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111.
Thermogravimetric analysis and kinetic study on pyrolysis of representative medical waste composition 总被引:1,自引:0,他引:1
To obtain detailed information on the pyrolysis characteristics, a thermogravimetric study on the pyrolysis of 14 typical medical waste compositions was carried out in thermogravimetric analysis (TGA) equipment using dynamic techniques in a stream of N(2). An index representing pyrolysis reactivity of waste was presented. Kinetic parameters were obtained by Coats-Redfern method and used to model the TG curve. The results showed that: (a) Plastic, protein, cellulosic material, synthetic fibre, and rubber entered pyrolysis process in succession. (b) There was one decomposition stage in the pyrolysis of one-off medical glove, operating glove, cellulosic waste, absorbable catgut suture and adhesive plaster, while other components had two obvious weight loss stages. (c) The obtained apparent activation energy for second stage pyrolysis was comparably higher than that for first stage. (d) Each stage was controlled by only one kinetic mechanism, in which kinetic parameters were constant. (e) The degradation kinetics of medical waste may be affected by special physical and chemical treatment in the product manufacturing process. (f) Among 13 waste samples, the pyrolysis index of cellulosic matter was the highest, which indicated cellulosic matter had strong pyrolysis reactivity. (g) With increasing heating rate, TG curve and DTG peak shifted to high temperatures and main reaction interval of the sample became longer. 相似文献
112.
Geotechnical and leaching properties of flowable fill incorporating waste foundry sand 总被引:1,自引:0,他引:1
Waste foundry sand (WFS) can be converted into flowable fill for geotechnical applications. In this study, WFS samples were obtained from 17 independent metal casting facilities with different casting processes, thus representing a good range of WFS properties. The laboratory studies include physical, geotechnical and leaching properties of flowable fills consisting of WFS, cement, and fly ash mixed to different water contents. The main properties measured include WFS physical properties (density, particle gradation, grain shape, and fine content), WFS flowable fill geotechnical properties (unconfined compressive strength, hydraulic conductivity, setting time, and bleeding), and the fill's leaching properties (heavy metals and organics in the bleed water and the leachate extracted from hardened WFS flowable fills). The test results indicate that in terms of the physical properties, most of the data fall within narrow ranges, although data from the copper/aluminum-based WFS samples might fall beyond the ranges. Geotechnical properties of WFS flowable fills in both fresh and hardened phases were verified conforming to the features of specified flowable fills. Material leaching analyses indicate that the toxicity of WFS flowable fills is below regulated criteria. A mix formulation range originated from this study is proposed for the design of WFS made flowable fill. 相似文献
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116.
Tao Y Yao S Xue B Deng J Wang X Feng M Hu W 《Journal of environmental monitoring : JEM》2010,12(12):2282-2289
Sources, partitioning and toxicological risk of 15 priority polycyclic aromatic hydrocarbons (PAHs) in surface sediments from drinking water sources of Taihu Lake, with an area of 2428 km(2) located in the most developed and populated area of China, were studied, and the results were compared with those in other lakes of China and the USA. Concentrations of the 15 PAHs in sediments ranged from 436.6 to 1334.9 ng g(-1) (dw). Gasoline combustion, coal combustion, diesel combustion from shipping and spillage of petroleum were apportioned to be the main sources of PAHs in this area by principal component analysis, which contributed 35.19%, 26.43%, 25.41% and 12.97% to the PAH sources estimated by further multiple linear regression. Levels of PAHs in sediments were negatively correlated with contents of clay and fine silt (<16 μm), while positively with contents of medium silt, coarse silt and sand (>16 μm). Humin with size larger than 16 μm contained the largest part of the burden of PAHs in sediments, but the specific partitioning domain (bound humic acid, lipid or insoluble residue) depended on properties of organic matter reflected by optical absorbance at 465 and 665 nm. Total toxic benzo[a]pyrene equivalent (TEQ(carc)) of the carcinogenic PAHs in sediments varied from 31.8 to 209.3 ngTEQ(carc) g(-1). Benzo[a]pyrene and dibenzo[a,h]anthracene contributed 45.36 and 25.31% to total TEQ(carc), posing high toxicological risk to this area. 相似文献
117.
Spatial and seasonal distribution of nitrogen in marsh soils of a typical floodplain wetland in Northeast China 总被引:3,自引:0,他引:3
Bai J Wang Q Deng W Gao H Tao W Xiao R 《Environmental monitoring and assessment》2012,184(3):1253-1263
Horizontal and profile distributions of nitrogen in marsh soils in different seasons were studied in a typical site within
the Erbaifangzi wetland in Northeast China. Results showed that there was higher spatial heterogeneity for nitrate nitrogen
(NO3--_{3}^{-}-N) and ammonium nitrogen (NH4+_{4}^{+}–N), as well as available nitrogen (AN), in surface soils in July compared to that in September. Relative to July, the mean
nitrogen contents in surface soils were slightly higher in September; however, in November, soils contained significantly
lower NO3--_{3}^{-}-N and NH4+_{4}^{+}–N, higher AN, organic nitrogen (Org-N), and total nitrogen (TN). Except for mineral nitrogen, no significant differences
were observed between Org-N and TN contents in September and November. Nitrogen contents generally declined exponentially
with depth along soil profiles in three sampling dates (July, September, and November), except for a significant accumulation
peak of NO3--_{3}^{-}-N at the 20–30 cm depth in September. However, NH4+_{4}^{+}–N contents showed a vertical alternation of “increasing and decreasing” in both July and September, while nearly kept constant
with depth in November. The depth ranking of nitrogen showed the shallowest distribution for AN, followed by Org-N and TN,
while deeper distributions for NO3--_{3}^{-}-N and NH4+_{4}^{+}–N. TN, Org-N, and AN were significantly correlated with soil organic matter and total phosphorus. Soil pH values were significantly
correlated with TN and AN contents in surface soils. Clay contents showed significant correlations with nitrogen contents
except for NO3--_{3}^{-}-N in surface soils and NH4+_{4}^{+}–N in profile soils. However, soil moisture was not significantly correlated with nitrogen contents among all soil samples. 相似文献
118.
Yan Yan Peng Shan Chenxing Wang Yuan Quan Di Wu Chunli Zhao Gang Wu Hongbing Deng 《Environmental monitoring and assessment》2017,189(4):191
Sustainable urban development focuses on enhancing urban well-being, while also balancing the demands of urban social and economic development, natural resource consumption, and environmental pollution. This work used general data envelopment analysis to assess the urban sustainability efficiency (USE) and sustainability potential (SP) in Lanzhou and Xiamen, two cities that are characteristic of urban areas in western and eastern China. The assessment indicator system included important natural and urban welfare factors as input and output indices, respectively. The results showed that overall urban sustainability efficiency increased in Lanzhou and Xiamen from 1985 to 2010, but that the sustainability of natural resources clearly decreased. The urban sustainability efficiency of Xiamen was higher than that of Lanzhou, and the sustainability potential of Xiamen was lower than that of Lanzhou; this indicates that Xiamen performed better in terms of urban sustainable development. The urban sustainability efficiency in Xiamen has increased with increasing urban population, and the rate and scale of economic development have been higher than in Lanzhou. The assessment and analysis performed in this study show that cities with different natural resources and development characteristics have different forms, patterns, and trajectories of sustainable development. 相似文献
119.
回顾了原子吸收光谱分析在我国环境、医学卫生和食品分析方面的应用概况。 相似文献
120.
Seasonal variations of monocarbonyl and dicarbonyl in urban and sub-urban sites of Xi’an,China 总被引:1,自引:0,他引:1
K. F. Ho Steven Sai Hang Ho W. T. Dai J. J. Cao Ru-Jin Huang Linwei Tian W. J. Deng 《Environmental monitoring and assessment》2014,186(5):2835-2849
Seventeen airborne carbonyls including monocarbonyls and dicarbonyls were determined in urban and sub-urban sites of Xi’an, China in three seasons in 2010. In winter, acetone was the most abundant carbonyl in the urban site due to usage of organic solvents in constructions and laboratories and its slower atmospheric removal mechanisms by photolysis and reaction with hydroxyl radical than those of formaldehyde and acetaldehyde. In the sub-urban site, acetaldehyde was the most abundant carbonyl, followed by formaldehyde and acetone. During summer, however, formaldehyde was the most dominant carbonyl in both sites. The photooxidations of a wide range of volatile organic compounds (VOCs) yielded much more formaldehyde than other carbonyls under high solar radiation and temperature. In the urban site, the average concentrations of dicarbonyls (i.e., glyoxal and methyglyoxal) in spring and summer were higher than that in winter. Transformation of aromatic VOCs emitted from fuel evaporation leads to the formation of 1,2-dicarbonyls. A reverse trend was observed in sub-urban sites, as explained by the relatively low abundances and accumulations of VOC precursors in the rural atmosphere during warm seasons. Moreover, cumulative cancer risk based on measured outdoor carbonyls (formaldehyde and acetaldehyde) in Xi’an Jiaotong University and Heihe was estimated (8.82?×?10?5 and 4.96?×?10?5, respectively). This study provides a clear map on the abundances of carbonyls and their source interpretation in the largest and the most economic city in Northwestern China. 相似文献