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981.
Dan Golomb James A. Fay Subramanyam Kumar 《Journal of the Air & Waste Management Association (1995)》2013,63(7):798-802
The large differences in seasonal rates of wet sulfate deposition observed at many receptors in eastern North America imply that reducing SO2 emissions only in the summer half of the year (April-September) would bring about greater annual wet sulfate deposition reductions than reducing emissions by the same amount year-round. Targeting the emission reductions to those source areas which contribute the bulk of summer depositions in ecologically sensitive areas would increase further the gain factor, defined as the ratio of annual fractional deposition decrement to annual fractional emission decrement. In the northeastern U.S., between 10 and 15 rain episodes deposit about 60 percent of the annual wet sulfate; reducing emissions in the dry periods preceding these heavy deposition episodes could further increase the gain factor. However, it is difficult to predict these episodes, and they do not occur simultaneously over large regions of the country. 相似文献
982.
Robert Paine Olga Samani Mary Kaplan Eladio Knipping Naresh Kumar 《Journal of the Air & Waste Management Association (1995)》2013,63(11):1341-1353
The performance of the AERMOD air dispersion model under low wind speed conditions, especially for applications with only one level of meteorological data and no direct turbulence measurements or vertical temperature gradient observations, is the focus of this study. The analysis documented in this paper addresses evaluations for low wind conditions involving tall stack releases for which multiple years of concurrent emissions, meteorological data, and monitoring data are available. AERMOD was tested on two field-study databases involving several SO2 monitors and hourly emissions data that had sub-hourly meteorological data (e.g., 10-min averages) available using several technical options: default mode, with various low wind speed beta options, and using the available sub-hourly meteorological data. These field study databases included (1) Mercer County, a North Dakota database featuring five SO2 monitors within 10 km of the Dakota Gasification Company’s plant and the Antelope Valley Station power plant in an area of both flat and elevated terrain, and (2) a flat-terrain setting database with four SO2 monitors within 6 km of the Gibson Generating Station in southwest Indiana. Both sites featured regionally representative 10-m meteorological databases, with no significant terrain obstacles between the meteorological site and the emission sources. The low wind beta options show improvement in model performance helping to reduce some of the overprediction biases currently present in AERMOD when run with regulatory default options. The overall findings with the low wind speed testing on these tall stack field-study databases indicate that AERMOD low wind speed options have a minor effect for flat terrain locations, but can have a significant effect for elevated terrain locations. The performance of AERMOD using low wind speed options leads to improved consistency of meteorological conditions associated with the highest observed and predicted concentration events. The available sub-hourly modeling results using the Sub-Hourly AERMOD Run Procedure (SHARP) are relatively unbiased and show that this alternative approach should be seriously considered to address situations dominated by low-wind meander conditions.Implications: AERMOD was evaluated with two tall stack databases (in North Dakota and Indiana) in areas of both flat and elevated terrain. AERMOD cases included the regulatory default mode, low wind speed beta options, and use of the Sub-Hourly AERMOD Run Procedure (SHARP). The low wind beta options show improvement in model performance (especially in higher terrain areas), helping to reduce some of the overprediction biases currently present in regulatory default AERMOD. The SHARP results are relatively unbiased and show that this approach should be seriously considered to address situations dominated by low-wind meander conditions. 相似文献
983.
S. Behrooz Ghorishi Carl F. Singer Wojciech S. Jozewicz Charles B. Sedman Ravi K. Srivastava 《Journal of the Air & Waste Management Association (1995)》2013,63(3):273-278
Abstract Efforts to develop multipollutant control strategies have demonstrated that adding certain oxidants to different classes of Ca-based sorbents leads to a significant improvement in elemental Hg vapor (Hg0), SO2, and NOx removal from simulated flue gases. In the study presented here, two classes of Ca-based sorbents (hydrated limes and silicate compounds) were investigated. A number of oxidizing additives at different concentrations were used in the Ca-based sorbent production process. The Hg0, SO2, and NOx capture capacities of these oxidant-enriched sorbents were evaluated and compared to those of a commercially available activated carbon in bench-scale, fixed-bed, and fluid-bed systems. Calcium-based sorbents prepared with two oxidants, designated C and M, exhibited Hg0 sorp-tion capacities (~100 μg/g) comparable to that of the activated carbon; they showed far superior SO2 and NOx sorption capacities. Preliminary cost estimates for the process utilizing these novel sorbents indicate potential for substantial lowering of control costs, as compared with other processes currently used or considered for control of Hg0, SO2, and NOx emissions from coal-fired boilers. The implications of these findings toward development of multipollutant control technologies and planned pilot and field evaluations of more promising multipollutant sorbents are summarily discussed. 相似文献
984.
Chun W. Lee Ravi K. Srivastava S. Behrooz Ghorishi Jarek Karwowski Thomas W. Hastings Joseph C. Hirschi 《Journal of the Air & Waste Management Association (1995)》2013,63(5):643-649
Abstract A study was conducted to investigate the effect of selective catalytic reduction (SCR) catalyst on mercury (Hg) speciation in bituminous and subbituminous coal combustion flue gases. Three different Illinois Basin bituminous coals (from high to low sulfur [S] and chlorine [Cl]) and one Powder River Basin (PRB) subbituminous coal with very low S and very low Cl were tested in a pilot-scale combustor equipped with an SCR reactor for controlling nitrogen oxides (NOx) emissions. The SCR catalyst induced high oxidation of elemental Hg (Hg0), decreasing the percentage of Hg0 at the outlet of the SCR to values <12% for the three Illinois coal tests. The PRB coal test indicated a low oxidation of Hg0 by the SCR catalyst, with the percentage of Hg0 decreasing from ~96% at the inlet of the reactor to ~80% at the outlet. The low Cl content of the PRB coal and corresponding low level of available flue gas Cl species were believed to be responsible for low SCR Hg oxidation for this coal type. The test results indicated a strong effect of coal type on the extent of Hg oxidation. 相似文献
985.
Douglas H. Lowenthal Naresh Kumar 《Journal of the Air & Waste Management Association (1995)》2013,63(8):926-934
Abstract The Interagency Monitoring of Protected Visual Environments (IMPROVE) equation used to assess compliance under the U.S. Environmental Protection Agency (EPA) Haze Rule assumes that dry mass scattering efficiencies for aerosol chemical components are constant. However, examination of aerosol size distributions and chemical composition during the Big Bend Regional Aerosol and Visibility Observational Study and the Southeastern Aerosol and Visibility Study suggests that volume and mass scattering efficiencies vary directly with increasing particle light scattering and aerosol mass concentration. This is consistent with the observation that particle distributions were shifted to larger sizes under more polluted conditions and appears to be related to aging of the aerosol during transport to remote locations. 相似文献
986.
987.
Sharma KK Dubey JK Deka SC Chandrasekaran S Kalpana Gupta P Kumar A Vandana Devi MJ Singh B Baruah AA Kennedy JS Sharma ID Patyal SK Nath A 《Chemosphere》2007,68(4):790-796
Spiromesifen (Oberon) is a new insecticide and miticide of chemical class ketoenol active against white flies (Bemisia spp., Trialeuroides spp.) and spider mites (Tetranychus and Panonychus spp.). Due to its potential significance in insect resistance management, it is important to establish its behaviour on crop and environment. In the present study, the degradation/dissipation of spiromesifen on tea crop under tropical environmental conditions was studied and its DT(50) (t(1/2)), and DT(90) (time to reduce to 90% of the initial value) were estimated. Spiromesifen was sprayed on tea crop after first rain flush at four different locations @ 96 and 192ga.i.ha(-1). Samples of tea leaves were drawn at 0, 1, 3, 5, 7, 10, 15, 21 and 30 days after treatment and that of soil at 10 days after treatment and at harvest from 0 to 15 and 15 to 30cm layers. After crude extraction of tea leaves for spiromesifen residues with acetone:water, the contents were partitioned with cyclohexane:ethyl acetate and cleaned up on Florosil column. Soil residues were also extracted similarly. Quantification of residues was done on GC-MS in Selected Ion Monitoring (SIM) mode in mass range 271-274m/z. The LOQ of this method was found to be 0.05microgg(-1) while LOD being 0.015microgg(-1). The DT(50) of spiromesifen when applied at recommended doses in tea leaves was found to be 5.0-8.5 days. Ninety-nine percent degradation was found to occur within 33-57 days after application. In soil, no residues of spiromesifen were detectable 10 days after treatment. 相似文献
988.
Singh G Gupta SK Kumar R Sunderarajan M 《Environmental monitoring and assessment》2007,130(1-3):173-185
The present study describes the development of empirical models for the prediction of various trace metals i.e., Mn, Cu, Fe,
Zn and Pb found in the leachates generated from the ash ponds of various thermal power plants. The dispersion phenomenon of
these trace metals followed first order reaction rate kinetics. The empirical models for individual trace metals derived from
the lab scale models data correlate well with the real field data with regression coefficients varying from 0.93 to 0.98.
The predicted concentrations of the trace metals varied within ±3% of the observed values in the leachates generated from
the ash ponds of four thermal power plants with standard deviation varying from 0.001 to 0.032. The empirical models derived
from the study can be applied for prediction of trace metals in leachates generated from similar thermal power plants. 相似文献
989.
Sharma KK Rao CS Dubey JK Patyal SK Parihar NS Battu RS Sharma V Gupta P Kumar A Kalpana Jaya M Singh B Sharma ID Nath A Gour TB 《Environmental monitoring and assessment》2007,132(1-3):25-31
In a field study carried out at three different locations, the dissipation of spiromesifen on cotton and chili was studied
and its DT50, and DT99 were estimated at each location. Spiromesifen was sprayed on chili at 96 and 192 g a.i. ha−1 and cotton at 120 and 240 g a.i. ha−1. Samples of chili fruits were drawn at 0, 1, 3, 5, 7, 10, 15, 21, 30 days after treatment and that of cotton seed and lint
at first picking and harvest. Soil samples were drawn 30 days after treatment from 0 to 15 and 15 to 30 cm layer. Quantification
of residues was done on GC–MS in Selected Ion Monitoring (SIM) mode in mass range 271–274 m/z. The LOQ of this method was
found 0.033 μg g−1, LOD being 0.01 μg g−1. The DT50 of spiromesifen when applied at recommended doses in chili fruits was found to be 2.18–2.40 days. Ninety-nine percent degradation
was found to occur within 14.5–16.3 days after application. Residues of spiromesifen were not detected in cotton seed and
lint samples at the first picking. In soil, no residues of spiromesifen were detectable 15 days after treatment. 相似文献
990.
Live feeds, especially Tubifex spp., which are collected from a wide variety of polluted habitats, are used by aquarium fish keepers in India. These habitats
receive domestic sewage and industrial wastes from nearby residential and industrial areas. Reports of morbidity and mortality
from aquarium fish culturists in and around Mumbai led to the present investigations on the ecology of these habitats with
a view to assess the water quality, presence of heavy metals in the environment and their bioaccumulation in Tubifex worms, and to examine whether these habitats could be exploited to meet the demand of the industry. Six natural red worm
(Tubifex spp.) collection centres in Mumbai and Thane districts of Maharashtra state in India constituting a major source of live
Tubifex supply to aquarium fish industry were evaluated for pollution, heavy metal concentration in water, sediments and in the body
tissues of Tubifex. Data revealed the presence of heavy metals in water and sediments at collection sites and bioaccumulation of cadmium, iron,
lead, zinc and copper in body tissues of Tubifex worms. Cadmium ranged from 2.38 to 7.21 mg/kg, iron 671.9 to 5738 mg/kg, lead 14.95 to 33.49 mg/kg, zinc 60.20 to 166.60 mg/kg
and copper 29.38 to 108.90 mg/kg of dry Tubifex worms. The study suggests that all the six collection sites are polluted and the red worms contaminated with heavy metals
and hence, unfit for use in aquaria or feeding any variety of fish or crustaceans in the hatcheries. 相似文献