全文获取类型
收费全文 | 21298篇 |
免费 | 184篇 |
国内免费 | 142篇 |
专业分类
安全科学 | 459篇 |
废物处理 | 857篇 |
环保管理 | 2343篇 |
综合类 | 4395篇 |
基础理论 | 4796篇 |
环境理论 | 9篇 |
污染及防治 | 5316篇 |
评价与监测 | 1449篇 |
社会与环境 | 1926篇 |
灾害及防治 | 74篇 |
出版年
2022年 | 163篇 |
2021年 | 193篇 |
2019年 | 150篇 |
2018年 | 292篇 |
2017年 | 303篇 |
2016年 | 451篇 |
2015年 | 322篇 |
2014年 | 533篇 |
2013年 | 1537篇 |
2012年 | 611篇 |
2011年 | 853篇 |
2010年 | 661篇 |
2009年 | 766篇 |
2008年 | 898篇 |
2007年 | 963篇 |
2006年 | 824篇 |
2005年 | 716篇 |
2004年 | 729篇 |
2003年 | 705篇 |
2002年 | 653篇 |
2001年 | 830篇 |
2000年 | 547篇 |
1999年 | 369篇 |
1998年 | 241篇 |
1997年 | 257篇 |
1996年 | 269篇 |
1995年 | 300篇 |
1994年 | 285篇 |
1993年 | 260篇 |
1992年 | 243篇 |
1991年 | 246篇 |
1990年 | 254篇 |
1989年 | 214篇 |
1988年 | 202篇 |
1987年 | 187篇 |
1986年 | 193篇 |
1985年 | 187篇 |
1984年 | 211篇 |
1983年 | 196篇 |
1982年 | 212篇 |
1981年 | 176篇 |
1980年 | 174篇 |
1979年 | 161篇 |
1978年 | 160篇 |
1977年 | 140篇 |
1976年 | 124篇 |
1975年 | 132篇 |
1974年 | 140篇 |
1973年 | 124篇 |
1972年 | 124篇 |
排序方式: 共有10000条查询结果,搜索用时 281 毫秒
951.
The concentrations of biocides leached from antifouling coatings are monitored in most of the developed countries. However, in India and many other developing countries, there is very little data available on the concentrations of biocides in ports and harbours. The first step was to obtain the order of magnitude levels of concentrations of biocides in the marine environment of the Visakhapatnam Harbour, and the MAM-PEC (Marine Antifoulant Model to Predict Environmental Concentrations) model was used to predict these values. The Visakhapatnam Port lies on the eastern coast of India, roughly halfway between Chennai and Kolkata, and is the largest port in India. This port is a natural harbour; the long and narrow outlet to the open sea makes it a 'poorly flushed' harbour. Predicted concentrations of tributyltin (TBT), copper, dichlofluanid, seanine, irgarol, diuron, tolylfluanid, and zinc pyrithione were computed. The results of the computations indicate that the levels of these biocides are comparable to those in many western countries. This gives credence to the fact that persistence of TBT and some other biocides is a global problem that cannot be ignored. 相似文献
952.
S. Maschio E. Furlani G. Tonello N. Faraone E. Aneggi D. Minichelli L. Fedrizzi A. Bachiorrini S. Bruckner 《Waste management (New York, N.Y.)》2009,29(11):2880-2885
The paper describes results obtained in the development of a previous research. We study here, in fast firing, the sintering behaviour and measure some properties of tiles containing a mixture of 60 wt% of paper mill sludge and 40 wt% of glass cullet. The behaviour of this material is compared to those displayed by materials obtained by the same mixture added with 10, 20 and 30 wt% of a natural red clay. In parallel, the same properties are measured also on a reference blend, which is presently used to produce commercial tiles. We show that powders containing 60 wt% of paper sludge and 40 wt% of glass cullet to which 30 wt% of clay is added give rise to materials that display a stable sintering process and have good hardness and strength and therefore could be used for the industrial production of tiles. 相似文献
953.
Nemli G Demirel S Gümüşkaya E Aslan M Acar C 《Waste management (New York, N.Y.)》2009,29(3):1129-1131
This study investigated some of the important physical (thickness swelling) and mechanical (modulus of rupture, modulus of elasticity and internal bond) properties of single-layer particleboard panels made from eucalyptus (Eucalyptus camaldulensis Dehn.), waste of grass clippings (Lolium perenne L.) and combinations of the two. The chemical properties (pH, holocelluse and alpha cellulose contents, and water, alcohol-benzene and 1% sodium hydroxide solubilities) of the raw materials were also determined. Panels with a 6:94 ratio of grass-to-eucalyptus particles had the required mechanical properties for interior fitments including furniture and general uses. Boards manufactured with 100% grass clippings exhibited the lowest quality. The overall panel properties improved with a lower percentage of grass clippings added. Based on initial results, it also appears that grass should compose no more than 13% to achieve acceptable panel properties for interior fitments and general uses. 相似文献
954.
Mårten Bryngelsson Erik G. Lindfeldt Jan Heller 《International Journal of Greenhouse Gas Control》2009,3(3):255-262
This study investigates the possibility of capturing CO2 from flue gas under pressurised conditions, which could prove to be beneficial in comparison to working under atmospheric conditions. Simulations of two hybrid combined cycles with pressurised fluidised bed combustion and CO2 capture are presented. CO2 is captured from pressurised flue gas by means of chemical absorption after the boiler but before expansion. The results show a CO2 capture penalty of approximately 8 percentage points (including 90% CO2 capture rate and compression to 110 bar), which makes the efficiency for the best performing cycle 43.9%. It is 5.2 percentage points higher than the most probable alternative, i.e. using a natural gas fired combined cycle and a pulverised coal fired condensing plant separately with the same fuel split ratio. The largest part of the penalty is associated with the lower mass flow of flue gas after CO2 capture, which leads to a decrease in work output in the expander and potential for feed water heating. The penalty caused by the regeneration of absorbent is quite low, since the high pressure permits the use of potassium carbonate, which requires less regeneration heat than for example the more commonly proposed monoethanolamine. Although the efficiencies of the cycles look promising it will be important to perform a cost estimate to be able to make a fair comparison with other systems. Such a cost estimate has not been done in this study. A significant drawback of these hybrid cycles in that respect is the complex nature of the systems that will have a negative effect on the economy. 相似文献
955.
Stormwater runoff from the University of California, Davis/U.S. Department of Energy Laboratory for Energy‐Related Health Research (UCD/US DOE LEHR) Superfund site located on the University of California campus in Davis, California, has been found to contain over 500 ng/L of total recoverable mercury, which is about ten times the California Toxics Rule criterion. This stormwater runoff is discharged to Putah Creek, which is Clean Water Act Section 303(d) listed as impaired for excessive mercury bioaccumulation in edible fish. A discussion is presented on the potential impact of the mercury in stormwater runoff from LEHR leading to excessive bioaccumulation of mercury in Putah Creek fish. The mercury in the stormwater runoff is derived from former flooding of the soils near the creek, which contains mercury derived from abandoned upstream mercury mines located in the Coast Range Vaca Hills to the west of LEHR. The implications of this situation for implementing a Total Maximum Daily Load (TMDL) to control mercury in stormwater runoff to Putah Creek are presented. © 2009 Wiley Periodicals, Inc. 相似文献
956.
K. Rajakumar V. Sarasvathy A. Thamarai Chelvan R. Chitra C. T. Vijayakumar 《Journal of Polymers and the Environment》2009,17(3):191-202
Polypropylene (PP) has achieved a dominating position and hence, their consumption increases thereby littering, which lead
to environmental pollution. Photodegradation seems to be a better choice because of naturally available sunlight as energy
source for degradation. The present work involves the study of the variation of degradation behavior of PP film during tropical
summer and winter seasons. The photodegradation is followed by Fourier transform infrared (FTIR) spectroscopic technique.
Various indices like hydroxyl, carbonyl, vinylidene, lactones, ester, carboxylic acid and crystallinity are calculated and
these values increased after a brief induction period. The variation in the mechanical properties like tensile strength and
elongation at break percentages are determined. The scanning electron microscopic (SEM) images of weathered PP showed surface
cracks when carbonyl index value increases sharply and the mechanical properties show a sudden decrease. Attempted life time
prediction using mathematical models showed that the carbonyl growth is more affected by ultraviolet (UV) and cumulative total
solar radiation for PP weathered during summer. The loss in tensile strength of PP weathered during summer is more dependent
on the average temperature and the UV portion of the total solar radiation whereas, intensity of UV radiation has profound
effect on the tensile strength of PP weathered during winter. 相似文献
957.
The Effect of Masterbatch Addition on the Mechanical, Thermal, Optical and Surface Properties of Poly(lactic acid) 总被引:1,自引:0,他引:1
F. Byrne P. G. Ward J. Kennedy N. Imaz D. Hughes D. P. Dowling 《Journal of Polymers and the Environment》2009,17(1):28-33
There has been considerable interest in the use of the biodegradable polymer poly(lactic acid) (PLA) as a replacement for
petroleum derived polymers due to ease of processability and its high mechanical strength. Other material properties have
however limited its wider application. These include its brittle properties, low impact strength and yellow tint. In an attempt
to overcome these drawbacks, PLA was blended with four commercially available additives, commonly known as masterbatches.
The effect of the addition of 1.5 wt% of the four masterbatches on the mechanical, thermal, optical and surface properties
of the polymer was evaluated. All four masterbatches had a slight negative effect on the tensile strength of PLA (3–5% reduction).
There was a four fold increase in impact resistance however with the addition of one of the masterbatches. Differential scanning
calorimetry demonstrated that this increase corresponded to a decrease in the polymer crystallinity. However there was an
associated increase in polymer haze with the addition of this masterbatch. The clarity of PLA was improved through the addition
of an optical brightener masterbatch, but the impact resistance remained low. The glass transition and melting temperatures
of PLA were not affected by the addition of the masterbatches, and no change was observed in surface energy. Some delay in
PLA degradation, in a PBS degradation medium at 50 °C, was observed due to blending with these masterbatches. 相似文献
958.
Amit Kapur Hendrik G. van Oss Gregory Keoleian Stephen E. Kesler Alissa Kendall 《Journal of Material Cycles and Waste Management》2009,11(2):155-165
A country-level stock and flow model for cement, an important construction material, was developed based on a material flow
analysis framework. Using this model, the contemporary cement cycle of the United States was constructed by analyzing production,
import, and export data for different stages of the cement cycle. The United States currently supplies approximately 80% of
its cement consumption through domestic production and the rest is imported. The average annual net addition of in-use new
cement stock over the period 2000–2004 was approximately 83 million metric tons and amounts to 2.3 tons per capita of concrete.
Nonfuel carbon dioxide emissions (42 million metric tons per year) from the calcination phase of cement manufacture account
for 62% of the total 68 million tons per year of cement production residues. The end-of-life cement discards are estimated
to be 33 million metric tons per year, of which between 30% and 80% is recycled. A significant portion of the infrastructure
in the United States is reaching the end of its useful life and will need to be replaced or rehabilitated; this could require
far more cement than might be expected from economic forecasts of demand for cement. 相似文献
959.
Mario C.R. Vidal Paulo V.R. Carvalho Marcello S. Santos Isaac J.L. dos Santos 《Journal of Loss Prevention in the Process Industries》2009,22(4):516-527
This article aims to describe the characteristics of collective working situations in complex systems – especially those in nuclear power plants – related to common forms of cooperation, in order to improve systems resilience. In addition, we will try to detail some aspects of collective working situations, emphasizing the differences between various forms of control. The similarities between work activities (multi-addressed messages, linkage to regulation, central and peripheral information) are nonetheless exposed. We conclude by proposing a contribution to support systems design, thus facilitating cooperation in teamwork activities. 相似文献
960.
V. Vađić J. Hršak N. Kalinić M. Čačković K. Šega 《Environmental monitoring and assessment》2000,65(1-2):147-153
Hydrogen sulphide, ammonia, nitrogen dioxide, mercaptans and sulphur dioxide (H2S, NH3, NO2, R-SH, SO2) concentrations were measured at the location in the vicinity of the waste dump to determine the air pollution level of these pollutants prior to the operation of the Mobile Thermal Treatment Plant. Samples were collected over one year period. Seasonal differences, and the influence of meteorological parameters (temperature, relative humidity, pressure and wind direction) on the air pollution levels were studied. Results show relatively low concentrations of H2S, NO2, R-SH and SO2, while NH3 levels were higher compared to the guideline values. Good weather conditions (high air pressure and low relative humidity) are connected to long range transport of NO2, while higher temperatures result in elevated NH3 and R-SH concentrations. Because of the predominant northeast wind direction (the same as the waste dump direction), the contribution of air pollution from the direction of the waste dump at the measuring site is significant, but that does not necessarily mean that the pollutants originated from that source. 相似文献