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排序方式: 共有474条查询结果,搜索用时 109 毫秒
151.
Trnovec T Dedík L Jusko TA Lancz K Palkovičová L Kočan A Šovčíková E Wimmerová S Tihányi J Patayová H Hertz-Picciotto I 《Chemosphere》2011,85(11):1687-1693
Investigators have typically relied on a single or few discrete time points as measures of polychlorinated biphenyl (PCB) body burden, however health effects are more likely to be the result of integrative exposure in time, optionally expressed as an area under the time curve (AUC) of PCB serum concentration. Using data from a subgroup of 93 infants from a birth cohort in eastern Slovakia—a region highly polluted by PCBs—we fit a system type model, customized to our longitudinal measures of serum PCB concentrations in cord, 6, 16, and 45 month blood specimens. The most abundant congener, PCB 153, was chosen for modeling purposes. In addition to currently used methods of exposure assessment, our approach estimates a concentration time profile for each subject, taking into account mean residence time of PCB 153 molecules in the body, duration of breast feeding, hypothetical PCB 153 concentration in steady-state without breast feeding and alternately without normal food intake. Hypothetical PCB 153 concentration in steady-state without normal food intake correlates with AUC (r = 0.84, p < 0.001) as well as with duration of breast feeding (r = 0.64, p < 0.001). It makes possible to determine each subject’s exposure profile expressed as AUC of PCBs serum concentration with a minimum model parameters. PCB body burden in most infants was strongly associated with duration of breast feeding in most, but not all children, was apparent from model output. 相似文献
152.
Lazar B Maslov L Romanić SH Gračan R Krauthacker B Holcer D Tvrtković N 《Chemosphere》2011,82(1):121-129
We analyzed 15 polychlorinated biphenyls (PCBs) and five organochlorine pesticides (OCPs) in fat tissue of 27 loggerhead sea turtles (Caretta caretta) from eastern Adriatic Sea with the curved carapace length ranging from 25.0 to 84.5 cm. The PCB profile was dominated by hexa- and hepta-chlorinated congeners, with PCB-153 (median: 114.9 ng g−1 wet mass), PCB-138 (80.0 ng g−1 w.m.), and PCB-180 (26.7 ng g−1 w.m.) detected with the highest levels. Toxic mono-ortho congeners PCB-118, PCB-105 and PCB-180 with dioxin-like toxicity were found in >70% samples. 4,4′-DDE (81.0 ng g−1 w.m.) prevailed the OCP signature, accounting for 80% of the total DDTs. A significant increasing trend in accumulation with size was found for PCB-52 (rs = 0.512, p < 0.01) and PCB-114 (rs = 0.421, p < 0.05). Comparison of our results with organochlorine contaminant (OC) pattern in some prey taxa suggest that contamination occurs primarily through the food web, with biomagnification factors of 0.14-6.99 which were positively correlated with the octanol-water partition coefficient (log Kow; p < 0.05). This study, based upon a fairly large sample size collected mostly from incidentally captured animals over a short time period (June 2001-November 2002), present a temporal snapshot of OC contamination in wild, free-ranging loggerheads from Adriatic feeding grounds and provide a baseline for monitoring the regional OC trends in this endangered species. 相似文献
153.
Josef Hrnčiřík Jiří Pšeja Jan Kupec Světlana Bernkopfová 《Journal of Polymers and the Environment》2010,18(2):98-103
This work focused on anaerobic biodegradation of blends composed of glycerol-plasticized polyvinyl alcohol (PVA) and biopolymer
(starch, gellan, xanthan) in an aqueous environment, after inoculation with digested activated sludge from a municipal wastewater
treatment plant. Glycerol degradability is comparable to degradability of used modifying agents. Modifying agents added in
the 20–40 wt% range proportionally increased biodegradation degree (Dt) calculated from balance of transformed carbon in the system. Biodegradation degree of polysaccharides and glycerol attained
95% and over. For PVA it was only 6.5% (in breakdown times up to 500 h). Content of polysaccharides favorably affects biodegradation
degree of polyvinyl alcohol blends, but at the expense of reduced mechanical properties of resultant products. 相似文献
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155.
Irena Ciglenečki Srđan Pichler Esad Prohić Božena Ćosović 《Water, Air, & Soil Pollution: Focus》2006,6(5-6):537-545
Geochemical, mineralogical and sedimentological analyses were carried out to contrast two different sites (respectively characterized
by permanently oxic and anoxic conditions) in a small, meromictic, seawater lake. In fact, due to relatively high organic
matter content, and reduced water exchange, the Rogoznica Lake has almost permanent anoxic conditions below the depth of 12 m,
where sediment can be considered an anoxic–sulphidic sedimentary environment. Different water column and sediments redox conditions
affect the distribution and speciation of major redox-sensitive metals (Fe, Mn, Mo), reduced sulphur species (RSS) and dissolved
organic C (DOC). Trace metals, especially those that accumulate in anoxic–sulphidic environments (Fe, Mo) showed a marked
enrichment in the solid phase, whereas the low solubility of sulphides leads to low porewater concentrations. The relatively
high sedimentary enrichment of Mo (up to 81 mg/kg) also confirms highly anoxic conditions within the Rogoznica Lake sediments.
Results clearly show that chemical species within the sediments will tend towards equilibrium between porewater and solid
phase according the prevailing environment conditions such as redox, pH, salinity, DOC. 相似文献
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