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为探究地表水体与沉积物中酚类化合物的污染分布特征和生态风险,选择天津市3个水源地与6条主要河流,采集了26个地表水样与6个沉积物样品,利用固相萃取与超声萃取、高效液相色谱-串联质谱法(HPLC-MS/MS)测定了水样及沉积物中1-萘酚(1-naphthol)、壬基酚(nonylphenol, NP)、双酚A(bisphenol A, BPA)、2-苯基苯酚(biphenyl-2-ol)、3,4-二氯酚(3,4-dichlorophenol)、四溴双酚A(tetrabromobisphenol A, TBBPA)和对叔丁基苯酚(p-tert-butylphenol, PTBP)等7种高关注酚类化合物的浓度水平,并应用物种敏感性分布(species sensitivity distribution, SSD)法和熵值法(ecological risk quotient, RQ)评估7种酚类化合物水环境和沉积物的生态风险。结果表明,地表水样中7种酚类化合物均全部检出;其中壬基酚的检出浓度最高,其次为四溴双酚A、对叔丁基苯酚、1-萘酚、2-苯基苯酚、3,4-二氯酚和双酚A。沉积物中酚类化合物的污染分布规律与水样相似,除双酚A外的目标物全部检出。其中,壬基酚浓度比其他物质浓度高2个数量级。风险评估结果显示,壬基酚对水环境与沉积物存在不可接受的风险;而四溴双酚A、对叔丁基苯酚、1-萘酚、2-苯基苯酚、3,4-二氯酚和双酚A则对环境具有较低风险或者存在一定的风险。 相似文献
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Xinjie Wang Yang Li Jian Zhao Hong Yao Siqi Chu Zimu Song Zongxian He Wen Zhang 《Frontiers of Environmental Science & Engineering》2020,14(4):56
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宁夏电网目前已接入3回直流,其中第1回直流为±660 kV接入,容量为4 GW;第2回直流为±800 kV,容量为8 GW;第3回直流为±800 kV,容量为10 GW,并正式形成了送端直流群。随着特高压直流的接入,宁夏电网发生直流故障的次数逐渐增多。针对第2回直流某次典型单极连续3次闭锁故障,详细介绍了事故发生的过程和故障前后宁夏电网运行方式及系统动态特性的变化情况。利用PSASP程序建立宁夏电网仿真模型,还原了故障前电网运行方式,并仿真再现了故障后的电网动态过程。通过仿真与实测结果的对比,进一步明确了直流故障期间电网特性的变化情况,同时验证了仿真模型的准确性。 相似文献
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Estelle Lefrançois Laure Apothéloz-Perret-Gentil Philippe Blancher Samuel Botreau Cécile Chardon Laura Crepin Tristan Cordier Arielle Cordonier Isabelle Domaizon Benoit J. D. Ferrari Julie Guéguen Jean-Christophe Hustache Louis Jacas Stephan Jacquet Sonia Lacroix Anne-Laurence Mazenq Alina Pawlowska Pascal Perney Jan Pawlowski Frédéric Rimet Jean-François Rubin Dominique Trevisan Régis Vivien Agnès Bouchez 《Environmental science and pollution research international》2018,25(34):33858-33866
The effectiveness of environmental protection measures is based on the early identification and diagnosis of anthropogenic pressures. Similarly, restoration actions require precise monitoring of changes in the ecological quality of ecosystems, in order to highlight their effectiveness. Monitoring the ecological quality relies on bioindicators, which are organisms revealing the pressures exerted on the environment through the composition of their communities. Their implementation, based on the morphological identification of species, is expensive because it requires time and experts in taxonomy. Recent genomic tools should provide access to reliable and high-throughput environmental monitoring by directly inferring the composition of bioindicators’ communities from their DNA (metabarcoding). The French-Swiss program SYNAQUA (INTERREG France-Switzerland 2017–2019) proposes to use and validate the tools of environmental genomic for biomonitoring and aims ultimately at their implementation in the regulatory bio-surveillance. SYNAQUA will test the metabarcoding approach focusing on two bioindicators, diatoms, and aquatic oligochaetes, which are used in freshwater biomonitoring in France and Switzerland. To go towards the renewal of current biomonitoring practices, SYNAQUA will (1) bring together different actors: scientists, environmental managers, consulting firms, and biotechnological companies, (2) apply this approach on a large scale to demonstrate its relevance, (3) propose robust and reliable tools, and (4) raise public awareness and train the various actors likely to use these new tools. Biomonitoring approaches based on such environmental genomic tools should address the European need for reliable, higher-throughput monitoring to improve the protection of aquatic environments under multiple pressures, guide their restoration, and follow their evolution. 相似文献
66.
Charlotte R. Dromard Mathilde Guéné Yolande Bouchon-Navaro Soazig Lemoine Sébastien Cordonnier Claude Bouchon 《Environmental science and pollution research international》2018,25(15):14294-14301
Chlordecone is an organochlorine pesticide, used in the Lesser Antilles from 1972 to 1993 to fight against a banana weevil. That molecule is very persistent in the natural environment and ends up in the sea with runoff waters. The objective of the present study is to evaluate the level of contamination in several trophic groups of marine animals according to their distance from the source of pollution. Samples of suspended matter, macroalgae, herbivorous fishes, detrivorous crustaceans, zooplanktivorous fishes, first- and second-order of carnivorous fishes, and piscivorous fishes have been collected in two sites, located downstream the contaminated sites (Goyave and Petit-Bourg), in three marine habitats (coastal mangroves, seagrass beds located 1.5 km from the shoreline, and coral reefs at 3 km offshore). Animals collected in mangroves were the most contaminated (mean concentrations 193 μg kg?1 in Goyave and 213 μg kg?1 in Petit-Bourg). Samples from seagrass beds presented intermediate concentrations of chlordecone (85 μg kg?1 in Goyave and 107 μg kg?1 in Petit-Bourg). Finally, samples from coral reefs were the less contaminated (71 μg kg?1 in Goyave and 74 μg kg?1 in Petit-Bourg). Reef samples, collected 3 km offshore, were two to three times less contaminated than those collected in mangroves. 相似文献
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Liang Peng Yanqing Ren Jidong Gu Pufeng Qin Qingru Zeng Jihai Shao Ming Lei Liyuan Chai 《Environmental science and pollution research international》2014,21(12):7631-7640
Novel magnetic carbonaceous bio-char was hydrothermal prepared from microalgae under different loadings of iron and its structures and surface chemistry were characterized with Fourier transform infrared (FTIR), X-ray photoelectron spectroscopy (XPS), scanning electron microscopy (SEM), and nitrogen adsorption-desorption isotherm (BET). The morphology of bio-char changed from sheet to particle as iron loading increased and its surface area also increased. When 3.0 g of dried microalgae and 6.0 mmol iron salt ((NH4)2SO4·FeSO4·6H2O) were mixed and treated, the obtained bio-char possessing the highest amount of oxygen-containing functional groups resulted in the best adsorption performance on tetracycline (TC). This adsorption process was fitted to Langmuir adsorption isotherm and the maximum adsorption capacity was 95.86 mg/g, which is higher than other bio-char reported. The iron loading contributed to the higher adsorption capacity of bio-char, which may be due to three factors, the high surface area, more hydrogen bonding, and bridging effects of the structural Fe for TC. Our data suggest that bio-char may have more important role in stabilization of pollutants in the environment. 相似文献
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