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81.
Distribution of perfluorochemicals between sera and milk from the same mothers and implications for prenatal and postnatal exposures 总被引:1,自引:0,他引:1
Kim SK Lee KT Kang CS Tao L Kannan K Kim KR Kim CK Lee JS Park PS Yoo YW Ha JY Shin YS Lee JH 《Environmental pollution (Barking, Essex : 1987)》2011,159(1):169-174
The levels of six perfluorocarboxylates (PFCAs), four perfloroalkylsulfonates (PFASs), and one sulfonamide were measured in paired samples of maternal serum, umbilical cord serum, and breast milk. The maternal and cord sera were strongly correlated with each other for all measured compounds (r > 0.5 and p < 0.01). Nevertheless, there was a significant difference in compound composition profile between the two sera matrices, with a more depletion of the longer chain compounds in cord serum. The transfer efficiency values from maternal to cord serum (TFCS/MS) decreased by 70% with each increasing unit of -CF2 chain within a PFCA group, and for perfluorooctanesulfonate (PFOS), by a half compared to perfluorooctanoate (PFOA). In contrast to the strong correlation in concentrations between the two sera matrices, the pattern of compounds in breast milk differed considerably with those in sera. Accordingly, compound- and matrix-specific transfer must be considered when assessing prenatal and postnatal exposure. 相似文献
82.
Yoo Jung Kim Jung-Hun Woo Young-Il Ma Suhyang Kim Jung Sik Nam Hakyoung Sung Ki-Chul Choi Jihyun Seo Jeong Su Kim Chang-Hee Kang Gangwoong Lee Chul-Un Ro Duk Chang Young Sunwoo 《Atmospheric environment (Oxford, England : 1994)》2009,43(34):5556-5566
In this study, background concentration sites of Deokjeok and Gosan, which were deemed suitable for monitoring the impact of long-range transported air pollutants, were selected. An investigation of the source types of pollutants, their locations, and relative quantitative contributions to the particulate concentrations at both sites using appropriate methodologies to make initial estimations was conducted. Episodic measurements of PM2.5, PM10, and size distribution, along with its ion and carbon components were performed from 2005 to 2007, and a comprehensive analysis of the results was conducted utilizing back trajectory analysis. As for frequency of wind direction, it was quite apparent that the two sites are heavily influenced by air masses originating from the eastern and northern regions of China. For PM2.5 and PM10, the mass concentrations from north and east China were higher than other cases, originating from the ocean. In the northerly-wind case, meteorological properties for Deokjeok and Gosan and the influence of carbon emissions from northwest Korea resulted in a changing of air mass properties during transport. As was the case with mass concentration, the highest contribution for ionic and carbon components of PM2.5 and PM10 for both sites appeared for the westerly wind case. A specially high relative contribution, greater than 1.4 times, was apparent in the secondary aerosol case because of a large influence of long-range transported pollutants from east China. Carbon components exhibited different behaviors for the northerly and westerly wind cases compared with secondary aerosol. The major reason for this discrepancy appears to be the carbon emissions from northwest Korea. 相似文献
83.
Tae-Wan Jeon Jong-Eun Park Sun-Kyoung Shin Jin-Soo Park Mi-Jeong Jeong 《Journal of Material Cycles and Waste Management》2016,18(2):329-339
In the present study, new congeners were selected for the efficient management of PCB containing waste and PCB contaminated waste, and the applicability of these new indicators was confirmed. As a result, 8 indicator congeners and 4 index peaks which were named “Proposed new method 1” and “Proposed new method 2” were selected. For the assessment of a novel quantitative method, comparative tests using conventional methods were conducted, and the factors for total PCB were calculated for each method. Results from these tests showed that the average values for the factors of CEN/TC19/WG22, DIN 51527, and the test method by the disposal regulation for ocean dumping in Korea were 1.86, 3.47, and 2.52, respectively, while those for the proposed new method 1 and proposed new method 2 were 2.98 and 5.56, respectively. For PCB contaminated waste, the factor was found to be 1.99, 3.42, and 3.02 using the conventional methods, 2.67 using the proposed new method 1, and 5.57 using the proposed new method 2. It is expected that, in accordance with the results of the present study, the management of PCB waste can be integrated, regardless of the type of waste involved. 相似文献
84.
Simultaneous Measurements of Atmospheric Pollutants and Visibility with a Long-Path DOAS System in Urban Areas 总被引:4,自引:0,他引:4
In this paper, the applicability of a Long-Path Differential Optical Absorption Spectroscopy (LP-DOAS) system was checked for the feasibility of the simultaneous measurement of trace gases (such as O3, NO2, SO2, and HCHO) and atmospheric visibility (light extinction by aerosols) in Asian urban areas. Field studies show that an LP-DOAS system can simultaneously measure the key pollutants (such as O3, NO2, SO2, and HCHO) at detection limits in the ppb/sub-ppb range as well as the Mie extinction coefficient with an uncertainty of 0.1 km–1 at time resolution of a few minutes. It is thus concluded that the use of LP-DOAS system is feasible for simultaneous measurement of gaseous pollutants as well as an atmospheric extinction coefficient which is tightly bound to fine particulate concentration. 相似文献
85.
The Triad Approach was field‐tested to determine if characterization objectives could be met for a brownfields property that had been identified as a future elementary school site. The new school is in response to a New Jersey Supreme Court ruling (the Abbott decision) that directed the state of New Jersey to fund school construction in poorer districts to expand physical facilities to relieve overcrowding. The Triad Approach is promoted by the United States Environmental Protection Agency as a process that has the potential to improve the timeliness and efficiency of site characterization, and the New Jersey Department of Environmental Protection (NJDEP) recently issued a policy statement supporting its potential. Aggressive school construction deadlines are contingent on property acquisitions that are relatively faster than the traditional investigatory process. In addition, given the future sensitive population, the investigations must be thorough. This case study is among the first studies to document the use of the Triad Approach for a future school site. The Triad Approach was used to define site conditions for six areas of concern in a two‐month time frame (from the start of the planning process to completed investigation). © 2004 Wiley Periodicals, Inc. 相似文献
86.
Indoor air quality (IAQ) directly affects the health of occupants. Household manufacturing equipment (HME) used for hobbies or educational purposes is a new and unexplored source of air pollution. In this study, we evaluated the characteristics of particulate and gaseous pollutants produced by a household laser processing equipment (HLPE). Various target materials were tested using a commercial HLPE under various operating conditions of laser power and sheath air flow rate. The mode diameters of the emitted particles gradually decreased as laser power increased, while the particle number concentration (PNC) and particle emission rate (PER) increased. In addition, as the sheath air flow rate quadrupled from 10 to 40 L/min, the mode diameter of the emitted particles decreased by nearly 25%, but the effect on the PNC was insignificant. When the laser induced the target materials at 53 mW, the mode diameters of particles were <150 nm, and PNCs were >2.0 × 104 particles/cm3. Particularly, analyses of sampled aerosols indicated that harmful substances such as sulfur and barium were present in particles emitted from leather. The carcinogenic gaseous pollutants such as acrylonitrile, acetaldehyde, 1,3-butadiene, benzene, and C8 aromatics (ethylbenzene) were emitted from all target materials. In an actual indoor environment, the PNC of inhalable ultrafine particles (UFPs) was >5 × 104 particles/cm3 during 30 min of HLPE operation. Our results suggest that more meticulous control methods are needed, including the use of less harmful target materials along with filters or adsorbents that prevent emission of pollutants. 相似文献
87.
Hong Guo Kwanho Jeong Jiyeon Lim Jeongwon Jo Young Mo Kim Jong-pyo Park Joon Ha Kim Kyung Hwa Cho 《环境科学学报(英文版)》2015
Of growing amount of food waste, the integrated food waste and waste water treatment was regarded as one of the efficient modeling method. However, the load of food waste to the conventional waste treatment process might lead to the high concentration of total nitrogen (T-N) impact on the effluent water quality. The objective of this study is to establish two machine learning models—artificial neural networks (ANNs) and support vector machines (SVMs), in order to predict 1-day interval T-N concentration of effluent from a wastewater treatment plant in Ulsan, Korea. Daily water quality data and meteorological data were used and the performance of both models was evaluated in terms of the coefficient of determination (R2), Nash–Sutcliff efficiency (NSE), relative efficiency criteria (drel). Additionally, Latin-Hypercube one-factor-at-a-time (LH-OAT) and a pattern search algorithm were applied to sensitivity analysis and model parameter optimization, respectively. Results showed that both models could be effectively applied to the 1-day interval prediction of T-N concentration of effluent. SVM model showed a higher prediction accuracy in the training stage and similar result in the validation stage. However, the sensitivity analysis demonstrated that the ANN model was a superior model for 1-day interval T-N concentration prediction in terms of the cause-and-effect relationship between T-N concentration and modeling input values to integrated food waste and waste water treatment. This study suggested the efficient and robust nonlinear time-series modeling method for an early prediction of the water quality of integrated food waste and waste water treatment process. 相似文献
88.
89.
Jeong CH Evans GJ Hopke PK Chalupa D Utell MJ 《Journal of the Air & Waste Management Association (1995)》2006,56(4):431-443
Continuous measurements of particle number concentrations were performed in Rochester, NY, and Toronto, Ontario, Canada during the 2003 calendar year. Strong seasonal dependency in particle number concentration was observed at two sites. The average number concentration of ambient particles was 9670 +/- 6960 cm(-3) in Rochester, whereas in Toronto the average number of particles was 28,010 +/- 13,350 cm(-3). The particle number concentrations were higher in winter months than in summer months by a factor of 1.5 in Rochester and 1.6 in Toronto. In general, there were also distinct diurnal variations of aerosol number concentration. The highest weekdays/weekends ratio of number concentration was typically observed during the rush-hour period in winter months with a ratio of 2.1 in Rochester and 2.0 in Toronto. The correlation in the total particle number concentrations between the two urban sites was stronger in winter because of the common urban traffic patterns, but weaker in summer because of local sulfur dioxide (SO2)-related particle formation events in Rochester in the summer. Strong morning particle formation events were frequently observed during colder winter months. Good correlations between particle number and carbon monoxide (CO) as well as temperature suggested that motorvehicle emissions lead to the formation of new particles as the exhaust mixes with the cold air. Regional nucleation and growth events frequently occurred in April. Local SO2-related particle formation events most frequently occurred in August. SO2 and UV-B were highly correlated with particle concentration, suggesting a high association of photochemical processes with these local events. A high directionality in a northerly direction was observed for particle number and SO2, indicating the influence of point sources located north of Rochester. 相似文献
90.
This work proposes a new potential application of waste coal fly ash as a K fertilizer support. Fly ash was reacted with KOH to facilitate the impregnation of K as well as to enhance the bonding force. In particular, the applied process resulted in a significant slow-releasing characteristic of fertilizer elements. To examine the effect of K impregnation, a few detailed leaching tests were carried out in terms of process variables such as reaction time and temperature, sintering time and temperature, and KOH concentration. The current experiment presented an optimum preparation condition that is competitive with conventional commercial fertilizers. The manufactured ash fertilizers inhibited release of the K elements. It was also found through the continuous leaching test with pure water that the ash fertilizer had excellent moisture absorbability. However, the effects of some trace elements in fly ash on soil health and crop productivity as well as environmental considerations need to be established with long-term studies. 相似文献