全文获取类型
收费全文 | 13189篇 |
免费 | 142篇 |
国内免费 | 111篇 |
专业分类
安全科学 | 360篇 |
废物处理 | 346篇 |
环保管理 | 1979篇 |
综合类 | 3301篇 |
基础理论 | 3103篇 |
环境理论 | 6篇 |
污染及防治 | 3327篇 |
评价与监测 | 589篇 |
社会与环境 | 365篇 |
灾害及防治 | 66篇 |
出版年
2018年 | 123篇 |
2017年 | 129篇 |
2016年 | 185篇 |
2015年 | 156篇 |
2014年 | 203篇 |
2013年 | 971篇 |
2012年 | 309篇 |
2011年 | 436篇 |
2010年 | 312篇 |
2009年 | 408篇 |
2008年 | 452篇 |
2007年 | 480篇 |
2006年 | 440篇 |
2005年 | 326篇 |
2004年 | 349篇 |
2003年 | 384篇 |
2002年 | 327篇 |
2001年 | 468篇 |
2000年 | 323篇 |
1999年 | 217篇 |
1998年 | 154篇 |
1997年 | 146篇 |
1996年 | 180篇 |
1995年 | 178篇 |
1994年 | 201篇 |
1993年 | 183篇 |
1992年 | 183篇 |
1991年 | 181篇 |
1990年 | 208篇 |
1989年 | 194篇 |
1988年 | 166篇 |
1987年 | 164篇 |
1986年 | 148篇 |
1985年 | 166篇 |
1984年 | 148篇 |
1983年 | 159篇 |
1982年 | 162篇 |
1981年 | 165篇 |
1980年 | 149篇 |
1979年 | 145篇 |
1978年 | 142篇 |
1977年 | 129篇 |
1976年 | 136篇 |
1975年 | 114篇 |
1974年 | 142篇 |
1973年 | 125篇 |
1972年 | 126篇 |
1971年 | 107篇 |
1970年 | 106篇 |
1967年 | 116篇 |
排序方式: 共有10000条查询结果,搜索用时 187 毫秒
591.
Mobility of radium and trace metals in sediments of the Winterbeek: Application of sequential extraction and DGT techniques 总被引:1,自引:0,他引:1
For several decades, phosphate ores containing 226Ra as well as several trace metals have been processed in Belgium to produce calcium phosphate for use in cattle food. The waste water is discharged in two small rivers, the Laak and the Winterbeek.In this study, the levels of 226Ra and trace metals in surface water and sediments of the Winterbeek were investigated and the mobility of these compounds was assessed using DGT (Diffusive Gradient in Thin Films) and sequential extraction techniques.The concentrations of 226Ra and trace metals in water and sediment indicate a decreasing trend in inputs to the Winterbeek.The mobility of 226Ra, assessed by DGT, is related to the reductive mobilization of Fe. The sequential extraction technique shows that at some stations an important fraction of 226Ra is found to labile sediment phases.Diffusive 226Ra sediment fluxes, are however, relatively small and have only a minor contribution to the water column concentration of 226Ra. 相似文献
592.
Richard C. Warner Carmen T. Agouridis Page T. Vingralek Alex W. Fogle 《Journal of the American Water Resources Association》2010,46(4):724-732
Warner, Richard C., Carmen T. Agouridis, Page T. Vingralek, and Alex W. Fogle, 2010. Reclaimed Mineland Curve Number Response to Temporal Distribution of Rainfall. Journal of the American Water Resources Association (JAWRA) 46(4): 724-732. DOI: 10.1111/j.1752-1688.2010.00444.x Abstract: The curve number (CN) method is a common technique to estimate runoff volume, and it is widely used in coal mining operations such as those in the Appalachian region of Kentucky. However, very little CN data are available for watersheds disturbed by surface mining and then reclaimed using traditional techniques. Furthermore, as the CN method does not readily account for variations in infiltration rates due to varying rainfall distributions, the selection of a single CN value to encompass all temporal rainfall distributions could lead engineers to substantially under- or over-size water detention structures used in mining operations or other land uses such as development. Using rainfall and runoff data from a surface coal mine located in the Cumberland Plateau of eastern Kentucky, CNs were computed for conventionally reclaimed lands. The effects of temporal rainfall distributions on CNs was also examined by classifying storms as intense, steady, multi-interval intense, or multi-interval steady. Results indicate that CNs for such reclaimed lands ranged from 62 to 94 with a mean value of 85. Temporal rainfall distributions were also shown to significantly affect CN values with intense storms having significantly higher CNs than multi-interval storms. These results indicate that a period of recovery is present between rainfall bursts of a multi-interval storm that allows depressional storage and infiltration rates to rebound. 相似文献
593.
Daniel L. Roelke Leslie Schwierzke Bryan W. Brooks James P. Grover Reagan M. Errera Theodore W. Valenti Jr. James L. Pinckney 《Journal of the American Water Resources Association》2010,46(1):76-91
Roelke, Daniel L., Leslie Schwierzke, Bryan W. Brooks, James P. Grover, Reagan M. Errera, Theodore W. Valenti, Jr., and James L. Pinckney, 2010. Factors Influencing Prymnesium parvum Population Dynamics During Bloom Initiation: Results from In-Lake Mesocosm Experiments. Journal of the American Water Resources Association (JAWRA) 46(1):76-91. DOI: 10.1111/j.1752-1688.2009.00392.x Abstract: The alga Prymnesium parvum forms large fish-killing blooms in many Texas lakes. In some of these lakes, however, P. parvum occurs but does not develop blooms. In this study, we investigated factors that may influence bloom initiation by conducting a series of in-lake experiments involving mixing of waters from Lake Whitney, which has a history of P. parvum blooms, with waters from Lake Waco where no blooms have occurred. In all experiments, the addition of Lake Waco waters resulted in a poorer performance of P. parvum. Various experimental treatments and field data show that differences in grazing, pathogens, nutrients, and salts between the two lakes were not likely factors that contributed to this observation. Industrial and agricultural contaminants, allelochemicals and algicidal chemicals were not measured as a part of this research. However, anthropogenic contaminants other than nutrients were not observed at levels exceeding water quality standards in Lake Waco in recent years. On the other hand, nuisance cyanobacteria are common in Lake Waco, where Microcystis sp. and Anabaena sp. were abundant during the initiation of our experiments, both taxa are known to produce chemicals with allelopathic properties. In addition, the emergent field of algal-heterotrophic bacteria interactions suggests that chemicals produced by heterotrophic bacteria should not be overlooked. Further research focusing on the chemical interactions between cyanobacteria and P. parvum, as well as the potential role of algicidal bacteria, in the initiation of P. parvum blooms is necessary, as it may be important to the management of these blooms. 相似文献
594.
Chuan-Yao Lin C.-C. Chang C.Y. Chan C.H. Kuo W.-C. Chen D. Allen Chu Shaw C. Liu 《Atmospheric environment (Oxford, England : 1994)》2010,44(2):182-193
To quantify the possible sources of the high ambient ozone concentration in the low troposphere over Taiwan, ozone sounding data from a two-year intensive field measurement program conducted in April and early May of 2004 and 2005 in northern Taiwan has been examined. We found that the vertical ozone distributions and occurrence of enhanced ozone in the lower troposphere (below 6 km) mainly resulted from (1)Type NE: the long-range transport of ozone controlled by the prevailing northeasterly winds below 2 km, (2)Type LO: the local photochemical ozone production process, and (3)Type SW: the strong southwest/westerly winds aloft (2–6 km). In the boundary layer (BL), where Asian continental outflow prevails, the average profile for type NE is characterized by a peak ozone concentration of nearly 65 ppb at about 1500 m altitude. For type LO, high ozone concentration with an average ozone concentration greater than 80 ppb was also found in the BL in the case of stagnant atmospheric and sunny weather conditions dominated. For type SW, significant ozone enhancement with average ozone concentration of 70–85 ppb was found at around 4 km altitude. It is about 10 ppb greater than that of the types NE and LO at the same troposphere layer owing to the contribution of the biomass burning over Indochina. Due to Taiwan's unique geographic location, the complex interaction of these ozone features in the BL and aloft, especially features associated with northeasterly and south/southwesterly winds, have resulted in complex characteristics of ozone distributions in the lower troposphere over northern Taiwan. 相似文献
595.
David L. MacIntosh James H. Stewart Theodore A. Myatt Joseph E. Sabato George C. Flowers Kirk W. Brown Dennis J. Hlinka David A. Sullivan 《Atmospheric environment (Oxford, England : 1994)》2010,44(2):262-270
CALPUFF is an atmospheric source-receptor model recommended by the U.S. Environmental Protection Agency for use on a case-by-case basis in complex terrain and wind conditions. The ability of the model to provide useful information for exposure assessments in areas with those topographical and meteorological conditions has received little attention. This is an important knowledge gap for use of CALPUFF outside of regulatory applications, such as exposure analyses conducted in support of risk assessments and health studies. We compared deposition of cadmium (Cd), lead (Pb), and zinc (Zn) calculated with CALPUFF as a result of emissions from a zinc smelter with corresponding concentrations of the metals measured in attic dust and soil samples obtained from the surrounding area. On a point-by-point analysis, predictions from CALPUFF explained 11% (lead) to 53% (zinc) of the variability in concentrations measured in attic dust. Levels of heavy metals in soil interpolated to 100 residential addresses from the distribution of concentrations measured in soil samples also agreed well with deposition predicted with CALPUFF: R2 of 0.46, 0.76, and 079 for Pb, Cd, and Zn, respectively. Community-average concentrations of Cd, Pb, and Zn measured in soil were significantly (p < 0.0001) and strongly correlated (R2 ranged from 0.77 to 0.98) with predicted deposition rates. These findings demonstrate that CALPUFF can provide reasonably accurate predictions of the patterns of long-term air pollutant deposition in the near-field associated with emissions from a discrete source in complex terrain. Because deposition estimates are calculated as a linear function of air concentrations, CALPUFF is expected to be reliable model for prediction of long-term average, near-field ambient air concentrations in complex terrain as well. 相似文献
596.
Bridget M. Day Bernhard Rappenglück Craig B. Clements Sara C. Tucker W. Alan Brewer 《Atmospheric environment (Oxford, England : 1994)》2010,44(33):4014-4023
The nocturnal boundary layer in Houston, Texas was studied using a high temporal and vertical resolution tethersonde system on four nights during the Texas Air Quality Study II (TexAQS II) in August and September 2006. The launch site was on the University of Houston campus located approximately 4 km from downtown Houston. Of particular interest was the evolution of the nocturnal surface inversion and the wind flows within the boundary layer. The land–sea breeze oscillation in Houston has important implications for air quality as the cycle can impact ozone concentrations through pollutant advection and recirculation. The results showed that a weakly stable surface inversion averaging in depth between 145 and 200 m AGL formed on each of the experiment nights, typically within 2–3 h after sunset. Tethersonde vertical winds were compared with two other Houston data sets (High Resolution Doppler Lidar and radar wind profiler) from locations near the coastline and good agreement was found, albeit with a temporal lag at the tethersonde site. This comparison revealed development of a land breeze on three nights which began near the coastline and propagated inland both horizontally and vertically with time. The vertical temperature structure was significantly modified on one night at the tethersonde site after the land breeze wind shift, exhibiting near-adiabatic profiles below 100 m AGL. 相似文献
597.
R.J. Wichink Kruit W.A.J. van Pul F.J. Sauter M. van den Broek E. Nemitz M.A. Sutton M. Krol A.A.M. Holtslag 《Atmospheric environment (Oxford, England : 1994)》2010,44(7):945-957
New parameterizations for surface–atmosphere exchange of ammonia are presented for application in atmospheric transport models and compared with parameterizations of the literature. The new parameterizations are based on a combination of the results of three years of ammonia flux measurements over a grassland canopy (dominated by Lolium perenne and Poa trivialis) near Wageningen, the Netherlands and existing parameterizations from literature. First, a model for the surface–atmosphere exchange of ammonia that includes the concentration at the external leaf surface is derived and validated. Second, a parameterization for the stomatal compensation point (expressed as Γs, the ratio of [NH4+]/[H+] in the leaf apoplast) that accounts for the observed seasonal variation is derived from the measurements. The new, temperature-dependent Γs describes the observed seasonal behavior very well. It is noted, however, that senescence of plants and field management practices will also influence the seasonal variation of Γs on a shorter timescale. Finally, a relation that links Γs to the atmospheric pollution level of the location through the ‘long-term’ NH3 concentration in the air is proposed. 相似文献
598.
Lambert A. Doezema Chris Bigley Gabriele Canzi Kylee Chang Andrew J. Hirning Joyce Lee Nick Von der Ahe 《Atmospheric environment (Oxford, England : 1994)》2010,44(7):900-908
The effect of sampling protocol on ambient air hydrocarbon mixing ratios was examined on eight sampling days in Los Angeles during 2007 and 2008. Four protocols, which were based on previously published multi-city urban hydrocarbon studies in the United States, were compared and differences were quantified. Whole air canister samples were collected and analyzed for nonmethane hydrocarbons (NMHCs). Differing sampling protocols resulted in large differences in mixing ratios, up to an order of magnitude, for certain NMHCs on the same sampling day. However, the magnitude of the variability between NMHC levels obtained by the four protocols was not consistent throughout the eight sampling days. It was found that sampling time, followed by sampling location, had the greatest influence on the magnitude of the mixing ratio. Ratios between hydrocarbons, often used in urban studies to gain information on emission sources, also varied depending on the protocol used. Comparison of absolute NMHC mixing ratios collected in urban environments using differing sampling protocols should be made with care. 相似文献
599.
X.X. Zhang P.J. Shi L.Y. Liu Y. Tang H.W. Cao X.N. Zhang X. Hu L.L. Guo Y.L. Lue Z.Q. Qu Z.J. Jia Y.Y. Yang 《Atmospheric environment (Oxford, England : 1994)》2010,44(13):1641-1648
Based on environmental monitoring data in 93 major cities and meteorological records at 398 weather stations in China from 1981 to 2007, total suspended particle (TSP) concentration, the intensity of dustfall, and sand and dust storm frequency (Fd) were analysed. During the past 27 years, the annual average TSP concentration (CTSP) in 93 cities was 402 μg m?3. Annual average CTSP decreased from the north to the south and from inland to the coast areas with a peak value of 628.8 μg m?3 in Lanzhou. In the 1980s, 1990s and 2000s, annual average CTSP was 628.7, 319.2, and 250.1 μg m?3, respectively. Annual average intensity of dustfall (Id) was 240.5 t km?2 a?1, decreased from northern to southern China and from inland to the coast areas with the maximum value of 717.2 t km?2 a?1 in Baotou. In the 1980s, 1990s and 2000s, annual average Id was 334.8, 220.9, 146 t km?2 a?1 respectively. Annual average Id in the Loess Plateau region was commonly higher than 200 t km?2 a?1. The annual average Fd decreased from arid regions in northwestern China to humid areas in southeastern China with two sand and sand storm centers existing in Xinjiang Taklamakan Desert and western Inner Mongolia. The annual average Fd in the 1980s, 1990s, 2000s was 16, 8, 6 days respectively, decreased steadily from 18 days in 1981–5 days in 2007. Annual average Id had a positive linear relation to annual average CTSP (R2 = 0.96). Annual average Fd had a positive relation with annual average CTSP (R2 = 0.97) as well as annual average Id (R2 = 0.94). TSP was the chief pollutant influencing Air Pollution Index (API) in northern China in spring and winter seasons. Sand and dust storm might be a major factor affecting the temporal variability and spatial distribution of TSP and dustfall in China. 相似文献
600.
James W. Rivers Philip S. Gipson Donald P. Althoff Jeffrey S. Pontius 《Environmental management》2010,45(2):203-216
Military training activities are known to impact individual species, yet our understanding of how such activities influence
animal communities is limited. In this study, we used long-term data in a case study approach to examine the extent to which
the local small landbird community differed between a site in northeast Kansas that experienced intensive disturbance from
military training activities (Ft. Riley Military Installation) and a similar, nearby site that experienced minimal human disturbance
(Konza Prairie Biological Station). In addition, we characterized how the regional pool of potential colonizers influenced
local community dynamics using Breeding Bird Survey data. From 1991 to 2001, most species of small terrestrial landbirds (73%)
recorded during breeding surveys were found at both sites and the mean annual richness at Ft. Riley (39.0 ± 2.86 [SD]) was
very similar to that of Konza Prairie (39.4 ± 2.01). Richness was maintained at relatively constant levels despite compositional
changes because colonizations compensated local extinctions at both sites. These dynamics were driven primarily by woodland
species that exhibited stochastic losses and gains and were present at a low local and regional abundance. Our results suggest
that military training activities may mimic natural disturbances for some species in this area because the small landbird
community did not differ markedly between sites with and sites without extensive human disturbance. Although our results suggest
that military training is not associated with large changes in the avian community, additional studies are needed to determine
if this pattern is found in other ecological communities. 相似文献