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11.
Oguchi M Murakami S Sakanakura H Kida A Kameya T 《Waste management (New York, N.Y.)》2011,31(9-10):2150-2160
End-of-life electrical and electronic equipment (EEE) has recently received attention as a secondary source of metals. This study examined characteristics of end-of-life EEE as secondary metal resources to consider efficient collection and metal recovery systems according to the specific metals and types of EEE. We constructed an analogy between natural resource development and metal recovery from end-of-life EEE and found that metal content and total annual amount of metal contained in each type of end-of-life EEE should be considered in secondary resource development, as well as the collectability of the end-of-life products. We then categorized 21 EEE types into five groups and discussed their potential as secondary metal resources. Refrigerators, washing machines, air conditioners, and CRT TVs were evaluated as the most important sources of common metals, and personal computers, mobile phones, and video games were evaluated as the most important sources of precious metals. Several types of small digital equipment were also identified as important sources of precious metals; however, mid-size information and communication technology (ICT) equipment (e.g., printers and fax machines) and audio/video equipment were shown to be more important as a source of a variety of less common metals. The physical collectability of each type of EEE was roughly characterized by unit size and number of end-of-life products generated annually. Current collection systems in Japan were examined and potentially appropriate collection methods were suggested for equipment types that currently have no specific collection systems in Japan, particularly for video games, notebook computers, and mid-size ICT and audio/video equipment. 相似文献
12.
Yuuki Miyata Kensuke Miyazaki Masahiro Miura Yasutaka Shimotori Masakazu Aoyama Hisayuki Nakatani 《Journal of Polymers and the Environment》2013,21(1):115-121
A novel solventless delignification of a defatted Picea glehnii wood flour sample was performed using a TiO2/polyethylene oxide (PEO) photocatalyst system. A cell wall structure of the wood flour was directly observed, showing that its lignin fraction was removed by the photodegradation. The total lignin amount was slightly decreased as compared with that of the pristine sample, and the vanillin formation was confirmed by the 1H-NMR measurement. The TiO2 worked as a radical initiator, and simultaneously acid and aldehyde compounds produced by the PEO photolysis did as an accelerator for the solventless delignification. Although the photocatalyst system showed high delignification activity even for a low molecular lignin model, the delignification of the wood flour sample was confined to the surface. It was found that the suppressed delignification behavior was due to crosslinked structure of lignin. 相似文献
13.
Masahiro?ShimadaEmail author Takahiko?Iida Kensuke?Kawarada Yoshifumi?Chiba Toshihiro?Mamoto Takayuki?Okayama 《Journal of Material Cycles and Waste Management》2004,6(2):111-118
We have previously manufactured activated carbon using waste paper board, which was prepared by adding 8% phenol resin adhesive to torn waste newspaper and hot-pressing. In this study, the pretreatment process of the raw material was simplified; the waste paper was extruded to form granules. The activated carbon was manufactured by the carbon dioxide activation method using the granules as the raw material. The properties of the activated carbon were evaluated based on the pore structure, the iodine adsorption number, and the adsorption of toluene vapor in a sealed chamber. The activated carbon, which was manufactured at an activation temperature of 1100°C and a treatment time of 60min, exhibited a specific surface area of 1241m2/g and an iodine adsorption number of 1120mg/g. These results were similar to those obtained for two commercially available activated carbons. The extent of toluene vapor adsorption by this activated carbon was similar to that observed for the two commercial activated carbons over a period of 130min. 相似文献
14.
Biodegradation of Polycaprolactone Powders Proposed as Reference Test Materials for International Standard of Biodegradation Evaluation Method 总被引:1,自引:0,他引:1
Masahiro Funabashi Fumi Ninomiya Masao Kunioka 《Journal of Polymers and the Environment》2007,15(1):7-17
Polycaprolactone (PCL) powders were prepared from PCL pellets using a rotation mechanical mixer. PCL powders were separated
by sieves with 60 and 120 meshes into four classes; 0–125 μm, 125–250 μm, 0–250 μm and 250–500 μm. Biodegradation tests of
PCL powders and cellulose powders in an aqueous solution at 25°C were performed using the coulometer according to ISO 14851.
Biodegradation tests of PCL powders and cellulose powders in controlled compost at 58°C were performed by the Mitsui Chemical
Analysis and Consulting Service, Inc. according to ISO 14855-1 and by using the Microbial Oxidative Degradation Analyzer (MODA)
instrument according to ISO/DIS 14855-2. PCL powders were faster biodegraded than cellulose powders. The reproducibility of
biodegradation of PCL powders is excellent. Differences in the biodegradation of PCL powders with different class were not
observed by the ISO 14851 and ISO/DIS 14855-2. An enzymatic degradation test of PCL powders with different class was studied
using an enzyme of Amano Lipase PS. PCL with smaller particle size was faster degraded by the enzyme. PCL powders with regulated sizes from 125 μm to 250 μm
are proposed as a reference material for the biodegradation test. 相似文献
15.
16.
将20头荷斯坦产奶奶牛随机分为对照组和试验Ⅰ~Ⅲ组,对照组饲喂全混日粮(TMR),试验Ⅰ组每头奶牛每天饲喂TMR加150.0 g复合脂肪酸,试验Ⅱ组每头奶牛每天饲喂TMR加150.0 g乳酸,试验Ⅲ组每头奶牛每天饲喂TMR加150.0 g复合脂肪酸/乳酸(质量比为1∶1),分析探讨了复合脂肪酸和乳酸对奶牛粪尿、氮、总磷排泄量和CH4释放量的影响.结果表明,相比对照组,试验Ⅲ组1头奶牛1年CH4释放量减少30.64 kg,粪尿、氮、总磷排泄量分别减少1.43 t、28.32 kg和2.36 kg,标准乳(FCM)提高3.28%.在奶牛饲料中添加乳酸和复合脂肪酸的混合酸,能有效抑制奶牛对土壤、水体及空气的污染,显著提高奶牛的生态效益和经济效益. 相似文献
17.
Use of X-ray absorption imaging to examine heterogeneous diffusion in fractured crystalline rocks 总被引:1,自引:0,他引:1
Altman SJ Uchida M Tidwell VC Boney CM Chambers BP 《Journal of contaminant hydrology》2004,69(1-2):1-26
Heterogeneous diffusion in different regions of a fractured granodiorite from Japan has been observed and measured through the use of X-ray absorption imaging. These regions include gouge-filled fractures, recrystallized fracture-filling material and hydrothermally altered matrix. With the X-ray absorption imaging technique, porosity, relative concentration, and relative mass of an iodine tracer were imaged in two dimensions with a sub-millimeter pixel size. Because portions of the samples analyzed have relatively low porosity values, imaging errors can potentially impact the results. For this reason, efforts were made to better understand and quantify this error. Based on the X-ray data, pore diffusion coefficients (Dp) for the different regions were estimated assuming a single diffusion rate and a lognormal multirate distribution of Dp. Results show Dp for the gouge-filled fractures are over an order of magnitude greater than those of the recrystallized fracture-filling material, which in turn is approximately two times greater than those for the altered matrix. The recrystallized fracture-filling material was found to exhibit the greatest degree of variability. The results of these experiments also provide evidence that diffusion from advective zones in fractures through the gouge-filled fractures and recrystallized fracture-filling material could increase the pore space available for matrix diffusion. This evidence is important for understanding the performance of potential nuclear waste repositories in crystalline rocks as diffusion is thought to be an important retardation mechanism for radionuclides. 相似文献
18.
Leaching characteristics of polycyclic aromatic hydrocarbons (PAHs) from spiked sandy soil 总被引:8,自引:0,他引:8
In order to evaluate the factors affecting leachability of hydrophobic organic pollutants (HOPs), we performed leaching tests under a variety of conditions using sandy soil contaminated with phenanthrene and pyrene. The results obtained were: (1) the shaking time, temperature, and dissolved humic matter (DHM, as coexisting matter) increased leachability; (2) ionic strength reduced leachability; and (3) the liquid-to-solid ratio and pH level had no effect on leaching concentration of HOPs. In DHM-added leaching tests assuming equilibrium with HOPs, DHM, and solid matrix, the partitioning (binding) coefficient of HOPs to DHM was accurately calculated with the equations proposed in this study. While we recommend taking into consideration the coexistence of DHM, it is difficult to use universally because its properties differ according to origin and extracting method. It is therefore reasonable to use an alternative reagent having an effect similar to that of DHM. 相似文献
19.
Hideo Okamura Masahiro Yagi Masanobu Kawachi Takeaki Hanyuda Hiroshi Kawai Iain Walker 《毒物与环境化学》2013,95(3):545-556
The environmental impact of two biocide-free antifouling paints, fluoropolymer and silicone types, painted on a test cylinder was assessed using a battery of ecotoxicity test and chemical analyses for organic micro-pollutants such as perfluoroalkyl substances (PFAS). A biocide paint containing zinc pyrithione (ZnPT2) and cuprous oxide was assessed as a positive control. A standardized laboratory rotating-cylinder method using each test cylinder with artificial seawater was performed for 45 days. After 1?h rotation, the leaked seawater was subjected for bioassay and chemical analyses twice weekly. The seawater extracts from the biocide paint showed adverse effects on bacteria, algae, and crustaceans, but those from the biocide-free paints did not. The leakage seawater from biocide-free paints, after 7-day continuous rotation, contained the same concentration levels of PFAS as blank seawater used to conduct the tests. Thus, no significant toxicities of the biocide-free paints were found under the conditions of this study. Simultaneous analysis of ZnPT2 and copper pyrithione (CuPT2) was developed using an HPLC with a polymeric resin column, showing that ZnPT2 was converted to CuPT2 by trans-chelation in the leakage seawater from the positive control paint. The experimental results using a laboratory rotating-cylinder method demonstrated that biocide-free paints did not markedly affect three species tested and no PFAS was detected. In contrast, biocide paint was significantly toxic to test species and toxicity of the extract on bacteria was partly responsible for CuPT2 produced in leakage seawater. Thus, a laboratory rotating-cylinder method may be applied for ecotoxicological assessment of antifouling paints. 相似文献
20.
The bumblebee Bombus terrestris is not only an effective pollinator, but also a potential invasive alien species outside its native range. Recently, nearly
30% of queens of the Japanese native species Bombus hypocrita sapporoensis and B. hypocrita hypocrita were estimated to copulate with B. terrestris males in the field, suggesting that indigenous bumblebees could be genetically deteriorated through hybrid production with
the introduced species. In this study, we evaluated hybrid production between the introduced B. terrestris and the indigenous B. hypocrita sapporoensis under laboratory conditions. The hatching rate of eggs derived from interspecific matings was 0% and 8.6% depending on the
direction of the cross, which was significantly lower than that from intraspecific matings of B. terrestris (76.9%) and B. hypocrita sapporoensis (78.9%). Genetic studies using microsatellite markers revealed that both haploid and diploid individuals were present in
the egg stage, whereas all hatched larvae were haploid. In addition, histological studies revealed that eggs derived from
interspecific matings terminated development 2 days after oviposition. These results strongly suggested that eggs derived
from interspecific matings are inviable due to post-mating isolation mechanisms. Mass release of exotic pollinators could
cause serious population declines of native bumblebee species. 相似文献