Atmosphericmixing ratios of carbonyl sulfide (COS) in Beijingwere intensivelymeasured from March 2011 to June 2013. COS mixing ratios exhibited distinct seasonal variation, with a maximumaverage value of 849 ± 477 pptv in winter and a minimal value of 372 ± 115 pptv in summer. The seasonal variation of COS was mainly ascribed to the combined effects of vegetation uptake and anthropogenic emissions. Two types of significant linear correlations (R2 > 0.66) were found between COS and CO during the periods from May to June and from October to March, with slopes (ΔCOS/ΔCO) of 0.72 and 0.14 pptv/ppbv, respectively. Based on the emission ratios of COS/CO from various sources, the dominant anthropogenic sources of COS in Beijing were found to be vehicle tire wear in summer and coal burning in winter. The total anthropogenic emission of COS in Beijing was roughly estimated as 0.53 ± 0.02 Gg/year based on the local CO emission inventory and the ΔCOS/ΔCO ratios. 相似文献
A sound scientific understanding of the factors affecting the environment is essential to guarantee the sustainable development of the world's economic and societal activities.Many environmental issues,such as air quality and climate change are intimately linked to atmospheric chemistry and physics,therefore research in these areas is of tremendous importance.Both anthropogenic and biogenic emissions contribute greatly to the chemical composition of the atmosphere.Even though the atmosphere is a self-cleaning system through its photochemically-driven reactions,the hazardous direct impacts of primary and secondary pollutants on human health and ecosystems are observable and have been evidenced on different scales from local to global (e.g.ozone hole,climate change,air quality…).The chemical processing of the species present in the atmosphere is one of the most important players in driving the evolution of the atmosphere. 相似文献
The effects of γ-irradiation pretreatment on anaerobic digestibility of sewage sludge was investigated in this paper. Parameters like solid components, soluble components, and biogas production of anaerobic digestion experiment for sewage sludge were measured. The values of these parameters were compared before and after γ-irradiation pretreatment. Total solid (TS), volatile solid (VS), suspended solid (SS), volatile suspended solid (VSS), and average floc size of samples decreased after γ-irradiation treatment. Besides, floc size distribution of sewage sludge shifted from 80–100 μm to 0–40 μm after γ-irradiation treatment at the doses from 0 to 30 kGy, which indicated the disintegration of sewage sludge. Moreover, microbe cells of sewage sludge were ruptured by γ-irradiation treatment, which resulted in the release of cytoplasm and increase of soluble chemical oxygen demand (SCOD). Both sludge disintegration and microbe cells rupture enhanced the subsequent anaerobic digestion process, which was demonstrated by the increase of accumulated biogas production. Compared with digesters fed with none irradiated sludge, the accumulated biogas production increased 44, 98, and 178 mL for digesters fed sludge irradiated at 2.48, 6.51, and 11.24 kGy, respectively. The results indicated that γ-irradiation pretreatment could effectively enhance anaerobic digestibility of sewage sludge, and correspondingly, could accelerate hydrolysis process, shorten sludge retention time of sludge anaerobic digestion process. 相似文献
Environmental Science and Pollution Research - Several studies have revealed a relationship between short-term exposure to air pollution and the exacerbation of certain skin conditions. This study... 相似文献
This study uses an environmental extension of the Leontief price model to analyse various tax rates on the carbon dioxide (CO2) and other greenhouse gases (GHGs) emissions that are generated by the most polluting sectors of the Chilean economy. By using this methodology, it is possible to obtain a counterfactual scenario for the prices, levels of production and emissions of each economic sector, as well as, for tax collection, consumer spending and the consumer price index. This analysis is important because Chile is internationally committed to reducing its emissions by 30% by 2030. According to the results, to meet the target CO2 emissions only using tax policies, tax should be approximately 20 times higher than their current levels in the electricity sector. Alternatively, a lower tax of US $30/ton of CO2 and other GHGs applied to all sectors of the economy could reduce CO2 and other GHGs emissions by up to 25.7% with less of a negative impact on the economy. 相似文献
Viscosity remedial technology, which uses a water-soluble polymer mixed with remedial fluids, has been introduced in recent years to improve the removal efficacy of perchloroethylene/tetrachloroethylene (PCE) by improving oxidant coverage (i.e. sweep efficiency). Xanthan gum and hydrolysed polyacrylamide (HPAM) are relatively stable with time and temperature and possess salt and oxidation resistance, indicating that they may be good flooding agents (the former is better than the latter in this work). In this work, we quantified the polymer directly improved oxidation of PCE during transport by using a two-dimensional flow tank. Using a low pore volume (≤3.0), the removal rate of the PCE increased with the polymer concentration before stabilizing at approximately 93.00 and 88.30% for xanthan and HPAM, respectively. In this work, over 80% of PCE was removed via less than 3.0 PV of the SDS solution, whereas complete removal (100%) was achieved with less than 3.0 PV of SDS foam. Furthermore, the new experimental discoveries demonstrate that xanthan is better than HPAM and SDS foam is a better remediation agent than the SDS solution for removing PCE.
Graphical abstract (Reaction device, A - inlet device (pump 1#), B - 2D tank, C - outflow device (pump 2#), D - data recording and processing device, E - microscopic expression, E (a) - KMnO4 flushing, E (b) - polymer solution flushing).
Environmental Science and Pollution Research - The cytotoxicity of nanoparticles (NPs) and their properties are important issues in nanotechnology research. Particularly, NPs affect the metabolism... 相似文献