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531.
Renbo Zhu Yongsheng Cai Yuxiang Chen Tong Yang Boyu Duan 《Journal of the Air & Waste Management Association (1995)》2016,66(4):402-411
Stainless steel plant dust is a hazardous by-product of the stainless steelmaking industry. It contains large amounts of Fe, Cr, and Ni, and can be potentially recycled as a raw material of inorganic black pigment in the ceramic industry to reduce environmental contamination and produce value-added products. In this paper, ceramic tiles prepared with black pigment through recycling of stainless steel plant dust were characterized in terms of physical properties, such as bulk density, water absorption, apparent porosity, and volume shrinkage ratio, as well as the long-term leaching behavior of heavy metals (Cr, Ni, Pb, Cd, and Zn). The results show that good physical properties of ceramic tiles can be obtained with 8% pigments addition, sample preparation pressure of 25 MPa, and sintering at 1200 ºC for 30 min. The major controlling leaching mechanism for Cr and Pb from the ceramic tiles is initial surface wash-off, while the leaching behavior of Cd, Ni, and Zn from the stabilized product is mainly controlled by matrix diffusion. The reutilization process is safe and effective to immobilize the heavy metals in the stainless steel plant dust.
Implications: Stainless steel plant dust is considered as a hazardous material, and it can be potentially recycled for black pigment preparation in the ceramic industry. This paper provides the characteristics of the ceramic tiles with black pigment through recycling stainless steel plant dust, and the long-term leaching behavior and controlling leaching mechanisms of heavy metals from the ceramic tile. The effectiveness of the treatment process is also evaluated. 相似文献
532.
533.
以68台燃油锅炉(≤10.5 MW)NO_x排放实测数据为基础,通过统计分析方法,研究了NO_x的排放特征;通过对比分析,探讨了我国燃油锅炉NO_x排放控制与管理现状,讨论了进一步加强我国燃油锅炉NO_x排放管理控制的可能性与可行性,并提出了相应的管理控制建议。结果表明,NO_x平均排放浓度为318.2 mg/m~3,基于燃料消耗量的平均排放因子为4.4 kg/t,基于燃料发热量的平均排放因子为102.8 ng/J,基于燃料氮含量的平均排放因子为2.1 mg/mg;建议采取分阶段控制的方式,逐步提高NO_x排放限制,从而实现控源减排目标。 相似文献
534.
Hang Xiao Hayley Hung Ying Duan Lei Frank Wania 《Atmospheric environment (Oxford, England : 1994)》2009,43(15):2401-2409
At locations without access to the electrical grid, a flow-through sampler (FTS) collects large volumes of air for the analysis of semi-volatile organic compounds (SVOCs). To test its performance under field conditions, an FTS and a traditional pumped high volume air sampler, both using polyurethane foam (PUF) as sampling medium, were co-deployed at the campus of the University of Toronto Scarborough from August 2006 to June 2007. Polybrominated diphenyl ethers (PBDEs) and various pesticides were quantified in the samples taken by both samplers to test the FTS's applicability to relatively non-volatile and slightly polar SVOCs. Air concentrations in samples taken with the FTS over five 2-week periods compare favourably with the average of the concentrations in several 24-h active high volume samples taken during the same period. In particular, time trends, temperature dependence relationships, and isomer ratios show a reasonable agreement between the two sampling techniques. An empirical linear solvation energy relationship for predicting the apparent theoretical plate number of the PUF assembly used in the FTS illustrates the effect of chemical properties, as well as temperature and wind speed, on sampling efficiency. In the absence of electrical power, the FTS can collect SVOCs from large air volumes as reliably and quantitatively as traditional HiVol samplers, although without separating gas and particle phase. 相似文献
535.
近年来,SiC材料作为一种新型的柴油车尾气颗粒物过滤材料获得了迅速发展,正逐步取代目前广泛应用的堇青石多孔陶瓷材料.结合堇青石和SiC过滤材料的性能特点,重点概述了2种SiC改性过滤材料(重结晶SiC.RSiC和硅结合SiC,Si-SiC)的研究和应用进展,并介绍了SiC颗粒物过滤器的市场现状和发展前景. 相似文献
536.
Characteristics of atmospheric non-methane hydrocarbons during haze episode in Beijing, China 总被引:1,自引:0,他引:1
Songjun Guo Jihua Tan Jingchun Duan Yongliang Ma Fumo Yang Kebin He Jimin Hao 《Environmental monitoring and assessment》2012,184(12):7235-7246
This study firstly focused on non-methane hydrocarbons (NMHCs) during three successive days with haze episode (16–18 August 2006) in Beijing. Concentrations of alkanes, alkenes, aromatic hydrocarbons, and ethyne all peaked at traffic rush hour, implying vehicular emission; and alkanes also peaked at non-traffic rush hour in the daytime, implying additional source. Especially, alkanes and aromatics clearly showed higher levels in the nighttime than that in the daytime, implying their active photochemical reactions in the daytime. Correlation coefficients (R 2) showed that propane, n-butane, i-butane, ethene, propene, and benzene correlated with ethyne (R 2?=?0.61–0.66), suggesting that their main source is vehicular emission; 2-methylpentane and n-hexane correlated with i-pentane (R 2?=?0.61–0.64), suggesting that gasoline evaporation is their main source; and ethylbezene, m-/p-xylene, and o-xylene correlated with toluene (R 2?=?0.60–0.79), suggesting that their main source is similar to that of toluene (e.g., solvent usage). The R 2 of ethyne, i-pentane, and toluene with total NMHCs were 0.58, 0.76, and 0.60, respectively, indicating that ambient hydrocarbons are associated with vehicular emission, gasoline evaporation, and solvent usage. The sources of other hydrocarbons (e.g., ethane) might be natural gas leakage, biogenic emission, or long-range transport of air pollutants. Measured higher mean B/T ratio (0.78?±?0.27) was caused by the more intensive photochemical activity of toluene than benzene, still indicating the dominant emission from vehicles. 相似文献
537.
Guofeng Wu Lijuan Cui Hongtao Duan Teng Fei Yaolin Liu 《Environmental monitoring and assessment》2013,185(5):4191-4206
Obtaining and analyzing the specific inherent optical properties (SIOPs) of water bodies is necessary for bio-optical model development and remote sensing-based water quality retrievals and, further, for related ecological studies of aquatic ecosystems. This study aimed to measure and analyze the specific absorption and backscattering coefficients of the main water constituents in Poyang Lake, China. The specific absorption and/or backscattering coefficients of the main water constituents at 85 sampling sites (47 in 2010 and 38 in 2011) were measured and analyzed as follows: (1) the concentrations of chlorophyll a (C CHL), suspended particulate matter (C SPM) (including suspended particulate inorganic matter (C SPIM) and suspended particulate organic matter (C SPOM)), and the absorption coefficients of total particulate (a p), phytoplankton (a ph), and non-pigment particulate (a d) were measured in the laboratory; (2) the total backscattering coefficients at six wavelengths of 420, 442, 470, 510, 590, and 700 nm, including the contribution of pure water, were measured in the field with a HydroScat-6 backscattering sensor, and the backscattering coefficients without the contribution of pure water (b b) were then derived by subtracting the backscattering coefficients of pure water from the total backscattering coefficients; (3) the specific absorption coefficients of total particulate ( $ a_{\mathrm{p}}^{ * } $ ), phytoplankton ( $ {a_{{\mathrm{ph}}}}^{ * } $ ), and non-pigment particulate ( $ a_{\mathrm{d}}^{ * } $ ) were calculated by dividing a p, a ph, and a d by C SPM, C CHL, and C SPIM, respectively, while the specific backscattering coefficients of total suspended particulate matter ( $ b_{\mathrm{b}}^{ * } $ ) were calculated by dividing b b by C SPM; and (4) the $ {a_{{\mathrm{ph}}}}^{ * } $ , $ a_{\mathrm{d}}^{ * } $ , $ a_{\mathrm{p}}^{ * } $ and $ b_{\mathrm{b}}^{ * } $ of the remaining samples (46 in 2010 and 36 in 2011) were visualized and analyzed, and their relations to C CHL, C SPIM or C SPM were studied, respectively. The main results are summarized as follows: (1) the $ {a_{{\mathrm{ph}}}}^{ * } $ values at 440 nm were 0.0367–0.7203 m2?mg?1 with a mean of 0.1623?±?0.1426 m2?mg?1 in 2010 and 0.0319–0.7735 m2?mg?1 with a mean of 0.3145?±?0.1961 m2?mg?1 in 2011; there existed significant, negative, and moderate correlations between $ {a_{{\mathrm{ph}}}}^{ * } $ and C CHL at 400–700 nm in 2010 and 2011 (p?<?0.05); (2) The $ a_{\mathrm{d}}^{ * } $ values at 440 nm were 0.0672–0.2043 m2?g?1 with a mean of 0.1022?±?0.0326 m2?g?1 in 2010 and 0.0559–0.1347 m2?g?1 with a mean of 0.0953?±?0.0196 m2?g?1 in 2011; there existed negative correlations between $ a_{\mathrm{d}}^{ * } $ and C SPIM, while the correlations showed overall decreasing and increasing trends before and after around 575 nm with increasing wavelengths, respectively; (3) The $ a_{\mathrm{p}}^{ * } $ values at 440 nm were 0.0690–0.1929 m2?g?1 with a mean of 0.1036?±?0.0298 m2?g?1 in 2010 and 0.0571–0.1321 m2?g?1 with a mean of 0.1014?±?0.0191 m2?g?1 in 2011, and the negative correlations between $ a_{\mathrm{p}}^{ * } $ and C SPM were found in both years; (4) The $ b_{\mathrm{b}}^{ * } $ at the six wavelengths generally decreased with increasing wavelengths, while the $ b_{\mathrm{b}}^{ * } $ values at 420 nm were lower than those at 442 nm for some samples; the correlation between $ b_{\mathrm{b}}^{ * } $ and C SPM increased with increasing wavelength. Such results can only represent the SIOPs during the sampling time periods, and more measurements and analyses considering different seasons need to be carried out in the future to comprehensively understand the SIOPs of Poyang Lake. 相似文献
538.
Dissolved inorganic tin (DISn) and its spatial variation were examined in Bohai Bay seawaters to understand the DISn behavior
and pollution in this area. DISn concentration gradually increased with the distance from the coast and showed a slight decrease
with the increasing depth from surface water, suggesting the scavenged behavior of tin with an atmospheric input to surface
water. Besides, the higher DISn values also were found near the Haihe Estuary inferring that the riverine input was a source
of DISn. Based on the data in this study, a preliminary estimate of the tin budget via riverine input and atmospheric deposition
has been established. According to our estimate, about 2 × 106 and 8.47 × 105 g/year of tin reach Bohai Bay via rivers and atmosphere. Environmental factors such as suspended particulate material, salinity,
total organic matter, pH, nutrients, and phytoplankton had the important influences on DISn distribution. Among them, the
negative correlation between DISn and phytoplankton at most stations might indicate the biological uptake of tin. 相似文献
539.
陕西省引汉济渭工程属于跨流域大型水利工程,5个单元工程呈线状跨越构造剥蚀山地和断陷盆地,工程地质性质差异大,易发生地质灾害。实地调查地质灾害点共72处,其中滑坡66处,崩塌3处,泥石流3处。现状评估认为地质灾害危险性中等13处,其余59处均为危险性小。预测评估认为工程本身可能遭受31处地质灾害威胁,危险性小28处,危险性中等3处;工程建设可能加剧地质灾害39处,危险性小36处,危险性中等3处;工程建设可能引发地质灾害30处,危险性小15处,危险性中等15处。综合评估工程主要位于危险性小的区段,受地质灾害危害不大,风险较低。 相似文献
540.
Fanhao Meng Min Qin Wu Fang Jun Duan Ke Tang Helu Zhang Dou Shao Zhitang Liao Yan Feng Yong Huang Ting Ni Pinhua Xie Jianguo Liu Wenqing Liu 《环境科学学报(英文版)》2022,34(4):297-307
To investigate nitrous acid(HONO) levels and potential HONO sources above crop rotation fields. The HONO fluxes were measured by the aerodynamic gradient(AG) method from 14 December 2019 to 2 January 2020 over an agricultural field in the Huaihe River Basin. The ambient HONO levels were measured at two different heights(0.15 and 1.5 m), showing a typical diurnal cycle with low daytime levels and high nighttime levels. The upward HONO fluxes were mostly observed during the day, whereas deposition... 相似文献