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701.
Removal of tetracycline from water by Fe-Mn binary oxide 总被引:2,自引:0,他引:2
Significant concerns have been raised over the presence of antibiotics including tetracyclines in aquatic environments. A series of Fe-Mn binary oxide with different Fe:Mn molar ratios was synthesized by a simultaneous oxidation and coprecipitation process for TC removal. Results showed that Fe-Mn binary oxide had higher removal efficiency than that of hydrous iron oxide and hydrous manganese oxide, and that the oxide with a Fe:Mn molar ratio of 5:1 was the best in removal than other molar ratios. The tetracycline removal was highly pH dependent. The removal of tetracycline decreased with the increase of initial concentration, but the absolute removal quantity was more at high concentration. The presence of cations and anions such as Ca2+, Mg2+, CO32- and SO42- had no significant effect on the tetracycline removal in our experimental conditions, while SiO32- and PO43- had hindered the adsorption of tetracycline. The mechanism investigation found that tetracycline removal was mainly achieved by the replacement of surface hydroxyl groups by the tetracycline species and formation of surface complexes at the water/oxide interface. This primary study suggests that Fe-Mn binary oxide with a proper Fe:Mn molar ratio will be a very promising material for the removal of tetracycline from aqueous solutions. 相似文献
702.
703.
坡度分析在昆明盆地断层分段中的应用 总被引:1,自引:0,他引:1
地面坡度是反映地形地貌变化的关键因子,应用坡度分析一定程度上可以反映断层的展布特征。本文收集整理昆明市区附近千余份钻孔数据,筛选其中238个钻孔进行钻孔层序分层和数据库的建设,使用ArcScene软件生成研究区地表、海埂组(QhH)底部以及官渡组(Qp3G)底部地层面的三维地质模型。应用ArcGIS软件中坡度分析模块,获得各个界面的坡度图,从坡度变化特征方面对研究区5条主要断层的活动性与分段特征进行了初步探讨。 相似文献
704.
西南部地区干旱突显出我国水资源的供求矛盾。中水回用可以提高水资源的使用效率、缓解水资源匮乏的问题,但从全国看,推行的阻力很大。建议通过立法,强制推行中水回用政策,以实现水资源的可持续利用和社会经济的可持续发展。 相似文献
705.
Xixi Wang Shiyou Shang Zhongyi Qu Tingxi Liu Assefa M. Melesse Wanhong Yang 《Journal of environmental management》2010,91(7):1511-1525
Wetlands are one of the most important watershed microtopographic features that affect hydrologic processes (e.g., routing) and the fate and transport of constituents (e.g., sediment and nutrients). Efforts to conserve existing wetlands and/or to restore lost wetlands require that watershed-level effects of wetlands on water quantity and water quality be quantified. Because monitoring approaches are usually cost or logistics prohibitive at watershed scale, distributed watershed models such as the Soil and Water Assessment Tool (SWAT), enhanced by the hydrologic equivalent wetland (HEW) concept developed by Wang [Wang, X., Yang, W., Melesse, A.M., 2008. Using hydrologic equivalent wetland concept within SWAT to estimate streamflow in watersheds with numerous wetlands. Trans. ASABE 51 (1), 55–72.], can be a best resort. However, there is a serious lack of information about simulated effects using this kind of integrated modeling approach. The objective of this study was to use the HEW concept in SWAT to assess effects of wetland restoration within the Broughton's Creek watershed located in southwestern Manitoba, and of wetland conservation within the upper portion of the Otter Tail River watershed located in northwestern Minnesota. The results indicated that the HEW concept allows the nonlinear functional relations between watershed processes and wetland characteristics (e.g., size and morphology) to be accurately represented in the models. The loss of the first 10–20% of the wetlands in the Minnesota study area would drastically increase the peak discharge and loadings of sediment, total phosphorus (TP), and total nitrogen (TN). On the other hand, the justifiable reductions of the peak discharge and loadings of sediment, TP, and TN in the Manitoba study area may require that 50–80% of the lost wetlands be restored. Further, the comparison between the predicted restoration and conservation effects revealed that wetland conservation seems to deserve a higher priority while both wetland conservation and restoration may be equally important. 相似文献
706.
Xiao-yan Qu Zhen-shan Li Xin-yuan Xie Yu-mei Sui Lei Yang You Chen 《Waste management (New York, N.Y.)》2009,29(10):2618-2624
It is recognized that information on both quantity and composition of residential waste is important for the effective planning of household waste handling infrastructure. In this paper, we present the results of a survey on household waste generation and composition in Beijing, China. Sample communities were selected by the integration of five indices including family population, income, age, and education. Wastes were sampled on a daily basis from 113 households in six different districts of Beijing City for ten days. The results showed that the generation rate of household wastes was 0.23 kg/pers/day. The bulk density was approximately 221 kg/m3, and the moisture content was approximately 50%. Household waste consisted of kitchen waste, paper/cardboard, plastics, textiles, metals, glass and other wastes, the proportion of each waste was approximately 69.3%, 10.3%, 9.8%, 1.3%, 0.8%, 0.6% and 2.7%, respectively. An evaluation of the relationship between daily per capita generation of household waste and socio-economic factors indicated that household size and income both showed a negative relationship with household waste generation (kg/pers/day). As for the effect of education, families with a secondary educational level produced fewer household wastes (kg/pers/day) than those with a primary or advanced educational level. 相似文献
707.
Wenjun Huang Haomiao Xu Xiaoshuang Liu Longlong Wang Shutang Li Leipeng Ji Zan Qu Naiqiang Yan 《环境科学学报(英文版)》2022,34(5):1-9
Fe3O4-based materials are widely used for magnetic separation from wastewater. However, they often suffer from Fe-leaching behavior under acidic conditions, decreasing their activity and limiting sustainable practical applications. In this study, covalent organic frameworks (COFs) were used as the shell to protect the Fe3O4 core, and the Fe3O4@COF core-shell composites were synthesized for As(III) removal from acid wastewater. The imine-linked COFs can in situ grow on the surface of the Fe3O4 core layer by layer with [COFs/Fe3O4]mol ratio of up to 2:1. The Fe-leaching behavior was weakened over a wide pH range of 1-13. Moreover, such composites keep their magnetic characteristic, making them favorable for nanomaterial separation. As(III) batch adsorption experiments results indicated that, when COFs are used as the shell for the Fe3O4 core, a balance between As(III) removal efficiencies and the thickness of the COF shell exists. Higher As(III) removal efficiencies are obtained when the [COFs/Fe3O4]mol ratios were < 1.5:1, but thicker COF shells were not beneficial for As(III) removal. Such composites also exhibited better As(III) removal performances in the pH range of 1–7. Over a wide pH range, the zeta potential of Fe3O4@COF core-shell composites becomes more positive, which benefits the capture of negative arsenic ions. In addition, thinner surface COFs were favorable for mass transfer and facilitating the reaction of Fe and As elements. Our study highlights the promise of using COFs in nanomaterial surface protection and achieving As(III) depth removal under acidic conditions. 相似文献
708.
709.
710.
Polybrominated diphenyl ethers in South China maternal and fetal blood and breast milk 总被引:19,自引:0,他引:19
Bi X Qu W Sheng G Zhang W Mai B Chen D Yu L Fu J 《Environmental pollution (Barking, Essex : 1987)》2006,144(3):1024-1030
Twenty-one-paired human fetal and maternal serum and 27 breast milk samples at South China were analyzed for concentrations of polybrominated diphenyl ethers (PBDEs). Seven PBDE congeners (BDE-28, -47, -99, -100, -153, -154, and -183) were quantified using gas chromatography/mass spectrometry (GC/MS). This is the first report to present the residue levels of PBDEs in human samples of China. The concentrations of total PBDEs ranged from 1.5 to 17 ng/g in the samples and were within the range reported in European samples for a similar population, but lower than human tissue levels in North America. BDE-47 and -153 were the dominant PBDE congeners in all samples and accounted for 60% of the total PBDEs. Further research is needed to determine the exposure route of PBDEs and their health effects. 相似文献