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161.
Manzetti Sergio Hadi Behzadi Andersen Otto David van der Spoel 《Environmental Chemistry Letters》2013,11(2):105-118
Nanotechnology globally represents a new direction within scientific development, where the atomic and electronic properties of molecules are used in a unique fashion to produce and construct new and exotic materials and products. Fullerenes (Bucky balls, C60) constitute a particular group within the field of nanotechnology. Fullerenes find applications in medicine, industrial chemistry and electronics. However, there are several unanswered questions about fullerenes and their toxicological properties. Most toxicological studies on fullerenes evolve around the in vitro and in vivo aspects of pristine C60 along with chemically modified C60 molecules. We reviewed toxicology reports on C60. We bring a critical and challenging evaluation of the electronic and quantum properties of C60 molecules in context with the implications on cellular factors and metabolites. The evaluation shows that the reactivity and quantum chemical properties of C60 can have unexpected effects in the cell, by principally absorbing metabolites, such as OH? and H+ ions and alter its reactivity. We thus challenge the present view of C60 solely based on empirical studies, based on the electronic properties of C60 that vary considerably with their size and reaction path. A further example of this is the absorption of divalent zinc ions, which shows an increase in reactivity of the C60 that presents an important pattern of chemical state, reactivity and toxicological potential. The results evaluate the toxicological potential of C60 from a different angle than conventional, by applying a blend of critical review of the findings on C60 toxicity, their chemical and electronic properties. 相似文献
162.
S. Otto W. Keller N. Drescher 《Journal of environmental science and health. Part. B》2013,48(3):179-191
Abstract A new gas chromatographic method reliable in the microgram range, was developed to measure ETU residues in various crops. Contrary to previously published procedures, this new method does not require prior derivatization of the ETU. The limit of sensitivity was shown to be 0.01 ppm using the flame photometric detector, FPD (sulfur mode, 394 nm). 相似文献
163.
Narayan Dhital Frédéric Raulier Pierre Y. Bernier Marie-Pierre Lapointe-Garant Frank Berninger Yves Bergeron 《Journal of Environmental Planning and Management》2015,58(12):2228-2249
Ecosystem-based management (EBM) of forests is gaining acceptance for its focus on the maintenance of the long-term integrity of ecosystem processes, but climate change challenges this view because of its impacts on these very processes. We have therefore evaluated the robustness of EBM to projected climate change, considering the role of climate on forest growth and fire regime in a boreal forest of eastern Canada. A climate sensitive growth index model was calibrated for three commercial species and used to project the evolution of merchantable volume for two climate scenarios (B1 and A2) under conventional and EBM strategies. Current burn rate and burn rates under future climate scenarios were also considered. Under the most extreme projected climate scenario, the periodic timber supply could be reduced by up to 79% through direct (growth reduction) and indirect (fire) effects. However, ecological indicators show that EBM is a more robust forest management strategy than conventional one demonstrating its adaptation potential to climate change at least in the short term. 相似文献
164.
Gerald Fischer Tina Frohne Lydia Gerharz Margit Hildebrandt Otto Klemm Katrin Mildenberger Carsten Nording Ingo Rehberger Manuel Schiffer Christos Stephan Voulkoudis 《Environmental Sciences Europe》2006,18(3):155-163
Objective and Background
The nitrogen oxides NO and NO2 and, in particular, their ratio (NO/NO2), play important roles in the radical-system of the atmospheric boundary layer. There were various indications upon a dropping NO/NO2-ratio in citiex over the last years, however, no proof has been given yet Especially in densely populated areas such as the federal state of North Rhine-Westphalia (NRW), such a change can have significant influences upon various atmospheric reactions. The objective of this investigation was to prove the existence of a systematic change of the NO/NO2-ratio, to describe the development of NOx over the past 2 decades at different locations and to determine the causes for this development.Methods
To detect changes of the NO/NO2-ratio we processed the data of 11 continuously operating air quality stations of the State Environment Agency (LUA NRW) with time series reaching back up to 20 years. We investigated rural stations, stations in the urban background and heavily traffic influenced locations. It was possible to calculate and assess the NO/NO2-ratio under consideration of the fast reaction of ozone with NO. There were clear indications towards existing trends and they could be determined as statistically significant using the nonparametric Mann-Kendall Test. The analysis of possible causes for the change of the NO/NO2-ratio focused upon the change of the global radiation, the change of the patterns of the atmosphetic circulation, and the frequency of cyclones and anticyclones meteorological conditions in Central Europe, the introduction of automotive catalytic converters, and the development of the atmospheric oxidation-capacity.Results and conclusions
The results are indicating a decline of the ratio at traffic-influenced stations with a statistical significance over 95%. The negative trend can also be detected at most urban background stations. It was problematic to perform the trend-analysis of the rural background station in the Egge-Mountains because of the fragmentary character of the dataset. Regional differences in the development of the NO/NO2-ratio indicate towards various causes. Crucial for the situation at the rural areas are the changed trajectories of cyclones and anticyclones as well as the decline of the atmospheric oxidation-capacity, while the traffic plays another important role at urban stations. The negative trend at the traffic-stations was intensified by the introduction of catalytic converters, which lead to a reduction in emissions of NOxRecommendations and prospects
The significance of the NO/NO2-ratio for the oxidation capacity of the atmosphere shows the necessity to further monitor this development. Previous investigations detected a decline in total NOx without examining the relative development of the two nitrogen oxides towards each other. Gaining insight into the local differences of this ratio helps to allocate sources and to develop understanding of the atmospheric processes. 相似文献165.
Otto J. Helweg John W. Labadie 《Journal of the American Water Resources Association》1976,12(4):681-694
ABSTRACT This paper briefly reviews the problem of ground water degradation from irrigation and present approaches to controlling ground water quality. As an alternative to these approaches, a management scheme called the Accelerated Salt TRANsport (ASTRAN) method is proposed as being a feasible solution to the problem of salt build-up in irrigated areas. A management algorithm for implementing the ASTRAN method is described. Results from modeling studies indicate that the ASTRAN method is cost-effective and encourages conjunctive use of ground water and surface water. 相似文献
166.
M. Hossein Sabet Otto J. Helweg 《Journal of the American Water Resources Association》1989,25(5):1047-1053
ABSTRACT: Construction of a “peaking storage tank” may reduce the operational cost of municipal water in the availability of a time-of-use energy rate. A peaking storage tank is used for storing water that is pumped from wells or other sources of supply during off-peak periods when energy costs are less for use during periods of on-peak water demand. The optimal size of a peaking storage tank is that which results in the minimum total cost, which includes both the storage construction cost and the cost of operation of the pumps. The operational cost for a given time-of-use rate is determined by help of a pipe network simulation model solved by the Newton-Raphson technique and a dynamic programming optimization model. A more simplified method is also introduced. Analyses show that low off-peak energy costs make the construction of peaking storage tanks economically attractive and reduce on-peak energy use, which results in electrical load leveling. 相似文献
167.
An isolated root uptake test (IRUT) was used to characterize the bioaccumulation of 14C-naphthol in excised root segments obtained from 6-month-old hydroponically grown plants: two varieties of fescue (Festuca arundinaceae Schreb.) and one variety of clover (Trifolium pratense L.). Naphthol uptake rates were directly related to naphthol concentration in the range 0.01 to 0.2 uM. The incubation time required for equilibrium to be reached between naphthol in root tissue and in solution was between 9 and 12 h. Tests using metabolic inhibitors, KCN, NaN3, and DNP, indicated that naphthol uptake may be the result of both passive and active mechanisms. Q10 values for naphthol uptake ranged from 1.05 to 1.16. 相似文献
168.
Christian C. Voigt Otto von Helversen Robert Michener Thomas H. Kunz 《Behavioral ecology and sociobiology》2001,50(1):31-36
Saccopteryx bilineata has a polygynous mating system in which males defend females in a harem territory. Harem defense and courtship include energetically costly flight maneuvers and hovering displays. We tested if (1) harem males have a greater field metabolic rate than non-harem males or females and if (2) the field metabolic rate of harem males is correlated with the number of females in a harem territory. We measured the energy budget in 32 S. bilineata with the doubly labeled water method and compared these estimates with behavioral observations in the daytime roost. Among adult bats, field metabolic rate varied with body mass by an exponent of approximately two. We found no significant difference in field metabolic rate or mass-specific field metabolic rate between harem and non-harem males. The mass-specific field metabolic rate of harem-males increased with harem size. The latter finding supports the hypothesis that the energy costs of courtship display and territorial defense influence the energy budget of harem males. Overall, field metabolic rates of S. bilineata were lower than those of similarly sized bats of the temperate zone and only 2.3 times above the basal metabolic rate recorded for this species. We suggest that male S. bilineata did not take advantage of their metabolic capacity because a prudent allocation of energy to activities of harem maintenance is an adaptive strategy for males in this mating system. 相似文献
169.
Otto Hänninen Stefano Zauli-Sajani Roberta De Maria Paolo Lauriola Matti Jantunen 《Environmental Modeling and Assessment》2009,14(4):419-429
Particulate matter air pollution is estimated to cause in the order of 350,000 excess deaths in the European Union calling for policy development and evaluation tools. In the current work, a model for PM10 exposures of children is developed using microenvironment time activities and infiltration of ambient pollution indoors, both evaluated against observations earlier and integrated with city-wide air quality models in the current work. The model is demonstrated using data from two cities in Italy. High-end short-term exposures are characterized by an episode-day situation in Turin, and annual mean exposures in downtown Bologna. The air quality model was unable to capture the highest levels during the episode, and therefore, the exposure model was adjusted using observed–modeled ratio from a monitoring station. Air quality model performance for the annual levels was significantly better. Annual exposure variability within the target population was 1.5-fold in the downtown area Bologna and tenfold during the episode day in Turin. 相似文献
170.
Klemm O Schemenauer RS Lummerich A Cereceda P Marzol V Corell D van Heerden J Reinhard D Gherezghiher T Olivier J Osses P Sarsour J Frost E Estrela MJ Valiente JA Fessehaye GM 《Ambio》2012,41(3):221-234
The collection of fog water is a simple and sustainable technology to obtain fresh water for afforestation, gardening, and as a drinking water source for human and animal consumption. In regions where fresh water is sparse and fog frequently occurs, it is feasible to set up a passive mesh system for fog water collection. The mesh is directly exposed to the atmosphere, and the foggy air is pushed through the mesh by the wind. Fog droplets are deposited on the mesh, combine to form larger droplets, and run down passing into a storage tank. Fog water collection rates vary dramatically from site to site but yearly averages from 3 to 10 l m−2 of mesh per day are typical of operational projects. The scope of this article is to review fog collection projects worldwide, to analyze factors of success, and to evaluate the prospects of this technology. 相似文献