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21.
Samples obtained from an industrialized valley in the East Alpine region were collected daily for a half year and analyzed using X-ray fluorescence to examine the elements Si,Al,Fe,Ca,Mg,Na,K,Zn,P,S and Cl.Some factors affecting the changes of these elements were considered,including time,elemental correlations,weekday,weekend and seasonal changes.Diagnostic analysis provided an insight into a decoupling behavior that occursin siliceous and carbonates minerals.A decrease in Si and Al and an increase in carbonates,Na,K,Zn and P were observed during the cold season.However,a consistently high correlation of Si and Al was observed in all seasons.It was established that such high levels originated from street surface abrasion.The increase in variability and absolute levels of carbonates during the cold season was demonstrated by adding carbonates to the street surface as gritting material to increase the grip on snowy surfaces.A marked increase in Na and Cl was observed in winter which may have been caused by thaw salt that is widely used in winter in Austria.This was associated with a significant increase in K,Zn,and P in the cold season that was the result of domestic space heating with wood.PM10 levels in December were 12 μg/m3 and were higher than levels detected in July.It was established that such high levels originated from mineral oxides,wood smoke,and inorganic ionic material(s). 相似文献
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Photoelectrocatalytic degradation of 4-chlorophenol and oxalic acid on titanium dioxide electrodes 总被引:26,自引:0,他引:26
Photocatalytically active thin TiO(2) films were produced by spin-coating or dip-coating an alkoxy precursor onto a transparent conducting electrode substrate and by thermal oxidation of titanium metal. The thin films were used to study the photoelectrocatalytic or photoelectrochemical degradation of oxalic acid and 4-chlorophenol (4-CP) under near UV (monochromatic, 365 nm) light irradiation. Degradation was monitored by a variety of methods. In the course of oxalic acid degradation, CO(2) formation accounted for up to 100% of the total organic carbon degradation for medium starting concentrations; for the degradation of 4-CP, less CO(2) was detected due to the higher number of oxidation steps, i.e. intermediates. Incident-photon-to-current conversion efficiency, educt degradation and product formation as well as Faradaic efficiencies were calculated for the degradation experiments. Quantum yields and Faradaic efficiencies were found to be strongly dependent on concentration, with maximum values (quantum yield) around 1 for the highest concentrations of oxalic acid. 相似文献
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Marian Leimbach Nico Bauer Lavinia Baumstark Ottmar Edenhofer 《Environmental Modeling and Assessment》2010,15(3):155-173
Within this paper, we present the novel hybrid model REMIND-R and its application in a climate policy context based on the
EU target to avoid a warming of the Earth’s atmosphere by more than 2°C compared to the pre-industrial level. This paper aims
to identify necessary long-term changes in the energy system and the magnitude of costs to attain such a climate protection
target under different designs of the post-2012 climate policy regime. The regional specification of mitigation costs is analyzed
in the context of globalization where regions are linked by global markets for emission permits, goods, and several resources.
From simulation experiments with REMIND-R, it turns out that quite different strategies of restructuring the energy system
are pursued by the regions. Furthermore, it is demonstrated that the variance of mitigation costs is higher across regions
than across policy regimes. First-order impacts, in particular, reduced rents from trade in fossil resources, prevail regardless
of the design of the policy regime. 相似文献
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Konstantinova Elizaveta Burachevskaya Marina Mandzhieva Saglara Bauer Tatiana Minkina Tatiana Chaplygin Victor Zamulina Inna Konstantinov Alexandr Sushkova Svetlana 《Environmental geochemistry and health》2022,44(2):349-368
Environmental Geochemistry and Health - Lake Atamanskoye is one of the most polluted aquatic environments in the South of Russia. This water body was affected by long-term pollution by effluent... 相似文献