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311.
Verifying emission factors and national POPs emission inventories for the UK using measurements and modelling at two rural locations 总被引:2,自引:0,他引:2
Lohmann R Lee RG Abbott J Coleman P Jones KC 《Journal of environmental monitoring : JEM》2006,8(1):79-88
Different approaches are used to verify the adequacy of emission factors (EFs) and their use in emission inventories of persistent organic pollutants (POPs). The applicability of EFs was tested using atmospheric dispersion modelling to predict atmospheric concentrations of polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs), dibenzo-p-dioxins (PCDDs) and dibenzofurans (PCDFs) and resulting toxic equivalents (SigmaTEQ) and particulate matter <10 microm (PM(10)) in two rural locations in northern England (UK). The modelling was based on general assumptions of fuel composition, consumption and heating needs to simulate emissions of POPs from the domestic burning of coal and wood where ambient measurements were made in the winter of 1998. The model was used to derive the local contribution to ambient air concentrations, which were estimated independently based on comparative air measurements. The results support the hypothesis that in both villages, the majority of PAHs and the lower chlorinated PCDFs were locally released. The situation for PCBs and polychlorinated naphthalenes (PCNs) was different. While the EFs show the release of both compound groups from the domestic burning of coal and wood, the ambient levels of these "legacy POPs" in the villages were still clearly dominated by other sources. Rural areas relying mainly on fossil fuels can exceed the proposed UK ambient air quality standard for benzo[a]pyrene during winter. The measured EFs were then used to estimate the importance of the domestic burning of coal and wood to national emission inventories for these compound classes. Extrapolations to the UK suggest that the domestic burning of pure wood and coal were minor emitters for chlorinated POPs but contributed strongly to PAH and PM(10) levels in 2000. Finally, the UK's national POPs emission inventories based on source inventories and EF, as used here, were compared to estimates derived using the increase in atmospheric concentration of selected POPs. 相似文献
312.
Infrared spectrometry is a versatile basis to analyse greenhouse gases in the atmosphere. A multicomponent air pollution software (MAPS) was developed for retrieval of gas concentrations from radiation emission as well as absorption measurements. Concentrations of CO, CH4, N2O, and H2O as well as CO2, NO, NO2, NH3, SO2, HCl, HCHO, and the temperature of warm gases are determined on-line. The analyses of greenhouse gases in gaseous emission sources and in ambient air are performed by a mobile remote sensing system using the double-pendulum interferometer K300 of the Munich company Kayser-Threde. Passive radiation measurements are performed to retrieve CO, N2O, and H2O as well as CO2, NO, SO2, and HCl concentrations in smoke stack effluents of thermal power plants and municipal incinerators and CO and H2O as well as CO2 and NO in exhausts of aircraft engines. Open-path radiation measurements are used to determine greenhouse gas concentrations at different ambient air conditions and greenhouse gas emission rates of diffusive sources as garbage deposits, open coal mining, stock farming together with additional compounds (e.g. NH3), and from road traffic together with HCHO. Some results of measurements are shown. A future task is the verification of emission cadastres by these inspection measurements. 相似文献
313.
Karim C. Abbaspour Rainer Schulin Ernst Schläppi Hannes Flühler 《Environmental Modeling and Assessment》1996,1(3):151-158
A data worth model is presented for the analysis of alternative sampling schemes in a special project where decisions have to be made under uncertainty. This model is part of a comprehensive risk analysis algorthm with the acronym BUDA. The statistical framework in BUDA is Bayesian in nature and incorporates both parameter uncertainty and natural variability. In BUDA a project iterates among the analyst, the decision maker, and the field work. As part of the analysis, a data worth model calculates the value of a data campaign before the actual field work, thereby allowing the identification of an optimum data collection scheme. A goal function which depicts the objectives of a project is used to discriminate among different alternatives. A Latin hypercube sampling scheme is used to propagate parameter uncertainties to the goal function. In our example the uncertain parameters are the parameters which describe the geostatistical properties of saturated hydraulic conductivity in a Molasse environment. Our results indicated that failing to account for parameter uncertainty produces unrealistically optimistic results, while ignoring the spatial structure can lead to an inefficient use of the existing data. 相似文献
314.
The radiocarbon content in creosote bush in the greater Los Angeles area has been found to reflect the distribution of smog. Indications are that smog in the even larger air basin of the San Joaquin Valley of California may be caused in part by recent biospheric emissions rather than by fossil fuel combustion alone. 相似文献
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316.
Rainer Haas 《Environmental Sciences Europe》1999,11(4):247-247
317.
The assessment of environmental impacts along the life cycle of biofuels is a complex and resource-demanding task that cannot be afforded by small producers in developing countries. Therefore, certification schemes bear the risk that small and independent producers will be locked out and the market for sustainable biofuels will be dominated by international investors and large-scale plantations. However, many environmental impacts of various production chains of biofuels and feedstocks are already known. This knowledge has been used to create a web-based questionnaire for a “Sustainability Quick Check for Biofuels” (SQCB, http://www.sqcb.org). SQCB reduces the need for user entries to the most relevant and best-known parameters of the biofuel production chain. Based on this user input, a specific inventory is automatically modelled and linked to background data. SQCB then calculates the environmental impact assessment and checks the results against sustainability criteria. Since the results are calculated immediately, key environmental factors can be interactively analyzed. One major goal of the SQCB is to support the market entrance for local biofuel producers, given that strengthening local stakeholders is a key driver for empowering rural communities in development countries. 相似文献
318.
Mikko Hupa Rainer Backman Sture Boström 《Journal of the Air & Waste Management Association (1995)》2013,63(11):1496-1501
This article discusses nitrogen oxide emissions from various types of boilers in Finland. The boilers have been classified into 61 classes according to their size, combustion technique, and main fuel. A specific emission coefficient (ng NO2/J = mg NO2/MJ) for each class has been determined, based on literature surveys and actual measurements. The total NOX emission has been calculated for each class, using the emission coefficient and energy statistics. The effect of various techniques for emission reduction has also been investigated. The development of NOX emissions has been estimated for both the case where no preventing actions have been taken and for four defined cases where alternative reduction measures are assumed The total NOX emission from energy production in Finland was 107,000 tons NO2 in 1987. Seventy-five percent of this amount originated in boilers larger than 1 MWfuel effect (input effect), and the rest in smaller boilers and industrial processes. The most important boiler classes from the NOX emission’s point of view were coal-fired boilers, with an emission of approximately 38,000 tons NO2, peat-fired boilers and boilers fired with a mixture of fuels, emitting approximately 12,000 tons NO2 each. By 2005, the total NOX emission from energy production would increase 50 percent to approximately 160,000 tons if left uncontrolled. The emission level would be 140,000 tons if primary reduction techniques are applied, and 110,000 tons NO2, if catalytic NOX reduction devices are installed in boilers larger than 300 MW. 相似文献
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