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121.
Mineralization of paracetamol in aqueous medium by anodic oxidation with a boron-doped diamond electrode 总被引:6,自引:0,他引:6
Brillas E Sirés I Arias C Cabot PL Centellas F Rodríguez RM Garrido JA 《Chemosphere》2005,58(4):399-406
The degradation of 100ml of solutions with paracetamol (N-(4-hydroxyphenyl)acetamide) up to 1 g l(-1) in the pH range 2.0-12.0 has been studied by anodic oxidation in a cell with a boron-doped diamond (BDD) anode and a graphite cathode, both of 3-cm2 area, by applying a current of 100, 300 and 450 mA between 25 and 45 degrees C. Complete mineralization is always achieved due to the great concentration of hydroxyl radical (*OH) generated at the BDD surface, with release of NH4+ and NO3- ions. The mineralization rate is pH-independent, increases with increasing applied current and temperature, but decreases when drug concentration raises from 315 mg l(-1). Reversed-phase chromatography revealed a similar complex paracetamol decay in acid and alkaline media. Ion-exclusion chromatography allowed the detection of oxalic and oxamic acids as ultimate carboxylic acids. When the same solutions have been comparatively treated with a Pt anode, a quite poor mineralization is found because of the production of much lower *OH concentration. Under these conditions, the degradation rate is enhanced in alkaline medium and polymerization of intermediates is favored in concentrated solutions. Paracetamol can be completely destroyed with Pt and its kinetics follows a pseudo-first-order reaction with a constant rate independent of pH. 相似文献
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Pimenteira CA Pereira AS Oliveira LB Rosa LP Reis MM Henriques RM 《Waste management (New York, N.Y.)》2004,24(9):889-897
The present paper aims to make the energy saving potential provided by waste recycling in Brazil evident by pointing out more specifically the benefits regarding climate change mitigation. In this case, based on the energy saved due to the recycling process of an exogenous amount of waste, we have built two scenarios in order to show the potential for indirectly avoiding CO2 emissions in the country as a result of the recycling process. According to the scenario, 1 Mt and 3.5 Mt of CO2, respectively, would be avoided per year due to solid waste recycling. The international context for greenhouse gas emissions reduction, such as the United Nations Framework Convention on Climate Change and its Kyoto Protocol has been taken into account. 相似文献
124.
Fernández Pilar Rose Neil L. Vilanova Rosa M. Grimalt Joan O. 《Water, Air, & Soil Pollution: Focus》2002,2(2):261-274
Spheroidal carbonaceous particles (SCP) and polycyclicaromatic hydrocarbons (PAH) have been measured in the dated sediment cores of 10 remote lakes distributed across Europe. The geographic trends were evaluated by examination of the superficial sediment fluxes and total sediment inventories. The highest levels of both markers were observed in the Eastern European lakes whereas the minimal values corresponded to the lake located in the Arctic. However, this SCP-PAH correlation was not observed after exclusion of the end member lakes from the series. The temporal trends of both pollutant markers are consistent with the history of pyrolytic emissions over Europe. However, the downcore SCP distributions are shorter than the PAH profiles in nearly all lakes. The differences are probably related to the different size particle fractions involved in the measurement of each marker, >5 and >1 m for SCP and PAH, respectively. Thus, the two proxies probably reflect pollution inputs from closer (SCP) and more distant sites (PAH). 相似文献
125.
Posada-Baquero R Niqui-Arroyo JL Bueno-Montes M Gutiérrez-Dabán A Ortega-Calvo JJ 《Environmental geochemistry and health》2008,30(2):159-163
The aim of this work was to develop a method to assess the microbial accessibility of native phenanthrene present in soils
and sediments. We developed an accelerated biodegradation assay, characterized by (a) inoculation with a sufficient number
of phenanthrene-degrading microorganisms, (b) monitoring of the biodegradation activity through 14C-mineralization measurements, and (c) single-step chemical analysis of the native compound in the residue. The use of 14C-labeling allowed the determination of the time period needed for biodegradation of the bioaccessible fraction of the native
chemical. The method was tested with environmental samples having a wide range of phenanthrene concentrations, i.e., from
background levels (μg kg-1) originating in soil from atmospheric deposition, to acute concentrations (g kg-1) corresponding to industrial pollution of soils and sediments. The results showed a wide range of bioaccessibility (15–95%
of the initial amount). The method can be used for the assessment of bioaccessibility involved in the management of polycyclic
aromatic hydrocarbon (PAH) pollution. 相似文献
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127.
The Power of Innovation and Strategic Sustainability Positioning: A Survey of the Mining Sector in Brazil
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Luciana Aparecida Barbieri da Rosa Clandia Maffini Gomes Jordana Marques Kneipp Ana Paula Perlin 《环境质量管理》2015,25(2):47-62
This study investigates the relationship between the power of innovation and the sustainability strategies of companies involved in the minerals extraction sector in Brazil. The study included companies associated with the Brazilian Mining Institute, and it used research surveys to gather data. Analysis of the survey data revealed that companies with highly intensive characteristics in regard to innovation and environmental activities (environmental management activities) also display offensive, or proactive, strategies for pursuing sustainability. 相似文献
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Silva Neicí Cáceres Poetini Márcia Rósula Bianchini Matheus Chimelo Almeida Francielli Polet Dahle Mustafá Munir Mustafa Araujo Stífani Machado Bortolotto Vandreza Cardoso Musachio Elize Aparecida Santos Ramborger Bruna Piaia Novo Diogo La Rosa Roehrs Rafael Mesko Marcia Foster Prigol Marina Puntel Robson Luiz 《Environmental science and pollution research international》2021,28(14):17519-17531
Environmental Science and Pollution Research - Manganese (Mn) is an essential element that, in excess, seems to be involved in the development of different neurodegenerative conditions.... 相似文献