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61.
Mitsuhiro Kubota Masahiro Hayashi Hitoki Matsuda Hirokazu Serizawa 《Journal of Material Cycles and Waste Management》2012,14(2):132-138
Combined ultrasonic (US) irradiation and sodium peroxodisulfate (Na2S2O8) treatment has been investigated for promotion of both decomposition of (4-chloro-2-methylphenoxy) acetic acid (MCPA) and mineralization of organic residues. This treatment is expected to accelerate both reactions, because the US cavitation effect promotes the production of radicals, such as SO 4 ? · and OH·, by the decomposition of Na2S2O8 and water. In this study, decomposition experiments were performed on 100?ppm MCPA aqueous solutions in a sonoreactor at reaction temperatures of 298?C333?K with US irradiation alone, Na2S2O8 treatment alone, and the combination of US and Na2S2O8 treatment. It was found that the combined treatment achieved a higher MCPA decomposition rate and total organic carbon (TOC) removal ratio than either treatment alone. The decomposition ratios of both MCPA and TOC increased with reaction temperature, and especially steep increases were observed at 333?K due to a significant promotion of thermal decomposition of Na2S2O8. The production of radical species was also promoted by the combined treatment. These results suggest that the higher MCPA decomposition rate and TOC removal ratio are due to the increased formation of sulfate and hydroxyl radicals via thermal and US decomposition of Na2S2O8. 相似文献
62.
Koji Tokimatsu Masahiko Aicha Kentaro Yoshida Masahiro Nishio Eiichi Endo Masaji Sakagami 《国际发展与全球生态学杂志》2016,23(6):541-552
We need a consistent methodology to measure the co-benefits of climate change mitigation across Asian countries. This study chose a strategy of modifying the Japan-specific life-cycle impact assessment method based on endpoint modeling (LIME) for wider application across countries. LIME has two dimensions. First, it is an environmental science that links the cause-and-effect chain. Second, it is an environmental valuation that weighs four endpoint damages in monetary terms through a conjoint analysis that is derived from an Internet-based questionnaire survey. This article describes the modification of the methodology for application of the conjoint analysis to weigh environmental impacts. We approached the investigation as follows. First, we conducted Internet surveys to measure marginal willingness-to-pay (MWTP). We used a sample of 112 respondents in their 20 s to 40 s, divided equally between men and women, in 11 cities across China, India, and Southeast Asia. The results obtained showed clear statistical significance and were comparable across the cities. Second, we attempted to develop functions (called benefit transfer functions) to simplify the measured MWTP in order to apply it across different Asian countries. The functions were derived through a stepwise meta-analytic method, a type of multiple regression analysis whose independent variable was MWTP and dependent variables were attributes of both respondents and surveyed cities. The functions showed that coal consumption and percentage of nature reserve were dependent variables. Then, the MWTPs estimated from the functions were compared with the measured MWTP for transfer error, which is calculated by the absolute value of the difference between the estimated value and the measured value divided by the latter. The transfer error was below 50% in about 90% of the 44 results (a combination of four endpoints and 11 cities), implying that the developed functions were statistically significant. 相似文献
63.
Leaching characteristics of polybrominated diphenyl ethers (PBDEs) from flame-retardant plastics 总被引:1,自引:0,他引:1
To investigate the effect of leachant on the leachability of polybrominated diphenyl ethers (PBDEs), we determined the leaching concentrations of PBDEs from flame-retardant plastic samples (TV housings and raw materials before molding processing) that are regarded as a source of PBDEs in landfill sites. The leachants used were distilled water, 20% methanol solution, and dissolved humic solution (DHS) of 1000 mg/l based on organic carbon. The leaching test conditions were a liquid-to-solid ratio of 100:1, and a contact period of five days, with twice-daily agitation in a temperature-controlled room of 30 degrees C without pH or ionic strength control. The leaching concentrations of PBDEs increased with increased content, and were found to be remarkably enhanced when methanol and DHS were used instead of distilled water. The enhancement of leachability in the presence of the latter was attributed to the cosolvency effect, and complex formations between the PBDEs and dissolved humic matter (DHM). PBDE concentrations in the leachate obtained from the leaching test and an actual landfill site revealed a significant presence of congeners below heptabromodiphenyl ethers (H7BDEs), detected in the leachate of the actual landfill, while significant amounts of nonabromodiphenyl ethers (N9BDEs) and decabromodiphenyl ether (D10BDE) were detected in the leachate of the leaching test. 相似文献
64.
Leachate samples were taken from seven different landfills and concentrations of brominated flame retardants (BFRs), i.e. polybrominated diphenyl ethers (PBDEs) and tetrabromobisphenol A (TBBPA), were quantified. Leaching characteristics of BFRs, especially factors affecting leachability, were clarified to obtain basic information regarding the release of BFRs into the environment. The results obtained for observed levels of the sum of PBDE-47, -99 and -100 were n.d.--4000 pg/l for the raw leachate and n.d. for the treated one, respectively, and those of TBBPA were n.d.--620,000 pg/l for the raw leachate and n.d.--11,000 pg/l for the treated one, respectively. Three sites that not only had crushed material from bulk wastes such as waste electric and electronic equipment, but also were under operation or within a year since closure, indicated a higher concentration of BFRs than the other sites. In particular extremely high concentration of PBDEs was observed at a site with a large amount of organics. Considering the leaching characteristics of BFRs, there exists the possibility that leachability of PBDEs is influenced by the presence of dissolved humic matter (DHM) in the leachate. The high removal efficiency for BFRs in the leachate treatment process was also confirmed. 相似文献
65.
The leaching behavior of dioxins from raw and treated fly ash (FA) under the coexistence of several types of surface-active agents (SAAs) was examined by batch leaching tests to obtain significant information not only for evaluating leachability of dioxins as hydrophobic organic pollutants (HOPs) under the severe environment in which SAAs coexist, but also for evaluating the reduction efficiency of dioxin-leachability from the treated FA. Enhancement of dioxin-leachability by sufficient addition of SAAs was observed in the leaching test, whereas addition of a smaller quantity depressed the leachability. The higher the degree of chlorination in PCDDs/PCDFs homologues, the more effectively the SAAs enhanced the leachability. Moreover, there was a large difference in the potential for leachability enhancement due to each surface activity, based on critical micelle concentration (CMC) of the SAAs although Aldrich humic acid enhanced the leachability at a much lower concentration than CMC. A comparison of the leachability in FA treated by several methods showed a difference in the reduction efficiency of leachability, depending on the adsorption of SAAs by each treated FA. 相似文献
66.
Sánchez-Bayo F Yamashita H Osaka R Yoneda M Goka K 《Journal of environmental science and health. Part. B》2007,42(3):279-286
To elucidate the ecological impacts of imidacloprid [1-(6-chloro-3-pyridylmethyl)-N-nitroimidazolidin-2-ylideneamine] on vegetable crops and their surrounding areas, arthropods on eggplant patches treated with this insecticide were monitored throughout two cultivation seasons, spring and autumn, and the results compared with those of control crops. Residues of imidacloprid in soil accounted for 4-8% of total applied, and concentrations outside the crop were always below 5 micro g/kg. Communities of the crop vegetation experienced significant density reductions, mostly of aphids, and had fewer species diversity during the first month. Those in the surrounding pasture were similarly affected though with less intensity, while non-target ground arthropods both inside and outside the crop only showed significant impacts in the two weeks after planting. 相似文献
67.
Akira Iguchi Shinpei Takai Masahiro Ueno Tsuneo Maeda Takashi Minami Isao Hayashi 《Marine Biology》2007,151(1):31-39
The population structures of Buccinum tsubai and Neptunea constricta were compared using partial sequences of the mitochondrial COI gene. B. tsubai included four genetically distinguishable subpopulations (Hokkaido, Yamagata-Toyama, Yamato Bank, and San’in), which is consistent
with the results of our previous study using mitochondrial 16SrRNA sequences. The genetic structure of N. constricta was also clear, but the lineage sorting corresponding to the geographical distribution was not as clear as that of B. tsubai. The difference between the genetic structures of these two species might be due to a difference in either their dispersal
abilities or the historic distribution patterns in the Sea of Japan. The fossil record and nested clade analyses support the
latter alternative. The four subpopulations of B. tsubai are estimated to have diverged 0.42–1.46 million years ago, providing support for the existence of intermediate water of
normal salinity and oxygen concentration capable of sustaining B. tsubai between the low-salinity surface water and anoxic deep water during the Pleistocene glacial periods. The genetic diversity
of the Yamato Bank subpopulation of B. tsubai was lower than that of the other subpopulations, which is likely attributable to the small size of the Yamato Bank subpopulation. 相似文献
68.
69.
Raknuzzaman Mohammad Ahmed Md Kawser Islam Md Saiful Habibullah-Al-Mamun Md Tokumura Masahiro Sekine Makoto Masunaga Shigeki 《Environmental science and pollution research international》2016,23(17):17298-17310
Environmental Science and Pollution Research - Trace metals contamination in commercial fish and crustaceans have become a great problem in Bangladesh. This study was conducted to determine seven... 相似文献
70.
Umme Salma Zohora Mohammad Shahedur Rahman Abdul Wahab Khan Masahiro Okanami Takashi Ano 《环境科学学报(英文版)》2013
To enhance the production of lipopeptide antibiotic iturin A, nutrient contents of the culture mediums were investigated in both submerged and biofilm fermentations. As a carbon source maltose and as nitrogen source, fish protein was used. In submerged fermentation maltose uptake was found lower (12%) compared to biofilm fermentation (15%) that was associated with higher cellular growth in biofilm. However, requirement of nitrogen (fish protein) concentration was found similar in both submerged and biofilm fermentations. Production of iturin A in submerged fermentation with 12% maltose and 5% fish protein was 4450 mg/L, and in biofilm fermentation it was 5050 mg/L when 15% maltose and 5% fish protein was used. 相似文献