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881.
酚类污染物解离态与非解离态光解特性及其速率常数的预测 总被引:3,自引:2,他引:1
以氙灯为光源模拟太阳光,通过研究不同pH条件下3种酚类污染物直接光解的过程,探讨了酚类污染物的解离对其光解规律的影响,并建立了解离态与非解离态酚类污染物光解速率常数的计算方法及预测模式.结果表明,随着pH从4.0增加到9.0,五氯酚的光解速率常数随之从25.30×10-4min-1增加到82.90×10-4min-1,而对硝基酚的光解速率常数相应从11.90×10-4min-1降低到了3.18×10-4min-1.苯酚的光解趋势与对硝基酚相似,当pH从4.0增加到11.0时,其光解速率常数依次从32.50×10-4min-1降低至13.40×10-4min-1.3种酚类化合物的光解总速率常数与解离度之间均满足幂函数变化规律.任意解离度条件下的解离态和非解离态光解速率常数,可根据幂函数的切线方程来确定.解离对酚类物质降解规律的影响主要是通过氧负离子的形成,改变苯环以及其他取代基团的活性而造成的.该研究结果为进一步了解天然水环境中酚类污染物的环境行为提供了理论参考. 相似文献
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高压静电场水处理技术是近几十年发展起来的、当今水处理领域中的一门高新技术。在此介绍了国内外高压静电场水处理机理和应用研究现状,并对今后高压静电场水处理技术研究提出几点展望。随着对高压静电场水处理机理研究的不断加强和完善。以及对高压静电水处理技术与其它水处理技术的联合水处理工艺研究的突破。高压静电场水处理技术有望成为一种极具应用前景的高效水处理技术。 相似文献
884.
谢凌江 《防灾科技学院学报》2010,12(3):110-113
灾难观是人类对灾害体系所持有的看法和态度,它随着人类社会的发展和进步处于不断的变化调整中,其整个过程构成文化的一个层面。本文从克拉克洪-斯托特柏克文化维度构架出发,选择"与环境的关系"和"人的本质"两个基点对比分析东西方文化灾难观的异同,对深刻理解各种文化在解释和应对灾难过程中的共性和相对性有着重要意义。 相似文献
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TGM measurements on board ships have proved to provide valuable complementary information to measurements by a ground based monitoring network. During the third China Arctic Research Expedition (from July 11 to September 24, 2008), TGM concentrations over the marine boundary layer along the cruise path were in-situ measured using an automatic mercury vapor analyzer. Here we firstly reported the results in Japan Sea, North Western Pacific Ocean and Bering Sea, where there are rare reports. The value ranged between 0.30 and 6.02 ng/m3 with an average of (1.52 ± 0.68) ng/m3, being slightly lower than the background value of Northern Hemisphere (1.7 ng/m3). Notably TGM showed considerably spatial and temporal variation. Geographically, the average value of TGM in Bering Sea was higher than those observed in Japan Sea and North Western Pacific Ocean. In the north of Japan Sea TGM levels were found to be lower than 0.5 ng/m3 during forward cruise and displayed obviously diurnal cycle, indicating potential oxidation of gaseous mercury in the atmosphere. The pronounced episode was recorded as well. Enhanced levels of TGM were observed in the coastal regions of southern Japan Sea during backward cruise due primarily to air masses transported from the adjacent mainland reflecting the contribution from anthropogenic sources. When ship returned back and passed through Kamchatka Peninsula TGM increased by the potential contamination from volcano emissions. 相似文献
888.
A numerical study of Reciprocating Superadiabatic Combustion of Premixed gases in porous media (hereafter, referred to as RSCP) is performed. In this system the transient combustion of methane-air mixture is stabilized in a porous media combustor by periodically switching flow directions. The mass, momentum, energy and species conservation equations are solved using a two-dimensional control volume method. Local thermal non-equilibrium between the gas and the solid phases is considered by solving separate energy equations for the two phases and coupling them through a convective heat transfer coefficient. The porous media is assumed to emit, absorb and isotropically scatter radiation. The influences of the dominating operating parameters, such as filtration velocity, equivalence ratio and half cycle on the temperature profile, heat release rate, radiant flux, radiant efficiency and combustion efficiency are discussed. The results show that coupling calculating of flow field, combustion reaction and volume radiation of the optically thick media is successively achieved and heat radiation plays an important role in the overall performance of the burner. The temperature profile inside the RSCP combustor has a typical trapezoidal shape and the profile of radiation flux is similar to sinusoidal shape. Compared with the conventional premixed combustion in porous medium, combustion behavior in RSCP combustor is superior, such as better thermal structure and higher radiation efficiency and combustion efficiency. 相似文献
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890.
通过试验证明,一定浓度的KCl溶液滴加到去离子水中,对去除水中微量的F离子有良好效果。该方法简单易行,十分适合氟离子选择电极法测定中无氟水的制备。 相似文献