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431.
本文详细论述了CuO-ZnO的特性与沉淀过程中pH值变化、沉淀剂种类、沉淀剂的加料方式和催化剂的热处理条件,以及活化气氛等因素之间的相互关系,实验中运用了XRD,BET,XPS等测试手段,对催化剂的结构及其表面性质进行了深入探讨,得到了催化剂的最佳含量组成和催化剂活性组份可能的存在状态。 相似文献
432.
在工业中试装置上进行了水蒸气/氨活化实验,同时开展了脉冲电源的调试运行、脱硫副产物收集一体化、工艺参数以及对副产物成份分析等实验。在烟气流量4500~11000m^3/h、反应器入口温度60-70℃、氨硫化学计量比约1:1、系统连续运行和采用一体化的单电场进行脱硫副产物收集的条件下.得到结果:水蒸气/氨活化脱硫效果明显,并且有较好的副产物收集功能,收集效率20%~30%;副产物中SO4^2-:SO3^2-大于95:5,脱硫效率稳定大于90%,副产物收率大于85%。 相似文献
433.
Jiménez P Parra R Baldasano JM 《Journal of the Air & Waste Management Association (1995)》2005,55(8):1085-1099
The location of the northeastern Iberian Peninsula (NEIP) in the northwestern Mediterranean basin, the presence of the Pyrenees mountain range (with altitudes > 3000 m), and the influence of the Mediterranean Sea and the large valley canalization of Ebro river induce an extremely complicated structure for the dispersion of photochemical pollutants. Air pollution studies in very complex terrains such as the NEIP require high-resolution modeling for resolving the very complex dynamics of flows. To deal with the influence of larger-scale transport, however, high-resolution models have to be nested in larger models to generate appropriate initial and boundary conditions for the finer resolution domains. This article shows the results obtained through the utilization of the MM5-EMICAT2000-CMAQ multiscale-nested air quality model relating the sensitivity regimes for ozone (O3)-nitrogen oxides (NOx)-volatile organic compounds (VOCs) in an area of high geographical complexity, like the industrial area of Tarragona, located in the NEIP. The model was applied with fine temporal (one-hour) and spatial resolution (cells of 24 km, 2 km, and 1 km) to represent the chemistry and transport of tropospheric O3 and other photochemical species with respect to different hypothetical scenarios of emission controls and to quantify the influence of different emission sources in the area. Results indicate that O3 chemistry in the industrial domain of Tarragona is strongly sensitive to VOCs; the higher percentages of reduction for ground-level O3 are achieved when reducing by 25% the emissions of industrial VOCs. On the contrary, reductions in the industrial emissions of NOx contribute to a strong increase in hourly peak levels of O3. At the same time, the contribution of on-road traffic and biogenic emissions to ground-level O3 concentrations in the area is negligible with respect to the pervasive weight of industrial sources. This analysis provides an assessment of the effectiveness of different policies for the control of emission of precursors by comparing the modeled results for different scenarios. 相似文献
434.
Guiling?L.?ZhangEmail author Jing?Zhang Jie?Xu Jingling?L.?Ren Sumei?M.?Liu 《Water, Air, & Soil Pollution: Focus》2007,7(6):645-654
CH4 concentrations in both the surface and bottom waters of Jiaozhou Bay were determined during four surveys in 2003, which showed
variability with both seasons and tidal cycles. Atmospheric fluxes of CH4 in Jiaozhou Bay showed obvious seasonal and spatial variations, with the highest values occurring in summer and the lowest
in winter. The annual emission of CH4 from Jiaozhou Bay was estimated to be . CH4 in the water column of Jiaozhou Bay was found to come from several land-sources including riverine water input, sewage water
input and groundwater input. The spatial and temporal variation in distributions and atmospheric fluxes of CH4 in Jiaozhou Bay was influenced mainly by the input of polluted river waters and the sewage effluents along the eastern coast,
which highlights the effects of human impacts on CH4 emission rates. 相似文献
435.
436.
Phosphate-induced differences in stabilization efficiency for soils contaminated with lead,zinc, and cadmium 总被引:1,自引:0,他引:1
Jie Ren Zhuo Zhang Mei Wang Guanlin Guo Ping Du Fasheng Li 《Frontiers of Environmental Science & Engineering》2018,12(2):10
Phosphates can cost-effectively decrease the mobility of Pb in contaminated soils. However, Pb always coexists with other metals in soil, their competitive reactions with phosphates have not been tested. In this study, the abilities of KH2PO4, K2HPO4, and K3PO4 to stabilize Pb, Zn, and Cd in soils contaminated with a single metal or a ternary metal for different phosphorus/metal molar ratios were investigated. Results indicated that the stabilization efficiency of KH2PO4, K2HPO4, and K3PO4 for Pb, Zn, and Cd in single metal contaminated soil (P/M ratio 0.6) was 96.00%–98.74%, 33.76%–47.81%, and 9.50%–55.79%, respectively. Competitive stabilization occurred in the ternary system, Pb exhibited a strong competition, the stabilization efficiency of Zn and Cd reduced by 23.50%–31.64%, and 7.10%–39.26%, respectively. Pyromorphite and amorphous lead phosphate formed with excess KH2PO4 or K2HPO4 addition, while K3PO4 resulted in the formation of a hydroxypyromorphite precipitate. Amorphous Zn and Cd phosphates and hydroxides were the primary products. The immobilization rate of Zn and Cd depends on pH, and increased significantly in response to the excess phosphate application. This approach provides insight into phosphate-induced differences in stabilization efficiency in soils contaminated with multiple metals, which is of theoretical and engineering significance.
相似文献
437.
华南退化草坡自然恢复中物种多度分布的动态与模拟 总被引:2,自引:0,他引:2
华南地区退化草坡自然恢复过程中物种多度格局的动态及其模拟,尚缺乏较为系统的研究.文章探讨是否不同演替阶段群落适合不同的种多度模型,是否存在一个最佳模型以揭示演替过程中群落结构的某些内在数量特征;还要推导多个模型的尺度转换形式.为此,在地处南亚热带的鹤山退化草坡选取处于不同演替阶段的2个典型群落样地,分木本层和草本层调查每个维管植物种的多度;且选择7个具有不同函数形式和广泛代表性的种多度模型,均在倍程(即log2)尺度下拟合数据,运用卡方检验和调整决定系数评估各个模型的适合性.结果表明:(1)7个模型的适合性顺序为:对数柯西>对数双曲正割>对数正态>对数级数>生态位优先占领>断棒>重叠生态位,其中对数柯西适合全部数据,重叠生态位则全部不适合;(2)各模型适合与否和演替阶段无关;(3)左截断对数柯西模型预测的种多度分布显示,随着群落演替,上层(木本层)罕见种比例减少、常见种比例增多,下层(草本层)则相反,这与实际相符.对数柯西分布具有普适性,能最好地反映退化草坡自然恢复中种多度分布的格局与动态. 相似文献
438.
439.
440.
上海都市工业区经济规模评价及其优化研究 总被引:7,自引:1,他引:7
工业空间集聚是区域经济发展与结构调整的重要组成部分,包括两种形式:一是农村区域广泛分布着的乡镇企业向周围工业小区的相对集中:二是都市区域工业通过辐射、扩散向新的工业区集中。工业区规模评价通常包括土地规模评价与经济规模评价两个方面。主要从经济规模入手,通过因子分析方法,计算出上海都市工业区经济规模状况的排序结果,并据此进行分析。计算结果发现:目前上海九大都市工业区的因子总分级分布均相对偏低,说明大多数工业区的整体经济规模尚小。为此,需要合理规划,组织协调,加大招商力度;逐步强化信息网络与中介服务功能,按照“限制数量、扩大规模、优化布局”的目标,促进上海都市工业区的优化发展。 相似文献