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41.
Polychlorinated dibenzo-p-dioxin, polychlorinated dibenzofuran and dioxin-like polychlorinated biphenyl concentrations in human liver, kidney, fat, blood, muscle, richly perfused tissue (brain, lung etc.) and skin were simulated to assess the health risk for Japanese fetuses. A 40-year time course of dioxin accumulation via food ingestion was simulated using a physiologically based pharmacokinetic (PBPK) model. In richly perfused tissue, the concentration estimated by the PBPK model showed better agreement with measured concentrations than that calculated by the one-compartment model. Fetal dioxin concentration was simulated based on the assumption that the fetal concentration was almost equal to the concentration in the mother's richly perfused tissue. To assess the reproductive risk, the estimated concentration in human fetus was compared with that in rat fetus in which reproductive function showed signs of alteration by 2,3,7,8-TCDD in previous reports [Toxicol. Appl. Pharmacol. 114 (1992) 118; 146 (1997) 11; Toxicol. Sci. 53 (2000) 411; 57 (2000) 275]. The present daily intake of 2,3,7,8-TCDD is approximately 1/50 of the amount that leads to possible reproductive toxicity in the next generation. However, when 29 kinds of dioxin congeners are considered, the present level is 1/5 of the hazardous levels. For species extrapolation of dioxin risk, further study on tissue concentration versus toxicity is required. 相似文献
42.
Specific accumulation of polychlorinated biphenyls and organochlorine pesticides in Japanese common squid as a bioindicator 总被引:4,自引:0,他引:4
Ueno D Inoue S Ikeda K Tanaka H Yamada H Tanabe S 《Environmental pollution (Barking, Essex : 1987)》2003,125(2):227-235
Organochlorines (OCs) representing Persistent Organic Pollutants (POPs) such as PCBs (polychlorinated biphenyls), DDTs (DDT and its metabolites), CHLs (chlordane compounds), HCHs (hexachlorocyclohexane isomers) and HCB (hexachlorobenzene) were determined in the liver of Japanese common squid (Todarodes pacificus) collected from the waters around Japan (Japan Sea and western North Pacific Ocean). Among OCs concentrations, PCBs (upto 5600 ng/g lipid wt.) were the highest, and those of other OCs were in the order of DDT> CHLs > HCHs > HCB. Studies on growth trend and seasonal variation of OCs in this species suggest a rapid reflection of the pollution levels in seawater where and when they were collected, regardless of body-length and time of collection. These results indicate that Japanese common squid is a suitable bioindicator for monitoring OCs pollution in waters around Japan. With regard to the geographical distribution of OCs in this species collected from waters around Japan, OCs concentrations in specimens from Japan Sea were higher than those from the Pacific Ocean. This result might reflect some existing of local pollution sources of OCs around Japan Sea, and slower water exchange between Japan Sea and open ocean. 相似文献
43.
Dependence of mechanochemically induced decomposition of mono-chlorobiphenyl on the occurrence of radicals 总被引:1,自引:0,他引:1
Mechanochemically induced dechlorination of mono-chlorobiphenyl (BP-Cl) on the surfaces of metal oxides was compared with that on metal hydroxides, using the three metals of Mg, Al, and La as examples. The metal oxides, such as gamma-alumina (gamma-Al2O3), magnesium oxide (MgO) and lanthanum oxide (La2O3) showed an efficient ability to dechlorinate the BP-Cl; however, BP-Cl remained in the ground samples when the hydroxides were used. From the product analysis using gas chromatography/mass spectrometry (GC/MS) and electron spin resonance (ESR) measurements, it was confirmed that the charge transfer from the O2- site on the surface of the oxide additives due to the intense grinding has plays a significant role in the decomposition of the chlorinated compound. Based on the observed dependence of the dechlorination on the radical occurrence, some practical methods were proposed to improve the destruction efficiency of the chlorinated organic compounds. 相似文献
44.
The tissue-blood partition coefficients for a physiologically based pharmacokinetic (PBPK) model were determined, and the concentrations of 17 congeners of polychlorinated dibenzo-p-dioxins and polychlorinated dibenzofurans (PCDD/Fs) in tissues in Japanese people were estimated using the model. According to the PBPK model established by Lawrence and Gobas [Chemosphere 35 (1997) 427-452], we assumed a steady-state fugacity model for Japanese people in general, and set the route of PCDD/Fs exposure only from food intake. The required partition coefficients for liver, kidney, adipose, muscle, skin, bile, gut and viscera (richly perfused tissue) were calculated using available autopsy data from eight Japanese men and women who were not accidentally exposed to PCDD/Fs. For validation of the partition coefficients, estimated PCDD/F concentrations in liver, kidney, fat, blood and muscle using the model were compared to other two sets of measured concentration data in Japanese tissues. Good agreement was obtained between estimated data and measured data, and most of the measured data were within the simulated concentration range in liver, kidney, blood and muscle. From these results, our model and calculated partition coefficients seem applicable for the estimation of congener-specific concentrations in human tissues. 相似文献
45.
Subramanian AN Tanabe S Tanaka H Hidaka H Tatsukawa R 《Environmental pollution (Barking, Essex : 1987)》1987,43(1):39-46
The gain and loss rates and the biological half-life of polychlorinated biphenyls (PCBs) and p,p'-DDE in wild birds were calculated using the values on burdens of these compounds in the bodies of adelie penguins in a previous report (Subramanian et al., 1986). The daily loss rate of PCBs (0.26%) was found to be higher than DDT compounds (0.12%) resulting in the longer biological half-life of the latter compounds (580 days) than PCBs (270 days). Hence, once DDT compounds are absorbed they are more persistent in the organisms' bodies due to their high lipophilicity and comparatively less metabolisable nature than PCBs. 相似文献
46.
Shunitz Tanaka Masayuki Kawai Yosuke Nakata Motoki Terashima Hideki Kuramitz Masami Fukushima 《毒物与环境化学》2013,95(4-6):95-102
The photo-Fenton reactions, which could yield hydroxyl radicals via the catalytic degradation of H2O2 by Fe(II), were focused as one of the abiotic degradation processes of bisphenol A (BPA) in surface waters. At pH 6, in the presence of H2O2 only, 32% of BPA was degraded after 120?min of irradiation. However, 97% of BPA was degraded in the presence of both H2O2 and Fe(II). Without light irradiation, no BPA degradation was observed even in the presence of Fe(II) and H2O2. These results show that photo-Fenton processes are effective in the natural attenuation of BPA in surface water. In addition, the presence of humic acids (HAs), which were of more aliphatic nature, resulted in enhancing BPA degradation via the photo-Fenton processes. Therefore, HAs can be one of the important factors in enhancing the degradation of BPA in surface water via the photo-Fenton processes. 相似文献
47.
Taro Miyoshi Thanh Phong Nguyen Terumi Tsumuraya Hiromu Tanaka Toru Morita Hiroki Itokawa Toshikazu Hashimoto 《Frontiers of Environmental Science & Engineering》2018,12(3):1
48.
Ishimori Hiroyuki Asada Shunsuke Sakaguchi Tomoyuki Sakaguchi Yoshiyuki 《Journal of Material Cycles and Waste Management》2022,24(4):1237-1250
Journal of Material Cycles and Waste Management - This paper presents whether some minerals in waste concrete and ferronickel slag are available for hydroponics instead of commercial fertilizer.... 相似文献
49.
Environmental Fluid Mechanics - The principle theme of this study is to introduce a novel countermeasure to reduce the energy of the overflowing floodwater by utilization of a water cushion. For... 相似文献
50.
Geographical variations in the trophic ecology of Japanese anchovy, Engraulis
japonicus, inferred from carbon and nitrogen stable isotope ratios 总被引:1,自引:0,他引:1
Carbon and nitrogen stable isotope ratios of Japanese anchovy (Engraulis japonicus) and their stomach contents were examined and compared among various regions around Japan. Geographical variations in the
isotope ratios were found between inshore and Pacific offshore regions. While most of the anchovy samples had isotope ratios
around −17.6‰ for δ13C and 10.0‰ for δ15N as median values, higher (more enriched) isotope values were found in the anchovy sampled from inshore regions. On the contrary,
lower (more depleted) values were found mostly in the anchovy from the Pacific offshore region including the Kuroshio Extension
and Kuroshio-Oyashio transition zones. Higher carbon isotope ratios in the inshore regions may reflect a carbon source from
benthic primary producers in addition to phytoplankton possibly through the consumption of the larvae of benthic organisms
such as bivalves or decapods, which were found in the stomach contents of the inshore anchovy. Variations in the nitrogen
isotope ratio may reflect not only differences in the trophic level of prey species, but also variations in the baseline level
of food webs. Stable isotope ratios are potentially a useful tool for understanding the stock/population structure and migration
of anchovy. The present findings indicate the potential importance of the “inshore–offshore” variations in the biology of
Japanese anchovy populations in the northwestern Pacific waters. 相似文献