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41.
The shrink-swell behavior of active clays in response to changes in physicochemical conditions creates great challenges for construction of geotechnical barriers for hazardous waste isolation, and is of significant importance for management of agricultural and natural resources. Initiation and evolution of desiccation cracks in active clays are strongly dependent on physicochemical initial and boundary conditions. To investigate effects of bentonite content (20, 40, 60%), pore fluid chemistry (0.05 and 0.5M NaCl) and drying rates (40 and 60°C) on cracking behavior, well-controlled dehydration experiments were conducted and X-ray Computed Tomography (CT) was applied to visualize and quantify geometrical features of evolving crack networks. A stochastic model based on the Fokker-Plank equation was adopted to describe the evolution of crack aperture distributions (CAD) and to assess the impact of physicochemical factors on cracking behavior. Analyses of crack porosity and crack specific surface area showed that both clay content and temperature had larger impact on cracking than pore fluid concentration. More cracks formed at high bentonite contents (40 and 60%) and at high drying rate (60°C). The drift, diffusion and source terms derived from stochastic analysis indicated that evaporative demand had greater influence on the dynamics of the CAD than solution chemistry. 相似文献
42.
Stefanie Grund Eric Higley René Schönenberger Marc J-F. Suter John P. Giesy Markus Hecker Henner Hollert 《Environmental science and pollution research international》2011,18(3):446-460
Introduction
The present study was part of a comprehensive weight-of-evidence approach with the goal of identifying potential causes for the declines in fish populations, which have been observed during the past decades in the Upper Danube River. 相似文献43.
De Maria S Rivelli AR Kuffner M Sessitsch A Wenzel WW Gorfer M Strauss J Puschenreiter M 《Chemosphere》2011,84(9):1256-1261
Although the beneficial effects on growth and trace element accumulation in Salix spp. inoculated with microbes are well known, little information is available on the interactions among trace elements and macronutrients. The main purpose of this study was to assess the effect of phytoaugmentation with the rhizobacteria Agromyces sp., Streptomyces sp., and the combination of each of them with the fungus Cadophora finlandica on biomass production and the accumulation of selected trace elements (Zn, Cd, Fe) and macronutrients (Ca, K, P and Mg) in Salix caprea grown on a moderately polluted soil. Dry matter production was significantly enhanced only upon inoculation with Agromyces sp. Regarding the phytoextraction of Cd and Zn, shoot concentrations were mostly increased after inoculation with Streptomyces sp. and Agromyces sp. + C. finlandica. These two treatments also showed higher translocation factors from roots to the leaves for both Cd and Zn. The accumulation of Cd and Zn in shoots was related to increased concentrations of K. This suggests that microorganisms that contribute to enhanced phytoextraction of Cd and Zn affect also the solubility and thus phytoavailability of K. This study suggests that the phytoextraction of Zn and Cd can be improved by inoculation with selected microbial strains. 相似文献
44.
Developing Effective Decision Support for the Application of “Gentle” Remediation Options: The GREENLAND Project
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Andy Cundy Paul Bardos Markus Puschenreiter Nele Witters Michel Mench Valerie Bert Wolfgang Friesl‐Hanl Ingo Müller Nele Weyens Jaco Vangronsveld 《补救:环境净化治理成本、技术与工艺杂志》2015,25(3):101-114
Gentle remediation options (GRO) are risk management strategies/technologies that result in a net gain (or at least no gross reduction) in soil function as well as risk management. They encompass a number of technologies, including the use of plant (phyto‐), fungi (myco‐), and/or bacteria‐based methods, with or without chemical soil additives or amendments, for reducing contaminant transfer to local receptors by in situ stabilization, or extraction, transformation, or degradation of contaminants. Despite offering strong benefits in terms of risk management, deployment costs, and sustainability for a range of site problems, the application of GRO as practical on‐site remedial solutions is still in its relative infancy, particularly for metal(loid)‐contaminated sites. A key barrier to wider adoption of GRO relates to general uncertainties and lack of stakeholder confidence in (and indeed knowledge of) the feasibility or reliability of GRO as practical risk management solutions. The GREENLAND project has therefore developed a simple and transparent decision support framework for promoting the appropriate use of gentle remediation options and encouraging participation of stakeholders, supplemented by a set of specific design aids for use when GRO appear to be a viable option. The framework is presented as a three phased model or Decision Support Tool (DST), in the form of a Microsoft Excel‐based workbook, designed to inform decision‐making and options appraisal during the selection of remedial approaches for contaminated sites. The DST acts as a simple decision support and stakeholder engagement tool for the application of GRO, providing a context for GRO application (particularly where soft end‐use of remediated land is envisaged), quick reference tables (including an economic cost calculator), and supporting information and technical guidance drawing on practical examples of effective GRO application at trace metal(loid) contaminated sites across Europe. This article introduces the decision support framework. ©2015 Wiley Periodicals, Inc. 相似文献
45.
Mathias Gadegast Ulrike Hirt Dieter Opitz Markus Venohr 《Regional Environmental Change》2012,12(3):571-580
Studies of nutrient emissions into surface waters are usually only performed for years in recent decades. However, estimating nutrient emissions for the more distant past enables us to identify the main factors responsible for the increasing nutrient contamination since the end of the nineteenth century. We focussed on the Oder River System for 1875–1944, divided into 10-year periods. Nutrient emissions into surface waters were calculated with the model MONERIS (MOdelling Nutrient Emissions in RIver Systems). For seven different pathways and eight sources, the total nitrogen (TN) emissions were quantified. The TN-emissions into the surface waters for 1880 amounted to 25,300 t?year?1, and by 1940, this value had almost doubled to 46,600?t?year?1. In 1880, 57% of TN-emissions into the surface waters derived from urban systems, due to the high amount of untreated waste water. In 1940, only 34% of TN-emissions into surface waters derived from urban systems, despite a population growth of about 27% since 1880; point sources via newly constructed waste water treatment plants (WWTPs) increased from 4% (1880) to 26% (1940). During the study period, the main changes in diffuse TN-emissions from agriculture were caused by inorganic fertilizer application and nitrogen deposition, while TN-emissions via urban sources were shifted to point sources due to population growth and the construction of new WWTPs. Furthermore, estimated TN-concentrations could make a contribution to construct benchmarks for nutrient concentrations according to the physiochemical properties to implement the European Water Framework Directive (WFD 2000). 相似文献
46.
Thorsten Bartels-Rausch Marcello Brigante Yasin F. Elshorbany Markus Ammann Barbara D'Anna Christian George Konrad Stemmler Marieme Ndour Jörg Kleffmann 《Atmospheric environment (Oxford, England : 1994)》2010,44(40):5443-5450
Laboratory studies on the heterogeneous conversion of nitrogen dioxide into nitrous acid on irradiated ice films containing humic acid are described. It was found that the presence of light in the visible range of the solar spectrum significantly enhances the rate of nitrous acid release from a humic acid doped ice film. This process might contribute to observed HONO production in snow, where the NO2 is thought to originate from nitrate photolysis. Analysis of the experimental data based on the Langmuir Hinshelwood model framework allowed quantification of the observed dependencies of the nitrous acid production rate on nitrogen dioxide concentration. The observed dependencies on the humic acid concentration as well as on the irradiation intensity were used to estimate light-driven HONO fluxes for environmental snow covers. 相似文献
47.
48.
Reiner Jaakson 《Journal of the American Water Resources Association》1973,9(6):1225-1233
ABSTRACT: Water-based outdoor recreation constitutes an important benefit in many multiple-use projects. One problem frequently encountered, however, is the fluctuation of the water-level in a reservoir, especially if draw-downs occur during the summer recreation season. The Trent Canal in Ontario, Canada, forms a unique recreation waterway of some 240 miles of canal and navigable lakes and rivers. For the control of the water in the canal, the Canadian Federal government manages 44 reservoir-lakes as water-storage sites to augment the flows in the canal. While most disputes in water allocation for recreation generally involve recreation uses versus other, non-recreation uses, in the case of the Trent Canal and its reservoir-lakes the dispute in water allocation exists between two competing recreation-uses: for recreation boating on the Canal and its waterway, and for recreation use of the reservoir-lakes. Each use has its own duty-of-water in terms of requirements, or water conditions, for its optimum use. On the reservoir-lakes, by far the largest recreation user-group, is made up of the owners of private shoreline summer cottages (cabins). Draw-downs on the reservoir-lakes, in some cases as much as 13 feet, hence constitute a negative externality imposed by the canal, especially since water-level lowering takes place continuously throughout the summer. In-depth interviews conducted with over 100 cottage-owners indicate four main conclusions. First, the previous user assumptions of the extent of the negative effect of water-level fluctuation on recreation had been exaggerated. Only in extreme draw-downs during infrequent dry years would draw-down constitute a serious imposition. Second, water-level fluctuation does constitute a form of inconvenience to the private riparian recreation property owners, but it does not generally reduce the quantity of recreation use of the reservoir-lakes. Third, there is evidence that reservoir-lake users have learned to adapt successfully to water-level draw-downs. Fourth, the shoreline physiography of the location of a riparian owner strongly influences the way in which draw-down affects attitudes and opinions. The complex jurisdictional split of the land and water resources of the region points to the need to establish a Trent Canal Authority, to oversee the proper use and development of the canal, its waterway, and the reservoir-lakes. 相似文献
49.
50.
Markus Hauck Sascha-René Jürgens Christoph Leuschner 《Environmental pollution (Barking, Essex : 1987)》2009,157(10):2776-2780
The depsidone fumarprotocetraric acid as well as the depsides perlatolic and thamnolic acids are lichen secondary metabolites. Their first dissociation constants (pKa1) in methanol were determined to be 2.7 for perlatolic acid and 2.8 for fumarprotocetraric and thamnolic acids by UV spectroscopy. Lower pKa1 values are, so far, not known from lichen substances. Several lichens producing at least one of these compounds are known for their outstanding tolerance to acidic air pollution. This is demonstrated by evaluating published pH preferences for central European lichens. The low pKa1 values suggest that strong dissociation of the studied lichen substances is a prerequisite for the occurrence of lichens with these compounds on very acidic substrata, as protonated lichen substances of different chemical groups, but not their conjugated bases, are known to shuttle protons into the cytoplasm and thereby apparently damage lichens. 相似文献