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91.
Phosphates for Pb immobilization in soils: a review 总被引:9,自引:0,他引:9
In its soluble ionic forms, lead (Pb) is a toxic element occurring in waters and soils mainly as the result of human activities.
The bioavailability of lead ions can be decreased by complexation with various materials in order to decrease their toxicity.
Pb chemical immobilization using phosphate addition is a widely accepted technique to immobilize Pb from aqueous solution
and contaminated soils. The application of different P amendments cause Pb in soils to shift from forms with high availability
to the most strongly bound Pb fractions. The increase of Pb in the residual or insoluble fraction results from formation of
pyromorphite Pb5(PO4)3X where X = F, Cl, Br, OH, the most stable environmental Pb compounds under a wide range of pH and Eh natural conditions.
Accidental pyromorphite ingestion does not yield bioavailable lead, because pyromorphite is insoluble in the intestinal tract.
Numerous natural and synthetic phosphates materials have been used to immobilize Pb: apatite and hydroxyapatite, biological
apatite, rock phosphate, soluble phosphate fertilizers such as monoammonium phosphate, diammonium phosphate, phosphoric acid,
biosolids rich in P, phosphatic clay and mixtures. The identification of pyromorphite in phosphate amended soils has been
carried out by different non destructive techniques such as X-ray diffraction, scanning electron microscopy coupled with energy
dispersive X-ray spectroscopy, X-ray absorption fine structure, transmission electron microscopy and electron microprobe analysis.
The effectiveness of in situ Pb immobilization has also been evaluated by selective sequential extraction, by the toxicity
leaching procedure and by a physiologically based extraction procedure simulating metal ingestion and gastrointestinal bioavailability
to humans. Efficient Pb immobilization using P amendments requires increasing the solubility of the phosphate phase and of
the Pb species phase by inducing acid conditions. Although phosphorus addition seems to be highly effective, excess P in soil
and its potential effect on eutrophication of surface water, and the possibility of As enhanced leaching remains a concern.
The use of mixed treatments may be a useful strategy to improve their effectiveness in reducing lead phyto- and bioavailability. 相似文献
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Christian Mougin Agnès Bouchez Laurence Denaix Isabelle Lamy François Laurent Fabrice Martin-Laurent Michel Mench 《Environmental science and pollution research international》2016,23(4):2974-2976
The fifth meeting of INRA’s national network of ecotoxicologists took place on 25 to 27 November 2014 in Biarritz, France. The main aim of the meeting was to bring together ecotoxicologists from INRA and associated partners, providing them ample opportunity to share and discuss their latest scientific results as well as the national policy of research in ecotoxicology and to precise perspectives for the network. 相似文献
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This study examines the relationship between national-level militarism and consumption-based carbon dioxide emissions. We analyze panel data from 1990 to 2010 for 81 nations to determine whether the magnitude of the effects of (1) military expenditures as percent of total gross domestic product and (2) military personnel as percent of total labor force on carbon emissions change over time. Results of two-way fixed effects models highlight the temporal stability of the environmental impacts of both national-level military characteristics. The findings also reveal that the effect of military expenditures on emissions is larger in the more developed OECD nations than in the developing non-OECD nations. Overall, the results support the treadmill of destruction perspective, which suggests that the nations’ militaries are an important social institution to consider in sustainability science research on the human drivers of global environmental change. 相似文献
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Fethi Amri 《Environmental science and pollution research international》2017,24(17):14567-14578
This study examines the relation between CO2 emissions, income, non-renewable, and renewable energy consumption in Algeria during the period extending from 1980 to 2011. Our work gives particular attention to the validity of environmental Kuznets curve (EKC) hypothesis. The autoregressive distributed lag (ARDL) with break point method outcome demonstrates the positive effect of non-renewable type of energy on CO2 emissions consumption. On the contrary, the results reveal an insignificant effect of renewable energy on environment improvement. Moreover, the results accept the existence of EKC hypothesis but the highest gross domestic product value in logarithm scale of our data is inferior to the estimated turning point. Consequently, policy-makers in Algeria should expand the ratio of renewable energy and should decrease the quota of non-renewable energy consumption. 相似文献
99.
Xu Li Zimeng Liu Qing Xu Zhongyi Jiang Guoliang Ma 《Environmental Modeling and Assessment》2017,22(3):243-255
In this paper, we construct a multi-stage coordinated programming model under tax system to control SO2 emission. The model is based on an explicitly formulated SO2 abatement cost function created under Chinese condition. Analysis of the effectiveness and impact on the economy of the model is carried out with consideration of game theory. By solving the model, theoretical results show that the volume-based multi-stage SO2 tax system has two properties: effectiveness and equal-rate. Based on these theoretical results, empirical study is also performed using Chinese historical data. Compared with yearly single-stage programming model, the tax rate generated by the coordinated multi-stage programming model is time-invariant and rather moderate in scale. The total abatement cost among planning years in our model is 21.03 % less than the actual number and 6.68 % less than that in the single-stage situation. The tax payment suggested by our model is 10.62 % less than by the single-stage model. In general, a coordinated multi-stage programming model helps reduce the overall costs of environmental protection while achieving the same emission control target with less burden added to the economy. 相似文献
100.
Metrics of water scarcity and stress have evolved over the last three decades from simple threshold indicators to holistic measures characterising human environments and freshwater sustainability. Metrics commonly estimate renewable freshwater resources using mean annual river runoff, which masks hydrological variability, and quantify subjectively socio-economic conditions characterising adaptive capacity. There is a marked absence of research evaluating whether these metrics of water scarcity are meaningful. We argue that measurement of water scarcity (1) be redefined physically in terms of the freshwater storage required to address imbalances in intra- and inter-annual fluxes of freshwater supply and demand; (2) abandons subjective quantifications of human environments and (3) be used to inform participatory decision-making processes that explore a wide range of options for addressing freshwater storage requirements beyond dams that include use of renewable groundwater, soil water and trading in virtual water. Further, we outline a conceptual framework redefining water scarcity in terms of freshwater storage. 相似文献