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981.
The present study investigated the photocatalytic activity of an S-doped TiO2 photocatalyst with regards to dimethyl sulfide degradation under visible-light irradiation, along with its deactivation and reactivation. The dimethyl sulfide conversion was between 85% and 93% for the lowest relative humidity range (10–20%) and close to 100% for the two higher relative humidity ranges (45–55% and 80–90%). The conversion was also close to 100% for the two lowest input concentrations (0.039 and 0.195 ppm), while it was between 91% and 96% at 3.9 ppm and between 85% and 90% at 7.9 ppm. In contrast to the input concentration dependences on conversion, the calculated degradation rates increased as input concentrations increased. The dimethyl sulfide conversion at low concentrations (≤0.39 ppm), which are associated with non-occupational inn occurring. However, catalyst deactivations were observed during the photocatalytic process whdoor air quality issues, was up to nearly 100% for long time periods (at least 603 h), without any significant catalyst deactivatioen higher concentrations (3.9 and 7.8 ppm) were used. The photocatalyst, reactivated by using two types of air (dried and humidified) under visible-light irradiation, did not regain all of its initial activities. Sulfate groups were qualitatively identified as the reaction products on the photocatalyst surface. In addition, gaseous byproducts, quantitatively determined, included dimethyl disulfide, methanol, and SO2. It is noteworthy that the peak concentration of dimethyl disulfide (0.79 ppm = 790 ppb), generated over the photocatalytic process with the highest dimethyl sulfide input concentration, exceeded the odor threshold value of 0.1–3.6 ppb for dimethyl disulfide. 相似文献
982.
983.
K.W. McDougall H. Wan C.R. Harris 《Journal of environmental science and health. Part. B》2013,48(2):293-301
Abstract The stability of dieldrin, aldrin, lindane, chlorpyrifos and prothiofos was determined in distilled water and in roof water from either galvanised or concrete tanks. Samples were stored in the dark at 23°C. Dieldrin and lindane were stable for the 36 week period. Aldrin dissipated rapidly with a half‐life of 4–5 weeks, with no dieldrin being formed. Chlorpyrifos and prothiofos also broke down, with half‐lives ranging 12–18 weeks and 11–14 weeks respectively. No significant effect of water type was found. For the purpose of domestic usage, an activated carbon filter would be essential otherwise all contaminated water would have to be disposed of safely. 相似文献
984.
公共管理与公众参与策略:于桥水库水质改善项目 总被引:3,自引:0,他引:3
环境问题是在人类的发展与资源的开发过程中产生的 ,是多种因素综合作用的结果 ,解决任何一个环境问题都将涉及到若干部门和公众 ,决不是一个部门所能完全胜任的。因此 ,采用公共管理与公众参与的模式解决环境问题 ,是改善环境质量的必然途径 ,是一个政府环境管理能力的综合体现。文章阐述了公共管理与公众参与的内涵、目标、目的、基本原则和实施程序等。 相似文献
985.
986.
987.
Dan Wan Jianhua Xu Jianbo Zhang Xuanchang Tong Jianxin Hu 《Atmospheric environment (Oxford, England : 1994)》2009,43(36):5822-5829
The halocarbons studied here are chemicals controlled in the 1987 Montreal Protocol on Substances that Deplete the Ozone Layer and its Amendments, which have both high ozone depleting potentials (ODPs) and high global warming potentials (GWPs). These halocarbons are mainly used for refrigeration, air-conditioning, foam blowing, tobacco expansion, aerosol propulsion, solvent cleaning, and fire fighting. China ratified the Montreal Protocol in 1991 and has been implementing the phase-out of halocarbons since then. In this paper, the emissions of halocarbons from China were estimated for 1995–2024 based on the historical consumption, the country program for complying with the Montreal Protocol, and the sector plans for phasing out halocarbons. The results show that China's compliance with the Montreal Protocol contributes greatly to both ozone protection and climate protection. 相似文献
988.
989.
In this study, the host-sensitivity and host-specificity of JC virus (JCV) and BK virus (BKV) polyomaviruses were evaluated by testing wastewater and fecal samples from nine host groups in Southeast Queensland, Australia. The JCV and BKV polyomaviruses were detected in 63 human wastewater samples collected from primary and secondary effluent, suggesting high sensitivity of these viruses in human wastewater. In the 81 animal wastewater and fecal samples tested, 80 were polymerase chain reaction (PCR) negative for the JCV and BKV markers. Only one sample (out of 81 animal wastewater and fecal samples) from pig wastewater was positive. Nonetheless, the overall host-specificity of these viruses to differentiate between human and animal wastewater and fecal samples was 0.99. To our knowledge, this is the first study in Australia that reports on the high specificity of JCV and BKV polyomaviruses. To evaluate the field application of these viral markers for detecting human fecal pollution, 20 environmental samples were collected from a coastal river. In the 20 samples tested, 15% (3/20) and 70% (14/20) samples exceeded the regulatory guidelines for Escherichia coli and enterococci levels for marine waters. In all, five (25%) samples were PCR positive for JCV and BKV, indicating the presence of human fecal pollution in the coastal river investigated. The results suggest that JCV and BKV detection using PCR could be a useful tool for identifying human-sourced fecal pollution in coastal waters. 相似文献
990.
Kaplan D Muñoz-Carpena R Wan Y Hedgepeth M Zheng F Roberts R Rossmanith R 《Journal of environmental quality》2010,39(5):1570-1584
Floodplain forests provide unique ecological structure and function, which are often degraded or lost when watershed hydrology is modified. Restoration of damaged ecosystems requires an understanding of surface water, groundwater, and vadose (unsaturated) zone hydrology in the floodplain. Soil moisture and porewater salinity are of particular importance for seed germination and seedling survival in systems affected by saltwater intrusion but are difficult to monitor and often overlooked. This study contributes to the understanding of floodplain hydrology in one of the last bald cypress [Taxodium distichum (L.) Rich.] floodplain swamps in southeast Florida. We investigated soil moisture and porewater salinity dynamics in the floodplain of the Loxahatchee River, where reduced freshwater flow has led to saltwater intrusion and a transition to salt-tolerant, mangrove-dominated communities. Twenty-four dielectric probes measuring soil moisture and porewater salinity every 30 min were installed along two transects-one in an upstream, freshwater location and one in a downstream tidal area. Complemented by surface water, groundwater, and meteorological data, these unique 4-yr datasets quantified the spatial variability and temporal dynamics of vadose zone hydrology. Results showed that soil moisture can be closely predicted based on river stage and topographic elevation (overall Nash-Sutcliffe coefficient of efficiency = 0.83). Porewater salinity rarely exceeded tolerance thresholds (0.3125 S m(-1)) for bald cypress upstream but did so in some downstream areas. This provided an explanation for observed vegetation changes that both surface water and groundwater salinity failed to explain. The results offer a methodological and analytical framework for floodplain monitoring in locations where restoration success depends on vadose zone hydrology and provide relationships for evaluating proposed restoration and management scenarios for the Loxahatchee River. 相似文献