A well-dated pollen record from a large lake located on the meadow-steppe ecotone provides a history of ecotone shift in response to monsoonal climate changes over the last 6000 years in the central Tibetan Plateau. The pollen record indicates that the ecotone shifted eastward during 6000-4900, 4400-3900, and 2800-1600 cal. yr BP when steppes occupied this region, whereas it shifted westward during the other intervals when the steppes were replaced by meadows. The quantitative reconstruction of paleoclimate derived from the pollen record shows that monsoon precipitation fluctuated around the present level over the last 6000 years in the central Tibetan Plateau. Three major drought episodes of 5600-4900, 4400-3900, and 2800-2400 cal. yr BP are detected by pollen signals and lake sediments. Comparison of our record with other climatic proxy data from the Tibetan Plateau and other monsoonal regions shows that these episodes are three major centennial-scale monsoon weakening events. 相似文献
Environmental Science and Pollution Research - This study evaluated the reutilization of waste materials (scrap tires, sewage sludge, and wood chips) to remove volatile organic compounds (VOCs)... 相似文献
This study analyzed the wintertime surface heat exchange for the Inner Mongolia reach of the Yellow River, China, based on the data from the nearby weather station at Wulateqianqi. In this analysis, the solar radiation is based on the observed data. Other components of the surface heat flux, that is, long‐wave radiation, and evaporative and conductive heat fluxes, are calculated. The relative importance of the contributions of long‐wave radiation, conductive, and evaporative heat fluxes are in descending order. The air temperature is the most important meteorological factor to the total heat flux. Although the wind speed influences evaporative and conductive heat fluxes, it has the least correlation with the total heat budget. The heat exchange coefficient for the linearized surface heat exchange equation is 21.87 W/(m2 °C), which is comparable with published values in the regions of United States and Canada with similar latitudes. 相似文献
To investigate the spatial distribution and diurnal variation of the chemical composition of PM2.5 pollution in an industrial city of southern Taiwan, 12-h PM2.5 was diurnally continuously collected simultaneously at the Kaoping Air Quality Zone (KAQZ) during one highly PM2.5-polluted episode. Water-soluble ions, metallic elements, carbonaceous contents, dicarboxylic acids, and anhydrosugars were analyzed to characterize the chemical fingerprint of PM2.5. Backward trajectory simulation and chemical mass balance (CMB) receptor modeling were applied to identify the potential sources of PM2.5 and their contributions. It showed that Chaozhou (rural area) accompanying the highest SORs and NORs suffered from the most severe PM2.5 pollution during the episode. Sulfate (SO42−) was probably formed by the atmospheric chemical reaction in the daytime, while NO3− processed at nighttime at the KAQZ. A homogeneous formation of NO3− occurred at Chaozhou. The concentrations of Zn, Pb, Fe, Cu, V, and Al, mainly emitted from anthropogenic sources, increased significantly at the KAQZ. The highest OC, SOC/OC, and DA/OCs at Daliao (industrial area) were attributed to the transformation of primary VOCs to secondary OC via photo-oxidation during the episode. Oxalic acid was mainly produced through photochemical reactions since a high correlation between oxalic acid and Ca2+ was observed at Nanzi (urban area) and Daliao during the episode. During the episode, PM2.5 mostly originated from local primary or secondary aerosol than long-range overseas transport. The dominant source was anthropogenic emissions, accounting for 67.1% and 70.4% of PM2.5 at Nanzi and Daliao, respectively. At Chaozhou, the contribution of anthropogenic emissions was the lowest (42.4%), but secondary aerosols had the highest contribution of 38.3% of PM2.5 among the three areas during the episode. 相似文献
Aeolian dust episodes (ADEs) have been an emergency disaster in the Kaoping River Valley during the rainy season (May-September), which can severely deteriorate ambient particulate air quality in the region surrounding the Kaoping River. Thus, this study aims to characterize the metallic fingerprint of Aeolian dust (AD) and investigate the effects of ADEs on ambient particulate air quality along the Kaoping River Valley. Four manual sampling sites adjacent to the riverside were selected to collect fine (PM2.5) and coarse (PM2.5–10) aerosol samples during and after the ADEs in the periods of six events. A total of 13 metallic elements were analyzed using an inductively coupled plasma-atomic emission spectrometer. With metallic elements analysis and nonparametric statistical methods of Wilcoxon rank-sum test and Kruskal-Wallis test, this study successfully derived the metallic indicators of ADEs. The mass ratios of crustal elements (Fe, Ca, or Al) to reference element (Cd) obtained during the ADEs were much higher than those obtained after the ADEs. High mass ratios of Fe/Cd, Ca/Cd, and Al/Cd in PM2.5-10 were observed on the influenced areas of ADEs. Among them, (Fe/Cd)2.5-10 was proven as the best indicator which can be applied to effectively validate the existence of ADEs and evaluate their influences on ambient air quality. Moreover, PM2.5 concentrations during the ADEs were 3-3.6 fold higher than those after the ADEs. PM2.5 should be a contributor to AD, even though the mass ratios of PM2.5/PM10 ranged from 0.05 to 0.20 during the ADEs. Our findings provide valuable information regarding the characteristics of the AD during the ADEs in the Kaoping River.
Implications: Indicators of (Fe/Cd)2.5-10 are approximately applied to observe the effects of ADEs. Local governments could realize the mechanisms of S- and NW-type aeolian dust episodes (ADEs). They can cause deterioration in different ways for the regional air quality surrounding Kaoping River Valley. Residents who have been living in the influenced areas can take precautions to prevent damage from aeolian dust. Strategies for curbing ADEs must reduce the area of bare lands by artificial measures in the long period of the sunny days during the rainy season. Future research should examine physical conditions of topsoils and other chemical composition in aeolian dust. 相似文献