this study we have investigated the use of direct photolysis with low-pressure (LP) Hg UV lamps and UV+hydrogen peroxide (H(2)O(2)) advanced oxidation process (AOP) for the degradation of a prototypic endocrine disrupter, bisphenol A (BPA), in laboratory water. Removal rates of BPA and formation of degradation products were determined by high performance liquid chromatography (HPLC) analysis. Changes in estrogenic activity were evaluated using both in vitro yeast estrogen screen (YES) and in vivo vitellogenin (VTG) assays with Japanese medaka fish (Oryzias latipes). Our results demonstrate that UV alone did not effectively degrade BPA. However, UV in combination with H(2)O(2) significantly removed BPA parent compound and aqueous estrogenic activity in vitro and in vivo. Removal rates of in vivo estrogenic activity were significantly lower than those observed in vitro, demonstrating differential sensitivities of these bioassays and that certain UV/AOP metabolites may retain estrogenic activity. Furthermore, the UV/H(2)O(2) AOP was effective for reducing larval lethality in treated BPA solutions, suggesting BPA degradation occurred and that the degradation process did not result in the production of acutely toxic intermediates. 相似文献
66.
Canopy leaf area index (LAI) is an important structural parameter of the vegetation controlling pollutant uptake by terrestrial ecosystems. This paper presents a computationally efficient algorithm for retrieval of vegetation LAI and canopy clumping factor from satellite data using observed Simple Ratios (SR) of near-infrared to red reflectance. The method employs numerical inversion of a physics-based analytical canopy radiative transfer model that simulates the bi-directional reflectance distribution function (BRDF). The algorithm is independent of ecosystem type. The method is applied to 1-km resolution AVHRR satellite images to retrieve a geo-referenced data set of monthly LAI values for the conterminous USA. Satellite-based LAI estimates are compared against independent ground LAI measurements over a range of ecosystem types. Verification results suggest that the new algorithm represents a viable approach to LAI retrieval at continental scale, and can facilitate spatially explicit studies of regional pollutant deposition and trace gas exchange. 相似文献
67.
András Bardossy Arne Färber Steffen Schönau Bernhard Westrich Thomas Jancke Gerhard Schmid Sven Wurms Karl Stahr Thomas Gaiser Harald Frauenknecht Thilo Streck Joachim Ingwersen Claudia Kreschnak Ulrich Kern Hilke Heppelmann Ekkehard Christoffels Ulrich Förstner Patrick Jacobs 《Environmental Sciences Europe》2006,18(1):67-69
68.
Summary We develop a model for the distribution of animals around encounter sites. It is particularly applicable to males attending mate-encounter sites, such as hilltops. Major predictions are: male distributions should be unstable; males should show little site tenacity, particularly when at low densities; males with low probability of mate capture should occupy subordinate positions; probability of mate capture is a better predictor of position than resource-holding potential; female choice favours despotic distributions; males should often patrol together. Several of these predictions are met, others are testable. We identify some parameters that should be more extensively studied. 相似文献
69.
A technique for measuring rates of RNA and DNA synthesis in sedimentary microbial communities has been adapted from methods developed for marine and freshwater microplankton research. The procedure measures the uptake, incorporation and turnover of exogenous [2, 3H]-adenine by benthic microbial populations. With minor modification, it is applicable to a wide range of sediment types. Measurement of nucleic acid synthesis rates are reported from selected benthic marine environments, including coral reef sediments (Kaneohe Bay, Oahu, Hawaii), intertidal beach sands (Oahu and southern California) and California borderland basin sediment (San Pedro Basin), and comparisons are made to selected water-column microbial communities. Biomass-specific rates of nucleic acid synthesis in sediment microbial communities were comparable to those observed in water-column assemblages (i.e., 0.02 to 2.0 pmol deoxyadenine incorporated into DNA [ng ATP]-1 h-1 and 0.2 to 8.9 pmol adenine incorporated into RNA [ng ATP]-1 h-1). DNA synthesis rates were used to calculate carbon production estimates ranging from 2 g C cm-3 h-1 in San Pedro Basin sediment (880 m water depth) to 807 g C cm-3 h-1 in coral reef sediment from the Kaneohe Bay. Microbial community specific growth rate, (d-1), estimated from DNA synthesis rates in surface sediments ranged from 0.1 in San Pedro Basin to 4.2 in Scripps Beach (La Jolla, California) intertidal sand. 相似文献
70.
Cycles of storm destruction and rebuilding of human facilities are as much a part of a predictable cycle of shoreline change
as destruction and re-establishment of landforms and wildlife habitat by natural processes. An evaluation of the human-induced
and natural geomorphic responses to three storms in two vulnerable developed areas in New Jersey reveals that storms can have
limited effect in re-establishing a natural coastal resource base of lasting significance. Reconstruction of coastal landscapes
by human action may be more rapid than natural restoration, decreasing the likelihood for geomorphic features to develop based
on natural processes. Reliance on storm processes to create new natural habitat in locations where there is human investment
in buildings and support infrastructure is not realistic unless a proactive stance is taken to include naturally-functioning
characteristics of the coastal system in reconstruction efforts. By striving to control construction of shorefront buildings
to reduce their potential for damage, managers may be taking attention away from the separate but critical issue of ensuring
that post-storm reconstruction effort include the potential for replacing loss of natural geomorphic features and wildlife
habitat. 相似文献