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Occurrence and removal of endocrine-disrupting chemicals in wastewater treatment plants in the Three Gorges Reservoir area, Chongqing, China 总被引:1,自引:0,他引:1
Ye X Guo X Cui X Zhang X Zhang H Wang MK Qiu L Chen S 《Journal of environmental monitoring : JEM》2012,14(8):2204-2211
Concentrations of six endocrine-disrupting compounds (EDCs), bisphenol A (BPA), estrone (E(1)), 17β-estradiol (E(2)), estriol (E(3)), 17α-ethynylestradiol (EE(2)) and diethylstilbestrol (DES), were assessed in influents, effluents and excess sludge in ten municipal wastewater treatment plants (WWTPs) in the Three Gorges Reservoir (TGR) area, Chongqing, China. Three types of activated sludge treatment processes, oxidation ditch (OD), reversed anaerobic-anoxic-oxic (rA(2)/O) technology and sequential batch reactor (SBR), were used in the surveyed WWTPs. These WWTPs were all combined landfill leachate-sewage treatment plants. All analytes were extracted by solid-phase extraction (SPE) in the dissolved phase and by accelerated solvent-based extraction (ASE) in sludge. Gas chromatography-mass spectrometry (GC-MS) was employed for the analysis of EDCs. Among these EDCs, BPA was the most frequently detected and abundant compound (100.0-10566.7 ng L(-1), 15.5-1210.7 ng L(-1) and 85.0-2470.4 ng g(-1) with respect to the influents, effluents and excess sludge samples). The greatest levels of steroidal estrogens in municipal influents were observed in E(3) which were all >100 ng L(-1), followed by E(1) (42.2-110.7 ng L(-1)) and E(2) (7.4-32.7 ng L(-1)), and in the effluents and sludge were E(1) > E(3) > E(2) which were all <31 ng L(-1) and 105 ng g(-1), respectively. Regarding synthetic estrogens, EE(2) was frequently detected in the influents, occurring below 50 ng L(-1), while DES was not detected at all. A high correlation coefficient was observed between the leachate-sludge ratio and concentrations of influent EDCs, and it was statistically significant (i.e., R > 0.65, P < 0.05), but removal efficiency of the EDCs did not show significant differences with OD, rA(2)/O and SBR processes. Furthermore, modification of treatment technology as well as operational parameters, such as hydraulic retention time (HRT), sludge retention time (SRT) and disinfection process (DP), were recommended to further eliminate the residual EDCs. 相似文献
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植物源杀虫剂川楝素对环境生物安全性评价 总被引:3,自引:0,他引:3
评价农药对环境中非靶标生物的毒性是新农药开发应用的重要环节.依据国家环境保护局"化学农药环境安全评价试验准则",测定了78%川楝素原粉和0.5%川楝素乳油对生态环境中非靶标生物的毒性,并进行了安全性评价.结果表明,川楝素原粉对鹌鹑、家蚕、蜜蜂、蚯蚓、瓢虫、蝌蚪等非靶标生物均为低毒;川楝素乳油对家蚕、蜜蜂、蚯蚓、瓢虫等均为低毒,对家蚕的生长发育具有一定的影响,对鹌鹑中毒,对蝌蚪高毒.可见,植物源杀虫剂川楝素对环境非靶标生物毒性低、较为安全,但在水田及桑园应慎用0.5%川楝素乳油. 相似文献
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城市供水水库的微塑料污染近年来受到广泛关注.密云水库作为北京市重要的饮用水水源地,有必要对其微塑料污染现状进行全面调查.本研究以密云水库的表层水、沉积物和鱼类为研究对象,调查了微塑料的丰度、分布和组成特征,揭示了微塑料的来源及生态风险.结果表明表层水,沉积物和鱼类肠道中微塑料的平均丰度分别为(6.83±1.87) n·L-1,(408±141) n·kg-1和(3.93±2.80) n·ind-1.微塑料在表层水和沉积物中的空间分布归因于水流方向、人类活动和水坝阻挡.鱼类肠道中微塑料丰度分布差异与栖息地和摄食习惯不同有关,水体上层的滤食性鱼类微塑料污染最严重.在所有样本中,纤维状、≤0.5 mm及透明的微塑料占比较高,聚对苯二甲酸乙二醇酯(47.64%)/聚丙烯(20.03%)和聚乙烯(18.35%)为主要聚合物类型.对微塑料污染特征分析,指出密云水库微塑料的主要来源为人类日常生活、渔业活动和农业生产活动,途径为大气沉降和降雨径流.利用风险指数和污染负荷指数对表层水和沉积物的微塑料污染进行评估,结果显示整体风险较低.本研... 相似文献